{"title":"电感应加热促进液态氢化有机物的可持续利用","authors":"","doi":"10.1016/j.joule.2024.05.020","DOIUrl":null,"url":null,"abstract":"<div><p>We propose the electrified catalytic inductive heating<span><span> system (ECIHS), which utilizes electromagnetic induction heating (IH) of a monolithic catalytic composite to induce direct and efficient heat transfer to the liquid-phase reaction environment. Herein, we demonstrated that the ECIHS could be utilized to extract hydrogen from liquid-phase perhydro-dibenzyltoluene (H18-DBT) within just 3.5 s, accounting for a 16.4-fold improvement in the reaction rate compared with conventional heating methods. This remarkable observation underscores the potential of the ECIHS for on-site hydrogen utilization, empowering various advanced applications such as hydrogen-powered vehicles. Furthermore, the capabilities of the ECIHS for efficient heat and mass transfer in the </span>liquid phase<span> are also translatable to a myriad of different chemical processing schemes with high industrial value. Overall, the ECIHS represents a major breakthrough in the development of sustainable chemical processing methods, further propelling efforts to achieve full decarbonization in the global chemical processing industry.</span></span></p></div>","PeriodicalId":343,"journal":{"name":"Joule","volume":"8 8","pages":"Pages 2374-2392"},"PeriodicalIF":38.6000,"publicationDate":"2024-08-21","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Electrified inductive heating for sustainable utilization of liquid hydrogenated organics\",\"authors\":\"\",\"doi\":\"10.1016/j.joule.2024.05.020\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>We propose the electrified catalytic inductive heating<span><span> system (ECIHS), which utilizes electromagnetic induction heating (IH) of a monolithic catalytic composite to induce direct and efficient heat transfer to the liquid-phase reaction environment. Herein, we demonstrated that the ECIHS could be utilized to extract hydrogen from liquid-phase perhydro-dibenzyltoluene (H18-DBT) within just 3.5 s, accounting for a 16.4-fold improvement in the reaction rate compared with conventional heating methods. This remarkable observation underscores the potential of the ECIHS for on-site hydrogen utilization, empowering various advanced applications such as hydrogen-powered vehicles. Furthermore, the capabilities of the ECIHS for efficient heat and mass transfer in the </span>liquid phase<span> are also translatable to a myriad of different chemical processing schemes with high industrial value. Overall, the ECIHS represents a major breakthrough in the development of sustainable chemical processing methods, further propelling efforts to achieve full decarbonization in the global chemical processing industry.</span></span></p></div>\",\"PeriodicalId\":343,\"journal\":{\"name\":\"Joule\",\"volume\":\"8 8\",\"pages\":\"Pages 2374-2392\"},\"PeriodicalIF\":38.6000,\"publicationDate\":\"2024-08-21\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Joule\",\"FirstCategoryId\":\"88\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S2542435124002484\",\"RegionNum\":1,\"RegionCategory\":\"材料科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, PHYSICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Joule","FirstCategoryId":"88","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S2542435124002484","RegionNum":1,"RegionCategory":"材料科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, PHYSICAL","Score":null,"Total":0}
Electrified inductive heating for sustainable utilization of liquid hydrogenated organics
We propose the electrified catalytic inductive heating system (ECIHS), which utilizes electromagnetic induction heating (IH) of a monolithic catalytic composite to induce direct and efficient heat transfer to the liquid-phase reaction environment. Herein, we demonstrated that the ECIHS could be utilized to extract hydrogen from liquid-phase perhydro-dibenzyltoluene (H18-DBT) within just 3.5 s, accounting for a 16.4-fold improvement in the reaction rate compared with conventional heating methods. This remarkable observation underscores the potential of the ECIHS for on-site hydrogen utilization, empowering various advanced applications such as hydrogen-powered vehicles. Furthermore, the capabilities of the ECIHS for efficient heat and mass transfer in the liquid phase are also translatable to a myriad of different chemical processing schemes with high industrial value. Overall, the ECIHS represents a major breakthrough in the development of sustainable chemical processing methods, further propelling efforts to achieve full decarbonization in the global chemical processing industry.
期刊介绍:
Joule is a sister journal to Cell that focuses on research, analysis, and ideas related to sustainable energy. It aims to address the global challenge of the need for more sustainable energy solutions. Joule is a forward-looking journal that bridges disciplines and scales of energy research. It connects researchers and analysts working on scientific, technical, economic, policy, and social challenges related to sustainable energy. The journal covers a wide range of energy research, from fundamental laboratory studies on energy conversion and storage to global-level analysis. Joule aims to highlight and amplify the implications, challenges, and opportunities of novel energy research for different groups in the field.