关于在层流火焰中利用角光散射进行烟尘测定的信号捕获考虑

IF 3.9 3区 环境科学与生态学 Q2 ENGINEERING, CHEMICAL Journal of Aerosol Science Pub Date : 2024-06-22 DOI:10.1016/j.jaerosci.2024.106429
M. Littin , A. Poux , G. Lefevre , M. Mazur , A. Fuentes , J. Yon
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引用次数: 0

摘要

众所周知,烟尘颗粒对健康和环境有害,减少工业系统中的烟尘颗粒产生量是实现绿色能源生产的一项重要任务。对这些微粒进行表征和精确建模至关重要,但也十分复杂。特别是,有关聚合体大小的信息仍然有限。角光散射是一种成熟的现场方法,可对烟尘聚集体进行精确、空间分辨和非侵入式表征。然而,相关的后处理容易产生各种误差。具体来说,光散射过程中的信号捕获可能会导致重大误差。此外,目前重建视线综合散射信号(阿贝尔反演)的技术本身就存在噪声。为了解决这两个问题,这项研究采用了一种基于片断样条函数的无噪声阿贝尔反演方法。该方法考虑了信号捕获,可应用于任何轴对称和空间连续的火焰。信号捕获效应的校正依赖于视线衰减(LOSA)的消光测量。该技术在五个不同角度的典型层流扩散乙烯火焰上进行了测试。评估了这种修正对等效单分散回旋半径(表示为 Rg∗)和前向散射系数(表示为 κvv(0∘))的影响。结果表明,Rg∗ 的计算对信号捕获效应是稳健的。但是,如果对这种效应进行校正,κvv(0∘)就会显著增加。
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On the consideration of signal trapping for soot sizing by angular light scattering in laminar flames

Soot particles are known to be harmful to health and the environment, and reducing their production in industrial systems is a crucial task in the pursuit of green energy production. Characterization and accurate modeling of these particles are essential yet complex. In particular, information on aggregate sizing remains limited. Angular light scattering is an established in-situ method for precise, spatially resolved, non-intrusive characterization of soot aggregates. However, the associated post-processing is prone to various error sources. Specifically, signal trapping during light scattering is suspected to lead significant errors. Moreover, current techniques for reconstructing the line-of-sight integrated scattering signal (Abel inversion) are inherently noisy. This work addresses both issues by implementing a noise-free Abel inversion method based on piecewise spline functions. This method accounts for signal trapping and can be applied to any axisymmetric and spatially continuous flame. The correction for the signal trapping effect relies on extinction measurements from the line-of-sight attenuation (LOSA). The technique is tested on a canonical laminar diffusion ethylene flame at five different angles. The impact of this correction is evaluated on the equivalent monodisperse radius of gyration, denoted as Rg, and the forward scattering coefficient, represented as κvv(0). The results show that the calculation of Rg is robust regarding signal trapping effect. However, correcting for this effect significantly increases κvv(0).

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来源期刊
Journal of Aerosol Science
Journal of Aerosol Science 环境科学-工程:化工
CiteScore
8.80
自引率
8.90%
发文量
127
审稿时长
35 days
期刊介绍: Founded in 1970, the Journal of Aerosol Science considers itself the prime vehicle for the publication of original work as well as reviews related to fundamental and applied aerosol research, as well as aerosol instrumentation. Its content is directed at scientists working in engineering disciplines, as well as physics, chemistry, and environmental sciences. The editors welcome submissions of papers describing recent experimental, numerical, and theoretical research related to the following topics: 1. Fundamental Aerosol Science. 2. Applied Aerosol Science. 3. Instrumentation & Measurement Methods.
期刊最新文献
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