Umkehr、臭氧探测仪和 COH 过站记录中的臭氧变化趋势

IF 5.2 1区 地球科学 Q1 ENVIRONMENTAL SCIENCES Atmospheric Chemistry and Physics Pub Date : 2024-07-08 DOI:10.5194/egusphere-2024-1821
Irina Petropavlovskikh, Jeannette D. Wild, Kari Abromitis, Peter Effertz, Koji Miyagawa, Lawrence E. Flynn, Eliane Maillard-Barra, Robert Damadeo, Glen McConville, Bryan Johnson, Patrick Cullis, Sophie Godin-Beekmann, Gerald Ancellet, Richard Querel, Roeland Van Malderen, Daniel Zawada
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引用次数: 0

摘要

摘要。本研究对瑞士/德国 Arosa/Davos/Hohenpeißenberg 观测站、法国上普罗旺斯观测站、科罗拉多州博尔德观测站、夏威夷茂纳罗亚观测站和希洛观测站以及新西兰劳德观测站的平流层臭氧剖面趋势进行了最新评估,重点关注 2000 年后的臭氧恢复期。利用 NOAA 多布森网络的垂直臭氧剖面图,通过 Umkehr 方法(最近进行了新的同质化)、臭氧探测仪和 NOAA COHesive SBUV/OMPS 星基记录(COH)进行采样,以与本研究中使用的地面站的地理坐标相匹配,从而得出趋势。使用平流层臭氧长期趋势和不确定性(LOTUS)独立线性趋势(ILT)回归模型的更新版本(0.8.0)对平流层臭氧时间序列的长期变化进行了分析。这项研究发现,从不同观测记录中得出的趋势具有一致性,这是了解《蒙特利尔议定书》及其修正案实施后臭氧层恢复情况的一个关键因素。北半球 Aros/Davos、OHP 和 MLO 的 Umkehr 记录均显示平流层中上层的正趋势,趋势峰值为 ~+2 %/十年。虽然从 COH 卫星记录中得出的上平流层臭氧趋势比 Umkehr 系统检测到的趋势更积极,但两者的一致性在两个西格玛的不确定性范围内。Umkehr 在 Boulder 和 Lauder 上平流层的趋势是正的,但在统计上并不显著,而 COH 的趋势更大,在统计上也很显著(在 2 sigma 范围内)。在平流层下部,根据 Umkehr 和臭氧探测仪记录得出的趋势大多为负值(除了 OHP 的臭氧探测仪趋势为正值),但不确定性相当大。在 LOTUS 模式中,对五个地面站点的其他动力学代用指标进行了研究。额外代用指标的使用并没有显著改变趋势,但等效纬度降低了 Umkehr 和 COH 在上平流层和高纬度趋势的不确定性。在低层,额外的预测因子(所有站点的对流层顶气压、在 MLO 的准两年涛动的两个额外分量、在 Arosa/Davos、OHP 和 MLO 的北极涛动)改善了模型拟合,减少了 Umkehr 和 sonde 的趋势不确定性。
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Ozone trends in homogenized Umkehr, Ozonesonde, and COH overpass records
Abstract. This study presents an updated evaluation of stratospheric ozone profile trends at Arosa/Davos/Hohenpeißenberg, Switzerland/Germany, Observatory de Haute Provence (OHP), France, Boulder, Colorado, Mauna Loa Observatory (MLO) and Hilo, Hawaii, and Lauder, New Zealand with focus on the ozone recovery period post 2000. Trends are derived using vertical ozone profiles from NOAA’s Dobson Network via the Umkehr method (with a recent new homogenization), ozonesondes, and the NOAA COHesive SBUV/OMPS satellite-based record (COH) sampled to match geographical coordinates of the ground-based stations used in this study. Analyses of long-term changes in stratospheric ozone time series were performed using the updated version (0.8.0) of the Long-term Ozone Trends and Uncertainties in the Stratosphere (LOTUS) Independent Linear Trend (ILT) regression model. This study finds a consistency of the trends derived from the different observational records, which is a key factor to the understanding of the recovery of the ozone layer after the implementation of the Montreal Protocol and its amendments that control ozone-depleting substances production and release into the atmosphere. The Northern Hemispheric Umkehr records of Aros/Davos, OHP, and MLO all show positive trends in the mid to upper stratosphere with trends peaking at ~+2 %/decade. Although the upper stratospheric ozone trends derived from COH satellite records are more positive than those detected by the Umkehr system, the agreement is within the two sigma uncertainty. Umkehr trends in the upper stratosphere at Boulder and Lauder are positive but not statistically significant, while COH trends are larger and statistically significant (within 2 sigma). In the lower stratosphere, trends derived from Umkehr and ozonesonde records are mostly negative (except for positive ozonesonde trends at OHP), however the uncertainties are quite large. Additional dynamical proxies were investigated in the LOTUS model at five ground-based sites. The use of additional proxies did not significantly change trends, but equivalent latitude reduced the uncertainty of the Umkehr and COH trends in the upper stratosphere and at higher latitudes. In lower layers, additional predictors (tropopause pressure for all stations, two extra components of Quasi-Biennial Oscillation at MLO, Arctic Oscillation at Arosa/Davos, OHP and MLO) improve the model fit and reduce trend uncertainties as seen by Umkehr and sonde.
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来源期刊
Atmospheric Chemistry and Physics
Atmospheric Chemistry and Physics 地学-气象与大气科学
CiteScore
10.70
自引率
20.60%
发文量
702
审稿时长
6 months
期刊介绍: Atmospheric Chemistry and Physics (ACP) is a not-for-profit international scientific journal dedicated to the publication and public discussion of high-quality studies investigating the Earth''s atmosphere and the underlying chemical and physical processes. It covers the altitude range from the land and ocean surface up to the turbopause, including the troposphere, stratosphere, and mesosphere. The main subject areas comprise atmospheric modelling, field measurements, remote sensing, and laboratory studies of gases, aerosols, clouds and precipitation, isotopes, radiation, dynamics, biosphere interactions, and hydrosphere interactions. The journal scope is focused on studies with general implications for atmospheric science rather than investigations that are primarily of local or technical interest.
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