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Analysis of level structure and monopole effects in Ca isotopes 钙同位素的水平结构和单极效应分析
IF 2.8 1区 物理与天体物理 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-18 DOI: 10.1007/s41365-024-01555-6
Jin Li, Ai-Xi Chen, Amir Jalili, Han-Kui Wang

Understanding the properties of nuclei near the double magic nucleus 40Ca is crucial for both nuclear theory and experiments. In this study, Ca isotopes were investigated using an extended pairing-plus-quadrupole model with monopole corrections. The negative-parity states of 44Ca were coupled with the intruder orbital (g_{9/2}) at 4 MeV. The values of (E_{4+})/(E_{2+}) agree well with experimental trend from 42Ca to 50Ca, considering monopole effects between (nu f_{7/2}) and (nu p_{3/2})((nu f_{5/2})). This monopole effect, determined from data of 48Ca and 50Ca, supports the proposed new nuclear magic number (N = 34) by predicting a high-energy (2^{+}) state in 54Ca.

了解双魔核 40Ca 附近原子核的性质对于核理论和实验都至关重要。在这项研究中,我们使用一个具有单极修正的扩展配对加四极模型对钙同位素进行了研究。44Ca 的负奇偶态与 4 MeV 的入侵轨道 (g_{9/2})耦合。考虑到(nu f_{7/2})和(nu p_{3/2})((nu f_{5/2}))之间的单极效应,(E_{4+})/(E_{2+})的值与从42Ca到50Ca的实验趋势一致。根据48Ca和50Ca的数据确定的这种单极效应,通过预测54Ca中的高能(2^{+})态,支持了所提出的新核魔数(N=34)。
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引用次数: 0
In-beam gamma rays of CSNS Back-n characterized by black resonance filter 用黑色共振滤波器表征 CSNS Back-n 的波束内伽马射线
IF 2.8 1区 物理与天体物理 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-18 DOI: 10.1007/s41365-024-01553-8
Jin-Cheng Wang, Jie Ren, Wei Jiang, Xi-Chao Ruan, Ying-Yi Liu, Hao-Lan Yang, Kuo-Zhi Xu, Xin-Yi Pan, Qi Sun, Jie Bao, Han-Xiong Huang, Hao-Fan Bai, Jiang-Bo Bai, Ping Cao, Qi-Ping Chen, Yong-Hao Chen, Wen-Hao Duan, An-Chuan Fan, Rui-Rui Fan, Chang-Qing Feng, Min-Hao Gu, Chang-Cai Han, Zi-Jie Han, Guo-Zhu He, Yong-Cheng He, Yang Hong, Yi-Wei Hu, Zhi-Jie Jiang, Ling Kang, Chang-Lin Lan, Bo Li, Feng Li, Qiang Li, Xiao Li, Yang Li, Jie Liu, Rong Liu, Shu-Bin Liu, Yi-Na Liu, Guang-Yuan Luan, Chang-Jun Ning, Yi-Jia Qiu, Wen-Kai Ren, Zhi-Zhou Ren, Zhao-Hui Song, Kang Sun, Zhi-Xin Tan, Jing-Yu Tang, Sheng-Da Tang, Li-Jiao Wang, Peng-Cheng Wang, Zhao-Hui Wang, Zhong-Wei Wen, Xiao-Guang Wu, Xuan Wu, Ze-Peng Wu, Cong Xia, Li-Kun Xie, Han Yi, Tao Yu, Yong-Ji Yu, Guo-Hui Zhang, Hang-Chang Zhang, Qi-Wei Zhang, Xian-Peng Zhang, Yu-Liang Zhang, Zhi-Yong Zhang, Mao-Yuan Zhao, Zhi-Hao Zhou, Ke-Jun Zhu, Chong Zou

