从太空监测欧洲人为氮氧化物排放情况

IF 5.2 1区 地球科学 Q1 ENVIRONMENTAL SCIENCES Atmospheric Chemistry and Physics Pub Date : 2024-07-03 DOI:10.5194/acp-24-7523-2024
Ronald J. van der A, Jieying Ding, Henk Eskes
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引用次数: 0

摘要

摘要。自从哨兵-5 号前体(S5P)卫星上的 TROPOMI 发射以来,二氧化氮观测数据的分辨率达到了 3.5×5 千米,这使得监测城市地区和工业设施规模的氮氧化物排放成为可能。在欧洲,每年都会报告国家总量和大型工业设施的排放量,并通过欧洲环境署(EEA)向公众公布。卫星观测可提供独立且更及时的氮氧化物排放信息。新版本的反演算法 DECSO(受卫星观测约束的每日排放量)已经开发出来,用于推导欧洲的每日排放量,并平均到月平均值地图上。据估计,单个网格单元的月排放量精度约为 25%。这些来自 DECSO 的卫星排放量已与官方报告的欧洲排放量和时空分类排放清单进行了比较。DECSO 的国家氮氧化物排放总量接近于报告的排放量和哥白尼大气监测服务(CAMS)编制的排放量。对 DECSO 和哥白尼大气监测服务的氮氧化物排放量的空间分布进行比较后发现,卫星得出的排放量在城市通常较高,而在大型发电厂则相似,在农村地区略低。
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Monitoring European anthropogenic NOx emissions from space
Abstract. Since the launch of TROPOMI on the Sentinel-5 Precursor (S5P) satellite, NO2 observations have become available with a resolution of 3.5× 5 km, which makes monitoring NOx emissions possible at the scale of city districts and industrial facilities. For Europe, emissions are reported on an annual basis for country totals and large industrial facilities and made publicly available via the European Environment Agency (EEA). Satellite observations can provide independent and more timely information on NOx emissions. A new version of the inversion algorithm DECSO (Daily Emissions Constrained by Satellite Observations) has been developed for deriving emissions for Europe on a daily basis, averaged to monthly mean maps. The estimated precision of these monthly emissions is about 25 % for individual grid cells. These satellite-derived emissions from DECSO have been compared to the officially reported European emissions and spatial–temporal disaggregated emission inventories. The country total DECSO NOx emissions are close to the reported emissions and the emissions compiled by the Copernicus Atmosphere Monitoring Service (CAMS). Comparison of the spatially distributed NOx emissions of DECSO and CAMS showed that the satellite-derived emissions are often higher in cities, while they are similar for large power plants and slightly lower in rural areas.
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来源期刊
Atmospheric Chemistry and Physics
Atmospheric Chemistry and Physics 地学-气象与大气科学
CiteScore
10.70
自引率
20.60%
发文量
702
审稿时长
6 months
期刊介绍: Atmospheric Chemistry and Physics (ACP) is a not-for-profit international scientific journal dedicated to the publication and public discussion of high-quality studies investigating the Earth''s atmosphere and the underlying chemical and physical processes. It covers the altitude range from the land and ocean surface up to the turbopause, including the troposphere, stratosphere, and mesosphere. The main subject areas comprise atmospheric modelling, field measurements, remote sensing, and laboratory studies of gases, aerosols, clouds and precipitation, isotopes, radiation, dynamics, biosphere interactions, and hydrosphere interactions. The journal scope is focused on studies with general implications for atmospheric science rather than investigations that are primarily of local or technical interest.
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