基于金属有机框架的锂离子电池和超级电容器材料的构建和应用最新进展

Dan Wei, Lingling Zhang, Yiming Wang, Shujun Qiu, Yumei Luo, Yongjin Zou, Fen Xu, Lixian Sun, Hailiang Chu
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摘要

金属有机框架(MOFs)是一种由有机多位连接体和金属节点组成的特殊三维结晶多孔晶格,具有独特的多孔性和高比表面积的特点,近年来作为电化学储能器件的电极材料引起了广泛的兴趣。在这篇论文中,我们概述了目前在原始 MOFs、MOF 复合材料和 MOF 衍生物的构建及其在超级电容器 (SC) 和锂离子电池 (LIB) 中作为电极材料的应用方面的研究进展。具体而言,我们讨论了基于 MOFs 的 SC 和 LIB 电极材料的不足之处。我们还详细介绍了通过将 MOFs 与其他导电材料相结合以及将 MOFs 衍生为金属硫化物、金属氧化物、金属磷化物和多孔碳来提高性能的创新工作。最后,我们初步展望了未来在掌握潜在机制方面所面临的挑战。这篇综述将为电化学储能领域基于 MOFs 的电极材料的开发和应用带来更多启发。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Recent progress on construction and applications of metal-organic frameworks-based materials for lithium-ion batteries and supercapacitors

Metal-organic frameworks (MOFs), a special sort of three-dimensional crystalline porous lattices composed of organic multi-site connectors and metal nodes, are characterized by unique porosity and high specific surface area, which have attracted a wide range of interest as electrode materials for the electrochemical energy storage devices in recent years. In this contribution, we outline the current research progress on the construction of pristine MOFs, MOF composites, and MOF derivatives and their applications as electrode materials in supercapacitors (SCs) and lithium-ion batteries (LIBs). Specifically, we discuss the shortcomings of MOFs-based electrode materials for SCs and LIBs. The innovative work on performance improvements by combining MOFs with other conductive materials and derivating MOFs into metal sulfides, metal oxides, metal phosphides, and porous carbon is also presented in detail. Finally, our perspectives on the challenges in the future for a grasp of the potential mechanisms are tentatively provided. This review will inspire more developments and applications of MOFs-based electrode materials for electrochemical energy storage.

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Issue Information Front Cover: Carbon Neutralization, Volume 3, Issue 6, November 2024 Inside Back Cover Image: Carbon Neutralization, Volume 3, Issue 6, November 2024 Back Cover Image: Carbon Neutralization, Volume 3, Issue 6, November 2024 A chronicle of titanium niobium oxide materials for high-performance lithium-ion batteries: From laboratory to industry
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