The back-streaming white-neutron beamline (Back-n) of the China Spallation Neutron Source is an essential neutron-research platform built for the study of nuclear data, neutron physics, and neutron applications. Many types of cross-sectional neutron-reaction measurements have been performed at Back-n since early 2018. These measurements have shown that a significant number of gamma rays can be transmitted to the experimental stations of Back-n along with the neutron beam. These gamma rays, commonly referred to as in-beam gamma rays, can induce a non-negligible experimental background in neutron-reaction measurements. Studying the characteristics of in-beam gamma rays is important for understanding the experimental background. However, measuring in-beam gamma rays is challenging because most gamma-ray detectors are sensitive to neutrons; thus, discriminating between neutron-induced signals and those from in-beam gamma rays is difficult. In this study, we propose the use of the black resonance filter method and a (hbox {CeBr}_{3}) scintillation detector to measure the characteristics of the in-beam gamma rays of Back-n. Four types of black resonance filters, 181Ta, 59Co, natAg, and natCd, were used in this measurement. The time-of-flight (TOF) technique was used to select the detector signals remaining in the absorption region of the TOF spectra, which were mainly induced by in-beam gamma rays. The energy distribution and flux of the in-beam gamma rays of Back-n were determined by analyzing the deposited energy spectra of the (hbox {CeBr}_{3}) scintillation detector and using Monte Carlo simulations. Based on the results of this study, the background contributions from in-beam gamma rays in neutron-reaction measurements at Back-n can be reasonably evaluated, which is beneficial for enhancing both the experimental methodology and data analysis.

中国散裂中子源后流白中子束线(Back-n)是为研究核数据、中子物理和中子应用而搭建的重要中子研究平台。自2018年初以来,Back-n已经进行了多种类型的横截面中子反应测量。这些测量结果表明,大量伽马射线可以随着中子束传输到Back-n的实验站。这些伽马射线通常被称为束内伽马射线,可以在中子反应测量中引起不可忽略的实验背景。研究束内伽马射线的特性对于了解实验背景非常重要。然而,测量束内伽马射线具有挑战性,因为大多数伽马射线探测器都对中子敏感,因此很难区分中子诱导的信号和束内伽马射线的信号。在这项研究中,我们提出使用黑色共振滤波器方法和闪烁探测器来测量Back-n的束内伽马射线特性。这次测量使用了四种黑色共振滤光片,即 181Ta、59Co、natAg 和 natCd。利用飞行时间(TOF)技术选择停留在 TOF 光谱吸收区的探测器信号,这些信号主要是由束内伽马射线引起的。通过分析(hbox {CeBr}_{3}) 闪烁探测器的沉积能谱和蒙特卡罗模拟,确定了Back-n的束内伽马射线的能量分布和通量。根据这项研究的结果,可以合理地评估在Back-n进行中子反应测量时束内伽马射线的背景贡献,这对改进实验方法和数据分析都是有益的。
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引用次数: 0
Properties of the phase diagram from the Nambu-Jona-Lasino model with a scalar-vector interaction 具有标量-矢量相互作用的南布-若纳-拉西诺模型相图的性质
IF 2.8 1区 物理与天体物理 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-18 DOI: 10.1007/s41365-024-01559-2
Yong-Hang Yang, He Liu, Peng-Cheng Chu

We investigated the properties of the phase diagram of high-order susceptibilities, speed of sound, and polytropic index based on an extended Nambu-Jona-Lasinio model with an eight-quark scalar-vector interaction. Non-monotonic behavior was observed in all these quantities around the phase transition boundary, which also revealed the properties of the critical point. Further, this study indicated that the chiral phase transition boundary and critical point could vary depending on the scalar-vector coupling constant (G_text {SV}). At finite densities and temperatures, the negative (G_text {SV}) term exhibited attractive interactions, which enhanced the critical point temperature and reduced the chemical potential. The (G_text {SV}) term also affected the properties of the high-order susceptibilities, speed of sound, and polytropic index near the critical point. The non-monotonic (peak or dip) structures of these quantities shifted to a low baryon chemical potential (and high temperature) with a negative (G_text {SV}). (G_text {SV}) also changed the amplitude and range of the nonmonotonic regions. Therefore, the scalar-vector interaction was useful for locating the phase boundary and critical point in QCD phase diagram by comparing the experimental data. The study of the non-monotonic behavior of high-order susceptibilities, speed of sound, and polytropic index is of great interest, and further observations related to high-order susceptibilities, speed of sound, and polytropic index being found and applied to the search for critical points in heavy-ion collisions and the study of compact stars are eagerly awaited.

