C56 类富勒烯结构的磁性和磁致性:蒙特卡罗研究

S. Idrissi, A. Jabar, L. Bahmad
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摘要

我们探索了由混合自旋 2 和 3/2 形成的 C56 富勒烯类体系的磁性和磁致性。我们使用 Metropolis 算法进行了蒙特卡罗模拟,并展示了不同物理参数的影响。我们还建立了零还原温度下不同平面的基态相图,这些平面由还原的外部磁场、还原的混合自旋之间的耦合相互作用以及还原的晶体场形成。我们发现,总磁化率预示了一个特定的还原临界温度值,这一点通过在磁感应强度中观察到的峰值得到了证实。为了阐明 C56 体系的磁熵变化 -ΔSm 的行为,在几个外磁场值下,我们发现还原临界温度值 tC 随还原外磁场的增加而增加。此外,我们还展示了最大 "磁熵变 "与还原外磁场的函数关系。我们发现,当增加外磁场降低值时,该参数几乎呈线性增长。所研究系统的磁滞周期显示,晶体场减小后,磁滞表面周期以及相应的减小矫顽磁场值随之减小。
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Magnetic and Magnetocaloric Properties of C56 like-Fullerene Structure: A Monte Carlo Study
We explored the magnetic and magnetocaloric properties of the C56 Fullerene-like system formed by the mixed spins 2 and 3/2. We applied Monte Carlo simulations using the Metropolis algorithm and show the effects of different physical parameters. We also established the ground state phase diagrams, at zero reduced temperature, in different planes formed by the reduced external magnetic field, the reduced coupling interaction between the mixed spins, and the reduced crystal field. We found that the total magnetizations predict a specific reduced critical temperature value, confirmed by the peaks observed in the magnetic susceptibilities. To elucidate the behavior of the magnetic entropy changes -ΔSm, of the C56 system, for several external magnetic field values we show that the reduced critical temperature value tC increases when increasing the reduced external magnetic field. In addition, we show the dependency of the maximum “magnetic entropy change” as a function of the reduced external magnetic field. We found an almost linear increase for this parameter when increasing the reduced external magnetic field values. The obtained hysteresis cycles of the studied system showed a decreasing effect of the reduced crystal field followed by a decrease of the magnetic hysteresis surface cycles, as well as the corresponding reduced coercive magnetic field values.
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