J R R Navodi Jayarathne*, Daniel Zimmerle, Richard S Kolodziej, Stuart Riddick and Kathleen M Smits,
{"title":"地下管道泄漏甲烷的流动和迁移:土壤表面条件的影响及对天然气泄漏分类的意义","authors":"J R R Navodi Jayarathne*, Daniel Zimmerle, Richard S Kolodziej, Stuart Riddick and Kathleen M Smits, ","doi":"10.1021/acs.estlett.4c00039","DOIUrl":null,"url":null,"abstract":"<p >Reducing methane (CH<sub>4</sub>) emissions from natural gas (NG) pipeline leaks is crucial to minimize global warming while also providing key safety benefits to communities. What is not well understood about pipeline leak scenarios is the impact of different soil surface conditions on the belowground leak transport behavior and subsequently the NG leak classification. In this study, we conducted a series of controlled leak experiments, varying based on the surface conditions including snow, moist soil layers, asphalt, and grass. Data indicated that temporary rain and snow surface cover conditions result in CH<sub>4</sub> concentrations extending 3 times further than the equivalent leak scenario under dry soil conditions, resulting in levels that pose heightened environmental and safety risks. Furthermore, after leak termination, CH<sub>4</sub> trapped under snow, moist soil, and asphalt surface conditions persisted for up to ∼12 days, with 5–15% CH<sub>4</sub> (v/v) conditions persisting underground for 7.5 days. Even after leak termination, NG continued to migrate laterally away from the leak source, extending the plume boundary by 2–4%. While efforts to study a wider range of environmental conditions are underway, the findings of this study provide crucial insight into identifying and prioritizing leaks from the perspectives of both safety and the environment.</p>","PeriodicalId":37,"journal":{"name":"Environmental Science & Technology Letters Environ.","volume":"11 6","pages":"539–545"},"PeriodicalIF":8.9000,"publicationDate":"2024-05-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://pubs.acs.org/doi/epdf/10.1021/acs.estlett.4c00039","citationCount":"0","resultStr":"{\"title\":\"Flow and Transport of Methane from Leaking Underground Pipelines: Effects of Soil Surface Conditions and Implications for Natural Gas Leak Classification\",\"authors\":\"J R R Navodi Jayarathne*, Daniel Zimmerle, Richard S Kolodziej, Stuart Riddick and Kathleen M Smits, \",\"doi\":\"10.1021/acs.estlett.4c00039\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Reducing methane (CH<sub>4</sub>) emissions from natural gas (NG) pipeline leaks is crucial to minimize global warming while also providing key safety benefits to communities. What is not well understood about pipeline leak scenarios is the impact of different soil surface conditions on the belowground leak transport behavior and subsequently the NG leak classification. In this study, we conducted a series of controlled leak experiments, varying based on the surface conditions including snow, moist soil layers, asphalt, and grass. Data indicated that temporary rain and snow surface cover conditions result in CH<sub>4</sub> concentrations extending 3 times further than the equivalent leak scenario under dry soil conditions, resulting in levels that pose heightened environmental and safety risks. Furthermore, after leak termination, CH<sub>4</sub> trapped under snow, moist soil, and asphalt surface conditions persisted for up to ∼12 days, with 5–15% CH<sub>4</sub> (v/v) conditions persisting underground for 7.5 days. Even after leak termination, NG continued to migrate laterally away from the leak source, extending the plume boundary by 2–4%. While efforts to study a wider range of environmental conditions are underway, the findings of this study provide crucial insight into identifying and prioritizing leaks from the perspectives of both safety and the environment.</p>\",\"PeriodicalId\":37,\"journal\":{\"name\":\"Environmental Science & Technology Letters Environ.\",\"volume\":\"11 6\",\"pages\":\"539–545\"},\"PeriodicalIF\":8.9000,\"publicationDate\":\"2024-05-09\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://pubs.acs.org/doi/epdf/10.1021/acs.estlett.4c00039\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Environmental Science & Technology Letters Environ.\",\"FirstCategoryId\":\"1\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acs.estlett.4c00039\",\"RegionNum\":2,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, ENVIRONMENTAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Environmental Science & Technology Letters Environ.","FirstCategoryId":"1","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.estlett.4c00039","RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
Flow and Transport of Methane from Leaking Underground Pipelines: Effects of Soil Surface Conditions and Implications for Natural Gas Leak Classification
Reducing methane (CH4) emissions from natural gas (NG) pipeline leaks is crucial to minimize global warming while also providing key safety benefits to communities. What is not well understood about pipeline leak scenarios is the impact of different soil surface conditions on the belowground leak transport behavior and subsequently the NG leak classification. In this study, we conducted a series of controlled leak experiments, varying based on the surface conditions including snow, moist soil layers, asphalt, and grass. Data indicated that temporary rain and snow surface cover conditions result in CH4 concentrations extending 3 times further than the equivalent leak scenario under dry soil conditions, resulting in levels that pose heightened environmental and safety risks. Furthermore, after leak termination, CH4 trapped under snow, moist soil, and asphalt surface conditions persisted for up to ∼12 days, with 5–15% CH4 (v/v) conditions persisting underground for 7.5 days. Even after leak termination, NG continued to migrate laterally away from the leak source, extending the plume boundary by 2–4%. While efforts to study a wider range of environmental conditions are underway, the findings of this study provide crucial insight into identifying and prioritizing leaks from the perspectives of both safety and the environment.
期刊介绍:
Environmental Science & Technology Letters serves as an international forum for brief communications on experimental or theoretical results of exceptional timeliness in all aspects of environmental science, both pure and applied. Published as soon as accepted, these communications are summarized in monthly issues. Additionally, the journal features short reviews on emerging topics in environmental science and technology.