我们研究了基于八夸克标量-矢量相互作用的扩展南布-若纳-拉西尼奥模型的高阶感性、声速和多向指数相图的性质。在相变边界附近观察到所有这些量的非单调行为,这也揭示了临界点的特性。此外,这项研究还表明,手性相变边界和临界点的变化取决于标量-矢量耦合常数(G_text {SV})。在有限密度和温度下,负的(Gtext {SV})项表现出吸引力相互作用,从而提高了临界点温度并降低了化学势。G (text {SV})项还影响临界点附近的高阶易感性、声速和多向指数。这些量的非单调(峰值或倾角)结构随着负的(Gtext {SV})项而转向低重子化学势(和高温)。(Gtext {SV})也改变了非单调区域的振幅和范围。因此,标量-矢量相互作用有助于通过比较实验数据来定位QCD相图中的相边界和临界点。对高阶感度、声速和多向指数的非单调行为的研究是非常有意义的,我们热切地期待着进一步发现与高阶感度、声速和多向指数有关的观测结果,并将其应用于重离子碰撞临界点的寻找和紧凑星的研究。
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引用次数: 0
Highly coupled off-resonance lattice design in diffraction-limited light sources 衍射受限光源中的高耦合非共振晶格设计
IF 2.8 1区 物理与天体物理 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-06 DOI: 10.1007/s41365-024-01511-4
Yi-Hao Gong, Shun-Qiang Tian, Xin-Zhong Liu, Shou-Zhi Xuan, Li-Yuan Tan, Ling-Long Mao

The round-beam operation presents many benefits for scientific experiments regarding synchrotron radiation and the weakening influences of intra-beam scattering in diffraction-limited synchrotron light sources. A round-beam generation method based on the global setting of skew quadrupoles and the application of a non-dominated sorting genetic algorithm was proposed in this study. Two schemes, including large-emittance coupling introduced via betatron coupling and vertical dispersion, were explored in a candidate lattice for an upgrade-proposal of the Shanghai synchrotron radiation facility. Emittance variations with lattice imperfections and their influence on the beam dynamics of beam optic distortions were investigated. The results demonstrated that a precise coupling control ranging from 10 to 100% was achieved under low optical distortion, whereas full-coupling generation and its robustness were achieved by our proposed method by adjusting the skew quadrupole components located in the dispersion-free sections. The Touschek lifetime increased by a factor of 2–2.5.

圆光束操作为同步辐射科学实验和减弱衍射限制同步辐射光源中光束内散射的影响带来了许多好处。本研究提出了一种基于倾斜四极的全局设置和非支配排序遗传算法的圆光束生成方法。在上海同步辐射设施升级方案的候选晶格中探索了两种方案,包括通过贝塔射线耦合和垂直色散引入的大幅射耦合。研究了发射率随晶格缺陷的变化及其对光束光学畸变的光束动力学的影响。结果表明,在低光学畸变条件下,可以实现从 10%到 100%的精确耦合控制,而通过调整位于无色散部分的偏斜四极分量,我们提出的方法可以实现全耦合产生及其稳健性。图谢克寿命增加了 2-2.5 倍。
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引用次数: 0
Possibility of reaching the predicted center of the “island of stability” via the radioactive beam-induced fusion reactions 通过放射性束诱导聚变反应到达 "稳定岛 "预测中心的可能性
IF 2.8 1区 物理与天体物理 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-04 DOI: 10.1007/s41365-024-01542-x
Ming-Hao Zhang, Ying Zou, Mei-Chen Wang, Gen Zhang, Qing-Lin Niu, Feng-Shou Zhang

Based on the dinuclear system model, the synthesis of the predicted double-magic nuclei ({^{298}hbox {Fl}}) and ({^{304}hbox {120}}) was investigated via neutron-rich radioactive beam-induced fusion reactions. The reaction ({^{58}hbox {Ca}}+{^{244}hbox {Pu}}) is predicted to be favorable for producing ({^{298}hbox {Fl}}) with a maximal ER cross section of ({0.301},hbox {pb}). Investigations of the entrance channel effect reveal that the ({^{244}hbox {Pu}}) target is more promising for synthesizing ({^{298}hbox {Fl}}) than the neutron-rich targets ({^{248}hbox {Cm}}) and ({^{249}hbox {Bk}}), because of the influence of the Coulomb barrier. For the synthesis of ({^{304}hbox {120}}), the maximal ER cross section of ({0.046},hbox {fb}) emerges in the reaction ({^{58}hbox {V}}+{^{249}hbox {Bk}}), indicating the need for further advancements in both experimental facilities and reaction mechanisms.

