{"title":"对 48Ca 引发的聚变-蒸发反应中重核和超重核合成的系统研究","authors":"Shi-Hao Zhu, Tian-Liang Zhao, Xiao-Jun Bao","doi":"10.1007/s41365-024-01483-5","DOIUrl":null,"url":null,"abstract":"<p>We systematically studied the evaporation residue cross sections of <span>\\(^{48}\\hbox {Ca}\\)</span>-induced reactions on lanthanide and actinide target nuclei under the Dinuclear System (DNS) model framework to check the reliability and applicability of the model. To produce new proton-rich Fl and Lv isotopes through hot fusion reactions in the superheavy element region with <span>\\(Z\\ge 104\\)</span>, we utilized the reactions <span>\\(^{48}\\hbox {Ca}+^{236,238,239}\\hbox {Pu}\\)</span> and <span>\\(^{48}\\hbox {Ca}+^{242,243,244,250}\\hbox {Cm}\\)</span>. However, owing to the detection limit of available equipment (0.1 pb), only <span>\\(^{283}\\hbox {Fl}\\)</span> and <span>\\(^{287-289}\\hbox {Lv}\\)</span>, which have the maximum evaporation residue cross section values of 0.149, 0.130, 9.522, and 0.309 pb, respectively, can be produced. Furthermore, to produce neutron-deficient isotopes of actinides near the proton drip line with <span>\\(Z=93-100\\)</span>, we attempted to generate the new isotopes (<span>\\(^{224-227}\\hbox {Pu}\\)</span>, <span>\\(^{228-232,237}\\hbox {Cm}\\)</span>) using the reactions <span>\\(^{48}\\hbox {Ca}+^{180, 182, 183}\\hbox {W}\\)</span> and <span>\\(^{48}\\hbox {Ca}+^{184, 186, 187, 192}\\hbox {Os}\\)</span>. The maximum evaporation residue cross section values are 0.07, 0.06, 0.26, and 0.30 nb for the former set of reactions, and 1.96 pb, 5.73 pb, 12.16 pb, 19.39 pb, 54.79 pb, and 6.45 nb for the latter, respectively. These results are expected to provide new information for the future synthesis of unknown neutron-deficient isotopes.</p>","PeriodicalId":19177,"journal":{"name":"Nuclear Science and Techniques","volume":"6 1","pages":""},"PeriodicalIF":3.6000,"publicationDate":"2024-07-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Systematic study of the synthesis of heavy and superheavy nuclei in 48Ca-induced fusion-evaporation reactions\",\"authors\":\"Shi-Hao Zhu, Tian-Liang Zhao, Xiao-Jun Bao\",\"doi\":\"10.1007/s41365-024-01483-5\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>We systematically studied the evaporation residue cross sections of <span>\\\\(^{48}\\\\hbox {Ca}\\\\)</span>-induced reactions on lanthanide and actinide target nuclei under the Dinuclear System (DNS) model framework to check the reliability and applicability of the model. To produce new proton-rich Fl and Lv isotopes through hot fusion reactions in the superheavy element region with <span>\\\\(Z\\\\ge 104\\\\)</span>, we utilized the reactions <span>\\\\(^{48}\\\\hbox {Ca}+^{236,238,239}\\\\hbox {Pu}\\\\)</span> and <span>\\\\(^{48}\\\\hbox {Ca}+^{242,243,244,250}\\\\hbox {Cm}\\\\)</span>. However, owing to the detection limit of available equipment (0.1 pb), only <span>\\\\(^{283}\\\\hbox {Fl}\\\\)</span> and <span>\\\\(^{287-289}\\\\hbox {Lv}\\\\)</span>, which have the maximum evaporation residue cross section values of 0.149, 0.130, 9.522, and 0.309 pb, respectively, can be produced. Furthermore, to produce neutron-deficient isotopes of actinides near the proton drip line with <span>\\\\(Z=93-100\\\\)</span>, we attempted to generate the new isotopes (<span>\\\\(^{224-227}\\\\hbox {Pu}\\\\)</span>, <span>\\\\(^{228-232,237}\\\\hbox {Cm}\\\\)</span>) using the reactions <span>\\\\(^{48}\\\\hbox {Ca}+^{180, 182, 183}\\\\hbox {W}\\\\)</span> and <span>\\\\(^{48}\\\\hbox {Ca}+^{184, 186, 187, 192}\\\\hbox {Os}\\\\)</span>. The maximum evaporation residue cross section values are 0.07, 0.06, 0.26, and 0.30 nb for the former set of reactions, and 1.96 pb, 5.73 pb, 12.16 pb, 19.39 pb, 54.79 pb, and 6.45 nb for the latter, respectively. These results are expected to provide new information for the future synthesis of unknown neutron-deficient isotopes.</p>\",\"PeriodicalId\":19177,\"journal\":{\"name\":\"Nuclear Science and Techniques\",\"volume\":\"6 1\",\"pages\":\"\"},\"PeriodicalIF\":3.6000,\"publicationDate\":\"2024-07-13\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Nuclear Science and Techniques\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://doi.org/10.1007/s41365-024-01483-5\",\"RegionNum\":1,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"NUCLEAR SCIENCE & TECHNOLOGY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Nuclear Science and Techniques","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1007/s41365-024-01483-5","RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"NUCLEAR SCIENCE & TECHNOLOGY","Score":null,"Total":0}
Systematic study of the synthesis of heavy and superheavy nuclei in 48Ca-induced fusion-evaporation reactions
We systematically studied the evaporation residue cross sections of \(^{48}\hbox {Ca}\)-induced reactions on lanthanide and actinide target nuclei under the Dinuclear System (DNS) model framework to check the reliability and applicability of the model. To produce new proton-rich Fl and Lv isotopes through hot fusion reactions in the superheavy element region with \(Z\ge 104\), we utilized the reactions \(^{48}\hbox {Ca}+^{236,238,239}\hbox {Pu}\) and \(^{48}\hbox {Ca}+^{242,243,244,250}\hbox {Cm}\). However, owing to the detection limit of available equipment (0.1 pb), only \(^{283}\hbox {Fl}\) and \(^{287-289}\hbox {Lv}\), which have the maximum evaporation residue cross section values of 0.149, 0.130, 9.522, and 0.309 pb, respectively, can be produced. Furthermore, to produce neutron-deficient isotopes of actinides near the proton drip line with \(Z=93-100\), we attempted to generate the new isotopes (\(^{224-227}\hbox {Pu}\), \(^{228-232,237}\hbox {Cm}\)) using the reactions \(^{48}\hbox {Ca}+^{180, 182, 183}\hbox {W}\) and \(^{48}\hbox {Ca}+^{184, 186, 187, 192}\hbox {Os}\). The maximum evaporation residue cross section values are 0.07, 0.06, 0.26, and 0.30 nb for the former set of reactions, and 1.96 pb, 5.73 pb, 12.16 pb, 19.39 pb, 54.79 pb, and 6.45 nb for the latter, respectively. These results are expected to provide new information for the future synthesis of unknown neutron-deficient isotopes.
期刊介绍:
Nuclear Science and Techniques (NST) reports scientific findings, technical advances and important results in the fields of nuclear science and techniques. The aim of this periodical is to stimulate cross-fertilization of knowledge among scientists and engineers working in the fields of nuclear research.
Scope covers the following subjects:
• Synchrotron radiation applications, beamline technology;
• Accelerator, ray technology and applications;
• Nuclear chemistry, radiochemistry, radiopharmaceuticals, nuclear medicine;
• Nuclear electronics and instrumentation;
• Nuclear physics and interdisciplinary research;
• Nuclear energy science and engineering.