不同类型地质碳封存中的断层渗漏行为与二氧化碳迁移

IF 0.6 4区 工程技术 Q4 ENERGY & FUELS Chemistry and Technology of Fuels and Oils Pub Date : 2024-05-14 DOI:10.1007/s10553-024-01701-1
Jiang Lu, Yanxin Lv, Xiaoyu Fang, Jinsong Zuo, Siyang Wang, Haibo Li, Chao Yuan, Weiji Liu
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引用次数: 0

摘要

地质碳储存被认为是缓解气候危机的有效措施。二氧化碳的封存方法取决于其相态和注入深度。本研究构建了断层-储层系统,以阐明不同地质封存环境下的断层泄漏行为和二氧化碳迁移。二氧化碳是浮还是沉,取决于二氧化碳和水之间的流体密度差。当二氧化碳注入深层含盐含水层时,由于二氧化碳的浮力作用,二氧化碳会沿着断层面优先向上迁移,二氧化碳羽流在盖层岩石下积聚,最终漂浮在储层顶部。在深海储层和火山玄武岩中封存二氧化碳时,没有观察到二氧化碳羽流向上迁移的现象。断层面是海洋二氧化碳封存过程中碳向下迁移的首选途径,提供了几乎无限的环境。与深海封存相比,火山玄武岩的下沉时间更短,因此用于碳封存更安全、更有效。研究表明,二氧化碳和水之间的流体密度差是决定二氧化碳下沉速度的决定性因素。这项寻找二氧化碳沉降储层的研究为移除和储存大量温室气体提供了一个很有前景的替代参考。
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Fault Leakage Behaviors and Co2 Migration in Different Types of Geological Carbon Storage

Geological carbon storage is considered to be an effective measure to mitigate climate crisis. The method in which CO2 is stored depends on its phase state and the depth at which it is injected. In this study, the fault-reservoir system is constructed to elucidate the fault leakage behaviors and CO2 migration in different geological storage environments. Whether CO2 is buoyant or sinking depends on the fluid density difference between CO2 and H2O. When carbon dioxide is injected into deep saline aquifer, CO2 would preferentially migrate upward along the fault plane due to CO2 buoyancy forces, and CO2 plume accumulates beneath the caprock and floats at the top of the reservoir eventually. For CO2 storage in deep ocean reservoir and volcanic basalt, no upward migration of CO2 plume is observed during carbon storage. Fault plane is the preferential pathway for carbon downward transportation during ocean-based CO2 storage, providing a virtually unlimited environment. Compared with deep ocean storage, the much shorter sinking times makes volcanic basalt for carbon storage safer and more effective. It is illustrated that the fluid density difference between CO2 and H2O is the decisive factor in determining CO2 sinking velocity. This investigation of searching CO2 sinking reservoirs provides a promising alterative reference for remove and storage large volumes of the greenhouse gas.

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来源期刊
Chemistry and Technology of Fuels and Oils
Chemistry and Technology of Fuels and Oils 工程技术-工程:化工
CiteScore
0.90
自引率
16.70%
发文量
119
审稿时长
1.0 months
期刊介绍: Chemistry and Technology of Fuels and Oils publishes reports on improvements in the processing of petroleum and natural gas and cracking and refining techniques for the production of high-quality fuels, oils, greases, specialty fluids, additives and synthetics. The journal includes timely articles on the demulsification, desalting, and desulfurizing of crude oil; new flow plans for refineries; platforming, isomerization, catalytic reforming, and alkylation processes for obtaining aromatic hydrocarbons and high-octane gasoline; methods of producing ethylene, acetylene, benzene, acids, alcohols, esters, and other compounds from petroleum, as well as hydrogen from natural gas and liquid products.
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