设计和制造靶向配位聚合物/MOFs 的基本概念的历史发展:个人经历。

IF 7 2区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Chemical record Pub Date : 2024-05-22 DOI:10.1002/tcr.202400038
Richard Robson
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摘要

本文介绍了配位聚合物/MOFs 设计和构建的基本思想和概念的历史发展过程--从 20 世纪 70 年代关于使用预组织构件构建目标聚合物结构的可能性的最早猜想,到 80 年代中期这些思想的初步实验实施,再到 90 年代 MOFs 名称的引入。本文所描述的对预组织构筑模块的早期探索工作,为随后 CP/MOF 领域研究活动的爆炸式增长,以及有望产生具有各种有用特性的无限范围的设计配位聚合物结构铺平了道路。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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The Historical Development of the Concepts Underlying the Design and Construction of Targeted Coordination Polymers/MOFs: A Personal Account

Presented here is a personal account of how the ideas and concepts underlying the design and construction of coordination polymers/MOFs developed historically - from the earliest conjectures in the 1970’s about the possibility of using pre-organized building blocks to construct targeted polymeric structures, to the initial experimental implementation of these ideas in the mid-80’s and to the introduction of the name MOFs in the 90’s. The early exploratory work with pre-organized building blocks described in this article paved the way for the subsequent explosion of research activity in the CP/MOF area and for the generation of an essentially unlimited range of designed coordination polymer structures promising a variety of useful properties.

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来源期刊
Chemical record
Chemical record 化学-化学综合
CiteScore
11.00
自引率
3.00%
发文量
188
审稿时长
>12 weeks
期刊介绍: The Chemical Record (TCR) is a "highlights" journal publishing timely and critical overviews of new developments at the cutting edge of chemistry of interest to a wide audience of chemists (2013 journal impact factor: 5.577). The scope of published reviews includes all areas related to physical chemistry, analytical chemistry, inorganic chemistry, organic chemistry, polymer chemistry, materials chemistry, bioorganic chemistry, biochemistry, biotechnology and medicinal chemistry as well as interdisciplinary fields. TCR provides carefully selected highlight papers by leading researchers that introduce the author''s own experimental and theoretical results in a framework designed to establish perspectives with earlier and contemporary work and provide a critical review of the present state of the subject. The articles are intended to present concise evaluations of current trends in chemistry research to help chemists gain useful insights into fields outside their specialization and provide experts with summaries of recent key developments.
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