整合移动和固定地点黑碳测量,弥合城市空气质量的时空差距。

IF 10.8 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL 环境科学与技术 Pub Date : 2024-07-01 DOI:10.1021/acs.est.3c10829
Chirag Manchanda, Robert A Harley, Julian D Marshall, Alexander J Turner, Joshua S Apte
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引用次数: 0

摘要

城市空气污染在空间和时间上会有很大的变化。然而,很少有监测策略能同时解决精细尺度的时空变化问题。在这里,我们提出了一种新的测量驱动时空建模方法,它超越了移动监测和固定地点传感器网络这两种互补采样范例的各自局限性。我们利用在加利福尼亚州西奥克兰市进行的为期 100 天的密集实地研究数据,开发、验证并应用该模型预测黑碳 (BC)。我们的时空模型利用从多污染物移动监测活动中得出的连贯空间模式,填补了低成本传感器网络中时间完整的黑碳数据的空间空白。我们的模型在重建精细时空分辨率(30 米,15 分钟)的模式方面表现出色,在移动(Pearson's R ∼ 0.77)和固定地点测量(R ∼ 0.95)方面都显示出很强的样本外相关性,同时揭示了单一监测方法无法有效捕捉的特征。该模型揭示了主要排放源附近的急剧浓度梯度,同时捕捉到了这些梯度的时间变化,为了解污染来源和动态提供了宝贵的信息。
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Integrating Mobile and Fixed-Site Black Carbon Measurements to Bridge Spatiotemporal Gaps in Urban Air Quality.

Urban air pollution can vary sharply in space and time. However, few monitoring strategies can concurrently resolve spatial and temporal variation at fine scales. Here, we present a new measurement-driven spatiotemporal modeling approach that transcends the individual limitations of two complementary sampling paradigms: mobile monitoring and fixed-site sensor networks. We develop, validate, and apply this model to predict black carbon (BC) using data from an intensive, 100-day field study in West Oakland, CA. Our spatiotemporal model exploits coherent spatial patterns derived from a multipollutant mobile monitoring campaign to fill spatial gaps in time-complete BC data from a low-cost sensor network. Our model performs well in reconstructing patterns at fine spatial and temporal resolution (30 m, 15 min), demonstrating strong out-of-sample correlations for both mobile (Pearson's R ∼ 0.77) and fixed-site measurements (R ∼ 0.95) while revealing features that are not effectively captured by a single monitoring approach in isolation. The model reveals sharp concentration gradients near major emission sources while capturing their temporal variability, offering valuable insights into pollution sources and dynamics.

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来源期刊
环境科学与技术
环境科学与技术 环境科学-工程:环境
CiteScore
17.50
自引率
9.60%
发文量
12359
审稿时长
2.8 months
期刊介绍: Environmental Science & Technology (ES&T) is a co-sponsored academic and technical magazine by the Hubei Provincial Environmental Protection Bureau and the Hubei Provincial Academy of Environmental Sciences. Environmental Science & Technology (ES&T) holds the status of Chinese core journals, scientific papers source journals of China, Chinese Science Citation Database source journals, and Chinese Academic Journal Comprehensive Evaluation Database source journals. This publication focuses on the academic field of environmental protection, featuring articles related to environmental protection and technical advancements.
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