{"title":"电催化将二氧化碳还原为 C4+ 产物","authors":"Xiangyun Ma, Boon Siang Yeo","doi":"10.1016/j.coelec.2024.101534","DOIUrl":null,"url":null,"abstract":"<div><p>Long-chain hydrocarbons and oxygenates are used as fuels as well as in many daily applications. The majority of these molecules are derived from fossil fuels, which is a non-renewable commodity. The electrocatalytic CO<sub>2</sub> reduction reaction (eCO<sub>2</sub>RR) has been recently found promising in producing C<sub>4+</sub> molecules. Herein, we summarize recent works on this topic. The design of C<sub>4+</sub>-producing catalysts is compared with those that produce C<sub>1</sub>–C<sub>3</sub> products. Mechanisms for the C–C coupling step are reviewed.</p></div>","PeriodicalId":11028,"journal":{"name":"Current Opinion in Electrochemistry","volume":"46 ","pages":"Article 101534"},"PeriodicalIF":7.9000,"publicationDate":"2024-05-10","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Electrocatalytic reduction of carbon dioxide to C4+ products\",\"authors\":\"Xiangyun Ma, Boon Siang Yeo\",\"doi\":\"10.1016/j.coelec.2024.101534\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Long-chain hydrocarbons and oxygenates are used as fuels as well as in many daily applications. The majority of these molecules are derived from fossil fuels, which is a non-renewable commodity. The electrocatalytic CO<sub>2</sub> reduction reaction (eCO<sub>2</sub>RR) has been recently found promising in producing C<sub>4+</sub> molecules. Herein, we summarize recent works on this topic. The design of C<sub>4+</sub>-producing catalysts is compared with those that produce C<sub>1</sub>–C<sub>3</sub> products. Mechanisms for the C–C coupling step are reviewed.</p></div>\",\"PeriodicalId\":11028,\"journal\":{\"name\":\"Current Opinion in Electrochemistry\",\"volume\":\"46 \",\"pages\":\"Article 101534\"},\"PeriodicalIF\":7.9000,\"publicationDate\":\"2024-05-10\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Current Opinion in Electrochemistry\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2451910324000954\",\"RegionNum\":2,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Current Opinion in Electrochemistry","FirstCategoryId":"92","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2451910324000954","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Electrocatalytic reduction of carbon dioxide to C4+ products
Long-chain hydrocarbons and oxygenates are used as fuels as well as in many daily applications. The majority of these molecules are derived from fossil fuels, which is a non-renewable commodity. The electrocatalytic CO2 reduction reaction (eCO2RR) has been recently found promising in producing C4+ molecules. Herein, we summarize recent works on this topic. The design of C4+-producing catalysts is compared with those that produce C1–C3 products. Mechanisms for the C–C coupling step are reviewed.
期刊介绍：
The development of the Current Opinion journals stemmed from the acknowledgment of the growing challenge for specialists to stay abreast of the expanding volume of information within their field. In Current Opinion in Electrochemistry, they help the reader by providing in a systematic manner:
1.The views of experts on current advances in electrochemistry in a clear and readable form.
2.Evaluations of the most interesting papers, annotated by experts, from the great wealth of original publications.
In the realm of electrochemistry, the subject is divided into 12 themed sections, with each section undergoing an annual review cycle:
• Bioelectrochemistry • Electrocatalysis • Electrochemical Materials and Engineering • Energy Storage: Batteries and Supercapacitors • Energy Transformation • Environmental Electrochemistry • Fundamental & Theoretical Electrochemistry • Innovative Methods in Electrochemistry • Organic & Molecular Electrochemistry • Physical & Nano-Electrochemistry • Sensors & Bio-sensors •
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