银簇组装材料:模型驱动的最新进展视角,聚焦 Ag12 簇组装。

IF 7 2区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Chemical record Pub Date : 2024-05-22 DOI:10.1002/tcr.202400052
Dr. Sourav Biswas, Prof. Yuichi Negishi
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引用次数: 0

摘要

尽管存在稳定性问题,对单个纳米团簇的探索仍在迅速推进。为了应对这一挑战,通过连接分子组装簇节点的方法已经成功实现。然而,簇节点的连接本身带来了多种可能性,尤其是当其他因素发挥作用时。虽然这种方法被证明能有效提高材料的稳定性,但其成功背后的具体原因仍然难以捉摸。在我们的实验室中,我们已经对琼脂簇组装材料进行了广泛的研究。因此,我们的目标是建立一个模型系统,以便对各种因素进行辨别,消除连接方法中不必要的复杂性。因此,我们希望在此提出的系统论述将对未来的工作做出重大贡献,帮助确定明确的优先事项,并为使用模型系统时出现的问题提供解决方案。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Silver Cluster Assembled Materials: A Model-Driven Perspective on Recent Progress, with a Spotlight on Ag12 Cluster Assembly

The exploration of individual nanoclusters is rapidly advancing, despite stability concerns. To address this challenge, the assembly of cluster nodes through linker molecules has been successfully implemented. However, the linking of the cluster nodes itself introduces a multitude of possibilities, especially when additional factors come into play. While this method proves effective in enhancing material stability, the specific reasons behind its success remain elusive. In our laboratory, we have undertaken extensive studies on Ag cluster-assembled materials. So, here our goal is to establish a model system that allows for the discernment of various factors, eliminating unnecessary complexities during the linking approach. So, we hope that the systematic discourse presented in here will contribute significantly to future endeavors, helping to set clear priorities, and provide solutions to concerns that arise when working with a model system.

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来源期刊
Chemical record
Chemical record 化学-化学综合
CiteScore
11.00
自引率
3.00%
发文量
188
审稿时长
>12 weeks
期刊介绍: The Chemical Record (TCR) is a "highlights" journal publishing timely and critical overviews of new developments at the cutting edge of chemistry of interest to a wide audience of chemists (2013 journal impact factor: 5.577). The scope of published reviews includes all areas related to physical chemistry, analytical chemistry, inorganic chemistry, organic chemistry, polymer chemistry, materials chemistry, bioorganic chemistry, biochemistry, biotechnology and medicinal chemistry as well as interdisciplinary fields. TCR provides carefully selected highlight papers by leading researchers that introduce the author''s own experimental and theoretical results in a framework designed to establish perspectives with earlier and contemporary work and provide a critical review of the present state of the subject. The articles are intended to present concise evaluations of current trends in chemistry research to help chemists gain useful insights into fields outside their specialization and provide experts with summaries of recent key developments.
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