Jiang Lu, Yanxin Lv, Xiaoyu Fang, Jinsong Zuo, Siyang Wang, Haibo Li, Chao Yuan, Weiji Liu
{"title":"不同类型地质碳封存中的断层渗漏行为与二氧化碳迁移","authors":"Jiang Lu, Yanxin Lv, Xiaoyu Fang, Jinsong Zuo, Siyang Wang, Haibo Li, Chao Yuan, Weiji Liu","doi":"10.1007/s10553-024-01701-1","DOIUrl":null,"url":null,"abstract":"<p>Geological carbon storage is considered to be an effective measure to mitigate climate crisis. The method in which CO<sub>2</sub> is stored depends on its phase state and the depth at which it is injected. In this study, the fault-reservoir system is constructed to elucidate the fault leakage behaviors and CO<sub>2</sub> migration in different geological storage environments. Whether CO<sub>2</sub> is buoyant or sinking depends on the fluid density difference between CO<sub>2</sub> and H<sub>2</sub>O. When carbon dioxide is injected into deep saline aquifer, CO<sub>2</sub> would preferentially migrate upward along the fault plane due to CO<sub>2</sub> buoyancy forces, and CO<sub>2</sub> plume accumulates beneath the caprock and floats at the top of the reservoir eventually. For CO<sub>2</sub> storage in deep ocean reservoir and volcanic basalt, no upward migration of CO<sub>2</sub> plume is observed during carbon storage. Fault plane is the preferential pathway for carbon downward transportation during ocean-based CO<sub>2</sub> storage, providing a virtually unlimited environment. Compared with deep ocean storage, the much shorter sinking times makes volcanic basalt for carbon storage safer and more effective. It is illustrated that the fluid density difference between CO<sub>2</sub> and H<sub>2</sub>O is the decisive factor in determining CO<sub>2</sub> sinking velocity. This investigation of searching CO<sub>2</sub> sinking reservoirs provides a promising alterative reference for remove and storage large volumes of the greenhouse gas.</p>","PeriodicalId":9908,"journal":{"name":"Chemistry and Technology of Fuels and Oils","volume":null,"pages":null},"PeriodicalIF":0.6000,"publicationDate":"2024-05-14","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Fault Leakage Behaviors and Co2 Migration in Different Types of Geological Carbon Storage\",\"authors\":\"Jiang Lu, Yanxin Lv, Xiaoyu Fang, Jinsong Zuo, Siyang Wang, Haibo Li, Chao Yuan, Weiji Liu\",\"doi\":\"10.1007/s10553-024-01701-1\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>Geological carbon storage is considered to be an effective measure to mitigate climate crisis. The method in which CO<sub>2</sub> is stored depends on its phase state and the depth at which it is injected. In this study, the fault-reservoir system is constructed to elucidate the fault leakage behaviors and CO<sub>2</sub> migration in different geological storage environments. Whether CO<sub>2</sub> is buoyant or sinking depends on the fluid density difference between CO<sub>2</sub> and H<sub>2</sub>O. When carbon dioxide is injected into deep saline aquifer, CO<sub>2</sub> would preferentially migrate upward along the fault plane due to CO<sub>2</sub> buoyancy forces, and CO<sub>2</sub> plume accumulates beneath the caprock and floats at the top of the reservoir eventually. For CO<sub>2</sub> storage in deep ocean reservoir and volcanic basalt, no upward migration of CO<sub>2</sub> plume is observed during carbon storage. Fault plane is the preferential pathway for carbon downward transportation during ocean-based CO<sub>2</sub> storage, providing a virtually unlimited environment. Compared with deep ocean storage, the much shorter sinking times makes volcanic basalt for carbon storage safer and more effective. It is illustrated that the fluid density difference between CO<sub>2</sub> and H<sub>2</sub>O is the decisive factor in determining CO<sub>2</sub> sinking velocity. This investigation of searching CO<sub>2</sub> sinking reservoirs provides a promising alterative reference for remove and storage large volumes of the greenhouse gas.</p>\",\"PeriodicalId\":9908,\"journal\":{\"name\":\"Chemistry and Technology of Fuels and Oils\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":0.6000,\"publicationDate\":\"2024-05-14\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Chemistry and Technology of Fuels and Oils\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://doi.org/10.1007/s10553-024-01701-1\",\"RegionNum\":4,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q4\",\"JCRName\":\"ENERGY & FUELS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Chemistry and Technology of Fuels and Oils","FirstCategoryId":"5","ListUrlMain":"https://doi.org/10.1007/s10553-024-01701-1","RegionNum":4,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q4","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
Fault Leakage Behaviors and Co2 Migration in Different Types of Geological Carbon Storage
Geological carbon storage is considered to be an effective measure to mitigate climate crisis. The method in which CO2 is stored depends on its phase state and the depth at which it is injected. In this study, the fault-reservoir system is constructed to elucidate the fault leakage behaviors and CO2 migration in different geological storage environments. Whether CO2 is buoyant or sinking depends on the fluid density difference between CO2 and H2O. When carbon dioxide is injected into deep saline aquifer, CO2 would preferentially migrate upward along the fault plane due to CO2 buoyancy forces, and CO2 plume accumulates beneath the caprock and floats at the top of the reservoir eventually. For CO2 storage in deep ocean reservoir and volcanic basalt, no upward migration of CO2 plume is observed during carbon storage. Fault plane is the preferential pathway for carbon downward transportation during ocean-based CO2 storage, providing a virtually unlimited environment. Compared with deep ocean storage, the much shorter sinking times makes volcanic basalt for carbon storage safer and more effective. It is illustrated that the fluid density difference between CO2 and H2O is the decisive factor in determining CO2 sinking velocity. This investigation of searching CO2 sinking reservoirs provides a promising alterative reference for remove and storage large volumes of the greenhouse gas.
期刊介绍:
Chemistry and Technology of Fuels and Oils publishes reports on improvements in the processing of petroleum and natural gas and cracking and refining techniques for the production of high-quality fuels, oils, greases, specialty fluids, additives and synthetics. The journal includes timely articles on the demulsification, desalting, and desulfurizing of crude oil; new flow plans for refineries; platforming, isomerization, catalytic reforming, and alkylation processes for obtaining aromatic hydrocarbons and high-octane gasoline; methods of producing ethylene, acetylene, benzene, acids, alcohols, esters, and other compounds from petroleum, as well as hydrogen from natural gas and liquid products.