在双核系统模型的基础上,通过富中子放射性束诱导聚变反应,研究了预测的双魔核({^{298}hbox {Fl}})和({^{304}hbox {120}})的合成。据预测,反应({^{58}hbox {Ca}+{^{244}hbox {Pu}})有利于产生({^{298}hbox {Fl}}),其最大ER横截面为({0.301},hbox {pb})。对入口通道效应的研究表明,由于库仑障碍的影响,({^{244}hbox {Pu}})靶比富中子靶({^{248}hbox {Cm}})和({^{249}hbox {Bk}})更有希望合成({^{298}hbox {Fl}})。对于({^{304}hbox {120}})的合成,在反应({^{58}hbox {V}+{^{249}hbox {Bk}})中出现了最大的ER横截面({0.046},hbox {fb}),这表明实验设施和反应机制都需要进一步发展。
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引用次数: 0
Passive neutron multiplicity device for 240Pu measurement based on FPGA 基于 FPGA 的 240Pu 测量无源中子倍率装置
IF 2.8 1区 物理与天体物理 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-04 DOI: 10.1007/s41365-024-01514-1
Yan Zhang, Hao-Ran Zhang, Ren-Bo Wang, Ming-Yu Li, Rui Chen, Hai-Tao Wang, Xiang-Ting Meng, Shu-Min Zhou, Bin Tang

A passive neutron multiplicity measurement device, FH-NCM/S1, based on field-programmable gate arrays (FPGAs), is developed specifically for measuring the mass of plutonium-240 (240Pu) in mixed oxide fuel. FH-NCM/S1 adopts an integrated approach, combining the shift register analysis mode with the pulse-position timestamp mode using an FPGA. The optimal effective length of the 3He neutron detector was determined to be 30 cm, and the thickness of the graphite reflector was ascertained to be 15 cm through MCNP simulations. After fabricating the device, calibration measurements were performed using a 252Cf neutron source; a detection efficiency of 43.07% and detector die-away time of 55.79 ({upmu })s were observed. Nine samples of plutonium oxide were measured under identical conditions using the FH-NCM/S1 in shift register analysis mode and a plutonium waste multiplicity counter. The obtained double rates underwent corrections for detection efficiency ((varepsilon)) and double gate fraction ((f_{rm d})), resulting in corrected double rates ((D_{rm c})), which were used to validate the accuracy of the shift register analysis mode. Furthermore, the device exhibited fluctuations in the measurement results, and within a single 20 s measurement, these fluctuations remained below 10%. After 30 cycles, the relative error in the mass of 240Pu was less than 5%. Finally, correlation calculations confirmed the robust consistency of both measurement modes. This study holds specific significance for the subsequent design and development of neutron multiplicity devices.

我们开发了一种基于现场可编程门阵列(FPGA)的被动中子倍率测量装置 FH-NCM/S1,专门用于测量混合氧化物燃料中钚 240(240Pu)的质量。FH-NCM/S1 采用集成方法,利用 FPGA 将移位寄存器分析模式与脉冲位置时间戳模式相结合。通过 MCNP 模拟,确定 3He 中子探测器的最佳有效长度为 30 厘米,石墨反射器的厚度为 15 厘米。装置制作完成后,使用 252Cf 中子源进行了校准测量;观察到探测效率为 43.07%,探测器消亡时间为 55.79 ({upmu })s 。在相同的条件下,使用移位寄存器分析模式下的 FH-NCM/S1 和钚废物倍率计数器测量了九个氧化钚样品。所获得的双倍率经过了探测效率((varepsilon))和双闸门分数((f_{rm d}))的修正,从而得到了修正后的双倍率((D_{rm c})),用来验证移位寄存器分析模式的准确性。此外,该装置在测量结果中表现出波动,在一次 20 秒的测量中,这些波动保持在 10% 以下。经过 30 个周期后,240Pu 质量的相对误差小于 5%。最后,相关计算证实了两种测量模式的稳健一致性。这项研究对中子倍率装置的后续设计和开发具有重要意义。
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引用次数: 0
Geant4 simulation of fast-electron bremsstrahlung imaging at the HL-3 tokamak Geant4 模拟 HL-3 托卡马克的快电子轫致辐射成像
IF 2.8 1区 物理与天体物理 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-03 DOI: 10.1007/s41365-024-01505-2
Shi-Kui Cheng, Yi-Po Zhang, Yue-Jiang Shi, Jie Zhang, Shuai Guan, Hong-Bing Xu, Qiu-Lei Yang

