全球人为汞排放情景

IF 5.2 1区 地球科学 Q1 ENVIRONMENTAL SCIENCES Atmospheric Chemistry and Physics Pub Date : 2024-06-27 DOI:10.5194/acp-24-7385-2024
Flora Maria Brocza, Peter Rafaj, Robert Sander, Fabian Wagner, Jenny Marie Jones
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引用次数: 0

摘要

摘要人为排放到大气中的汞(Hg)是对人类和环境健康的长期危害。联合国《汞问题水俣公约》正寻求通过一系列政策,从禁止某些汞用途到减少不同活动中无意释放的汞,来降低人为汞排放。除了独立的汞政策外,减少温室气体、颗粒物(PM)和二氧化硫的战略也可以降低汞排放,从而带来共同利益。本研究利用温室气体-空气污染互动与协同作用(GAINS)模型,研究了不同的清洁空气和气候政策对未来全球汞排放的影响。基准情景假定了当前的能源使用和汞排放趋势,以及当前的清洁空气立法、汞政策和气候政策。此外,我们还探讨了《水俣公约》的影响、气候和严格空气污染政策的共同效益以及最大可行的汞减排措施。由于全球化石燃料和传统生物质使用量的减少,2050 年前的汞排放预测显示,所有情景下燃烧部门的汞排放都有明显减少,基线减排量为 33%,如果将严格的气候控制和最有效的汞控制结合起来,减排量可达 90%。在当前空气污染政策下,水泥和有色金属的排放量在所有情景下都会增加,但如果采取针对汞的严格措施,到 2050 年可分别减少 72% 和 46%。其他排放物(包括废弃物)是本研究中一个重要的不确定来源,根据气候和清洁空气政策的不同,其预测值在 2050 年增加 22% 到减少 54% 之间。汞减排的绝对潜力最大,但绝对排放量的不确定性也最大的领域是小规模和手工黄金生产,在这一领域,减排措施可消除 601-1371 吨(95% 置信区间)的汞年排放量,但估计值的不确定性非常高,可能会使所有其他领域的减排努力黯然失色。总的来说,90% 的汞排放都在《水俣公约》的规定范围内。总之,研究结果表明,除了严格的气候、可吸入颗粒物和二氧化硫政策外,还必须实施有针对性的汞控制政策,以实现汞排放的大幅减少。
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Global scenarios of anthropogenic mercury emissions
Abstract. Anthropogenic mercury (Hg) emissions to the atmosphere are a long-lived hazard to human and environmental health. The UN Minamata Convention on Mercury is seeking to lower anthropogenic mercury emissions through a mix of policies from banning certain Hg uses to reducing unintentional Hg release from different activities. In addition to independent Hg policy, strategies to mitigate greenhouse gases, particulate matter (PM) and SO2 may also lower Hg emissions as a co-benefit. This study uses the Greenhouse Gas–Air Pollution Interactions and Synergies (GAINS) model to examine the effect of different clean air and climate policies on future global Hg emissions. The baseline scenario assumes current trends for energy use and Hg emissions as well as current legislation for clean air, mercury and climate policy. In addition, we explore the impact of the Minamata Convention, the co-benefits of climate and stringent air pollution policies, and maximum feasible reduction measures for Hg. Hg emission projections until 2050 show noticeable reductions in combustion sectors for all scenarios due to a decrease in global fossil fuel and traditional biomass use, leading to emission reductions of 33 % at baseline and up to 90 % when combining stringent climate controls and the most efficient Hg controls. Cement and non-ferrous metal emissions increase in all scenarios with current air pollution policy but could be reduced by up to 72 % and 46 %, respectively, in 2050 with stringent Hg-specific measures. Other emissions (including waste) are a significant source of uncertainty in this study, and their projections range between a 22 % increase and a 54 % decrease in 2050, depending on both climate and clean air policy. The largest absolute reduction potential for Hg abatement but also the largest uncertainties regarding absolute emissions lie in small-scale and artisanal gold production, where abatement measures could eliminate annual Hg emissions in the range of 601–1371 t (95 % confidence interval), although the uncertainties in the estimate are so high that they might eclipse reduction efforts in all other sectors. In total, 90 % of Hg emissions are covered by provisions of the Minamata Convention. Overall, the findings emphasize the necessity to implement targeted Hg control policies in addition to stringent climate, PM and SO2 policies to achieve significant reductions in Hg emissions.
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来源期刊
Atmospheric Chemistry and Physics
Atmospheric Chemistry and Physics 地学-气象与大气科学
CiteScore
10.70
自引率
20.60%
发文量
702
审稿时长
6 months
期刊介绍: Atmospheric Chemistry and Physics (ACP) is a not-for-profit international scientific journal dedicated to the publication and public discussion of high-quality studies investigating the Earth''s atmosphere and the underlying chemical and physical processes. It covers the altitude range from the land and ocean surface up to the turbopause, including the troposphere, stratosphere, and mesosphere. The main subject areas comprise atmospheric modelling, field measurements, remote sensing, and laboratory studies of gases, aerosols, clouds and precipitation, isotopes, radiation, dynamics, biosphere interactions, and hydrosphere interactions. The journal scope is focused on studies with general implications for atmospheric science rather than investigations that are primarily of local or technical interest.
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