Muhammad Asim Mushtaq, Muhammad Ahmad, Attia Shaheen, Andleeb Mehmood, Ghulam Yasin, Muhammad Arif, Zahid Ali, Pengyan Li, Sumaira Nazar Hussain, Mohammad Tabish, Anuj Kumar, Saira Ajmal, Waseem Raza, Mansoor Akhtar, Ali Saad and Dongpeng Yan*,
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Advancing the Development of Hollow Micro/nanostructured Materials for Electrocatalytic Water Splitting: Current State, Challenges, and Perspectives
Electrocatalytic water splitting is commonly regarded as a sustainable and clean method to generate hydrogen and oxygen, which is deemed to be efficient for the utilization of renewable energy. Electrocatalysts are essential components to enhance electrochemical efficiency and optimize product yield. Hollow micro/nanostructures possess large specific surface areas, multiple voids, and tunable chemical compositions, making them suitable for use as direct catalysts or as supports for electrochemical reactions. This review summarizes recent advancements in structural and functional designs of micro/nanostructured hollow materials as electrocatalysts for an enhanced water-splitting process. We emphasize ideas and strategies to create various hollow electrocatalysts for oxygen/hydrogen evolution processes. Subsequently, a comprehensive summary of recent studies on hollow borides, carbides, oxides, phosphides, selenides, sulfides, alloys, MXenes, and various heterostructured electrocatalysts containing hollow hosts is provided. Furthermore, we highlight the current challenges and perspectives of hollow micro/nanostructures for electrocatalytic water splitting.
期刊介绍：
ACS Materials Letters is a journal that publishes high-quality and urgent papers at the forefront of fundamental and applied research in the field of materials science. It aims to bridge the gap between materials and other disciplines such as chemistry, engineering, and biology. The journal encourages multidisciplinary and innovative research that addresses global challenges. Papers submitted to ACS Materials Letters should clearly demonstrate the need for rapid disclosure of key results. The journal is interested in various areas including the design, synthesis, characterization, and evaluation of emerging materials, understanding the relationships between structure, property, and performance, as well as developing materials for applications in energy, environment, biomedical, electronics, and catalysis. The journal has a 2-year impact factor of 11.4 and is dedicated to publishing transformative materials research with fast processing times. The editors and staff of ACS Materials Letters actively participate in major scientific conferences and engage closely with readers and authors. The journal also maintains an active presence on social media to provide authors with greater visibility.
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