To further research on high-parameter plasma, we plan to develop a two-dimensional hard X-ray (HXR) imaging system at the HL-3 tokamak to measure HXRs with energies ranging from 20 to 300 keV. The application of an array-structured detector ensures that this system can measure HXR-radiation spectra from the entire plasma cross section. Therefore, it is suitable for the study of fast-electron physics, such as radio-frequency wave current drives, fast electrons driving instabilities, and plasma disruptions in fusion research. In this study, we develop a simulation for calculating fast-electron bremsstrahlung in the HL-3 tokamak based on the Monte Carlo simulation code Geant4, in which the plasma geometry and forward scattering of fast-electron bremsstrahlung are considered. The preliminary calculation results indicate that the HXR energy deposition on the detector is symmetrically distributed, even though the plasma distribution is asymmetric owing to the toroidal effect. These simulation results are helpful in constructing the relationship between the energy deposition on the detector and parameter distribution on the plasma cross section during HL-3 experiments. This is beneficial for the reconstruction of the fast-electron-distribution function and for optimizing the design of the HXR-imaging system.

为了进一步研究高参数等离子体,我们计划在 HL-3 托卡马克开发一个二维硬 X 射线(HXR)成像系统,以测量能量范围为 20 至 300 千伏的 HXR。阵列结构探测器的应用确保该系统能够测量整个等离子体截面的 HXR 辐射谱。因此,它适用于研究快电子物理学,如射频波电流驱动、快电子驱动不稳定性和聚变研究中的等离子体破坏。在本研究中,我们基于蒙特卡罗模拟代码 Geant4 开发了一种模拟计算方法,用于计算 HL-3 托卡马克中的快电子轫致辐射,其中考虑了等离子体的几何形状和快电子轫致辐射的正向散射。初步计算结果表明,尽管等离子体的分布由于环状效应而不对称,但探测器上的 HXR 能量沉积是对称分布的。这些模拟结果有助于构建 HL-3 实验期间探测器上的能量沉积与等离子体截面参数分布之间的关系。这有利于重建快速电子分布函数和优化 HXR 成像系统的设计。
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引用次数: 0
A real-time calibration method based on time-to-digital converter for accelerator timing system 基于时数转换器的加速器计时系统实时校准方法
IF 2.8 1区 物理与天体物理 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-03 DOI: 10.1007/s41365-024-01510-5
Qi-Hao Duan, Liang Ge, Yan-Hao Jia, Jie-Yu Zhu, Wei Zhang

The high-intensity heavy-ion accelerator facility (HIAF) is a scientific research facility complex composed of multiple cascade accelerators of different types, which pose a scheduling problem for devices distributed over a certain range of 2 km, involving over a hundred devices. The white rabbit, a technology-enhancing Gigabit Ethernet, has shown the capability of scheduling distributed timing devices but still faces the challenge of obtaining real-time synchronization calibration parameters with high precision. This study presents a calibration system based on a time-to-digital converter implemented on an ARM-based System-on-Chip (SoC). The system consists of four multi-sample delay lines, a bubble-proof encoder, an edge controller for managing data from different channels, and a highly effective calibration module that benefits from the SoC architecture. The performance was evaluated with an average RMS precision of 5.51 ps by measuring the time intervals from 0 to 24,000 ps with 120,000 data for every test. The design presented in this study refines the calibration precision of the HIAF timing system. This eliminates the errors caused by manual calibration without efficiency loss and provides data support for fault diagnosis. It can also be easily tailored or ported to other devices for specific applications and provides more space for developing timing systems for particle accelerators, such as white rabbits on HIAF.

高强度重离子加速器设施(HIAF)是由多台不同类型的级联加速器组成的科研设施群,其设备分布在一定范围内(2 千米),涉及百余台设备,这给设备调度带来了难题。技术增强型千兆以太网 "白兔 "已显示出调度分布式授时设备的能力,但仍面临如何高精度获取实时同步校准参数的挑战。本研究提出了一种校准系统,它基于在基于 ARM 的片上系统(SoC)上实现的时间数字转换器。该系统包括四条多采样延迟线、一个防气泡编码器、一个用于管理不同通道数据的边缘控制器,以及一个受益于 SoC 架构的高效校准模块。通过测量从 0 到 24,000 ps 的时间间隔,每次测试 120,000 个数据,评估了平均有效值精度为 5.51 ps 的性能。本研究提出的设计改进了 HIAF 定时系统的校准精度。这不仅消除了手动校准造成的误差,而且不会降低效率,并为故障诊断提供了数据支持。它还可以很容易地定制或移植到其他设备上用于特定应用,并为开发粒子加速器(如 HIAF 上的白兔)计时系统提供了更大的空间。
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引用次数: 0
Sustainability-oriented prioritization of nuclear fuel cycle transitions in China: a holistic MCDM framework under uncertainties 以可持续发展为导向确定中国核燃料循环过渡的优先次序:不确定性条件下的整体 MCDM 框架
IF 2.8 1区 物理与天体物理 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-09-03 DOI: 10.1007/s41365-024-01504-3
Lei Wang, Ru-Xing Gao, Hyo On Nam, Hong Jang, Won Il Ko, Chun-Dong Zhang, Guo-An Ye, Wen-Heng Jing

