FeTe0.55Se0.45 中拓扑带状结构的轨道成分和持久狄拉克表面态

IF 11.6 1区 物理与天体物理 Q1 PHYSICS, MULTIDISCIPLINARY Physical Review X Pub Date : 2024-06-11 DOI:10.1103/physrevx.14.021043
Y.-F. Li, S.-D. Chen, M. García-Díez, M. I. Iraola, H. Pfau, Y.-L. Zhu, Z.-Q. Mao, T. Chen, M. Yi, P.-C. Dai, J. A. Sobota, M. Hashimoto, M. G. Vergniory, D.-H. Lu, Z.-X. Shen
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引用次数: 0

摘要

FeTe0.55Se0.45(FTS)在现代凝聚态物理学中占据了一个特殊的位置,它是电子相关性、拓扑学和非常规超导性的交叉点。由于沿Γ-Z方向的dxz带和pz带之间的带反转,FTS的体电子结构被预测为拓扑非三维的。然而,在狄拉克表面态(DSS)的真实性以及带状结构与理论带反转图的实验偏差方面仍然存在争论。在这里,我们通过全面的角度分辨光发射光谱研究来解决这些争论。我们首先观察到了与 kz 无关的持久性 DSS。然后,通过将 FTS 与沿 Γ-Z 没有波段反转的 FeSe 进行比较,我们确定了 pz 波段的存在以及 dxz 波段和 pz 波段之间反转的光谱重量指纹。此外,我们还在保持晶体对称性的紧密结合模型框架下,提出了带状结构的重正化方案。我们的研究结果强调了相关性对改变带状结构的重要影响,并有力地证明了这种非常规超导体中拓扑带状结构的存在。
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Orbital Ingredients and Persistent Dirac Surface State for the Topological Band Structure in FeTe0.55Se0.45
FeTe0.55Se0.45 (FTS) occupies a special spot in modern condensed matter physics at the intersections of electron correlation, topology, and unconventional superconductivity. The bulk electronic structure of FTS is predicted to be topologically nontrivial due to the band inversion between the dxz and pz bands along ΓZ. However, there remain debates in both the authenticity of the Dirac surface states (DSSs) and the experimental deviations of band structure from the theoretical band inversion picture. Here we resolve these debates through a comprehensive angle-resolved photoemission spectroscopy investigation. We first observe a persistent DSS independent of kz. Then, by comparing FTS with FeSe, which has no band inversion along ΓZ, we identify the spectral weight fingerprint of both the presence of the pz band and the inversion between the dxz and pz bands. Furthermore, we propose a renormalization scheme for the band structure under the framework of a tight-binding model preserving crystal symmetry. Our results highlight the significant influence of correlation on modifying the band structure and make a strong case for the existence of topological band structure in this unconventional superconductor.
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来源期刊
Physical Review X
Physical Review X PHYSICS, MULTIDISCIPLINARY-
CiteScore
24.60
自引率
1.60%
发文量
197
审稿时长
3 months
期刊介绍: Physical Review X (PRX) stands as an exclusively online, fully open-access journal, emphasizing innovation, quality, and enduring impact in the scientific content it disseminates. Devoted to showcasing a curated selection of papers from pure, applied, and interdisciplinary physics, PRX aims to feature work with the potential to shape current and future research while leaving a lasting and profound impact in their respective fields. Encompassing the entire spectrum of physics subject areas, PRX places a special focus on groundbreaking interdisciplinary research with broad-reaching influence.
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