A sustainability-oriented assessment of the nuclear energy system can provide informative and convincing decision-making support for nuclear development strategies in China. In our previous study, four authentic nuclear fuel cycle (NFC) transition scenarios were proposed, featuring different development stages and exhibiting distinct environmental, economic, and technical characteristics. However, because of the multiple and often conflicting criteria embedded therein, determining the top-priority NFC alternative for a sustainability orientation remains challenging. To address this issue, this study proposed a novel hybrid multi-criteria decision-making framework comprising fuzzy AHP, PROMETHEE GAIA, and MOORA. Initially, an improved fuzzy AHP weighting model was developed to determine criteria weights under uncertainty and investigate the influence of various weight aggregation and defuzzification approaches. Subsequently, PROMETHEE GAIA was used to address conflicts among the criteria and prioritize alternatives on a visualized k-dimensional GAIA plane. As a result, the alternative for direct recycling PWR spent fuel in fast reactors is considered the most sustainable. Furthermore, a sensitivity analysis was conducted to examine the influence of criteria weight variation and validate the screening results. Finally, using MOORA, some significant optimization ideas and valuable insights were provided to support decision-makers in shaping nuclear development strategies.

对核能系统进行以可持续发展为导向的评估,可为中国核电发展战略提供翔实且令人信服的决策支持。在我们之前的研究中,提出了四种真实的核燃料循环(NFC)过渡方案,它们处于不同的发展阶段,并表现出不同的环境、经济和技术特征。然而,由于其中蕴含着多种标准,而且这些标准往往相互冲突,因此,从可持续发展的角度确定最优先的核燃料循环替代方案仍具有挑战性。为解决这一问题,本研究提出了一种新型混合多标准决策框架,包括模糊 AHP、PROMETHEE GAIA 和 MOORA。首先,建立了一个改进的模糊 AHP 权重模型,以确定不确定条件下的标准权重,并研究各种权重聚合和去模糊化方法的影响。随后,利用 PROMETHEE GAIA 解决标准之间的冲突,并在可视化的 k 维 GAIA 平面上确定备选方案的优先次序。结果,在快堆中直接循环利用压水堆乏燃料的替代方案被认为最具可持续性。此外,还进行了敏感性分析,以研究标准权重变化的影响,并验证筛选结果。最后,利用 MOORA 提供了一些重要的优化思路和有价值的见解,为决策者制定核发展战略提供了支持。
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引用次数: 0
A seven-crystal spectrometer for high-energy resolution X-ray spectroscopy at Shanghai Synchrotron Radiation Facility 上海同步辐射设施用于高能分辨率 X 射线光谱分析的七晶光谱仪
IF 2.8 1区 物理与天体物理 Q1 NUCLEAR SCIENCE & TECHNOLOGY Pub Date : 2024-08-31 DOI: 10.1007/s41365-024-01486-2
Bing-Bao Mei, Liang-Xin Wang, Song-Qi Gu, Xiao-Zhi Su, Shuo Zhang, Yao Wei, Jing-Yuan Ma, Zheng Jiang, Fei Song

A Johann-type X-ray spectrometer was successfully developed at the hard X-ray branch (in-vacuum undulator with a 24-mm periodic length) of the energy material beamline (E-line) at the Shanghai Synchrotron Radiation Facility (SSRF). This spectrometer was utilized to implement X-ray emission spectroscopy (XES), high-energy resolution fluorescence-detected X-ray absorption spectroscopy (HERFD-XAS), and resonant inelastic X-ray scattering. Seven spherically bent crystals were positioned on the respective vertical 500-mm-diameter Rowland circles, adopting an area detector to increase the solid angle to 1.75(%) of 4 (pi) sr, facilitating the study of low-concentrate systems under complex reaction conditions. Operated under the atmosphere pressure, the spectrometer covers the energy region from 3.5 to 18 keV, with the Bragg angle ranging from 73(^{circ }) to 86(^{circ }) during vertical scanning. It offers a promised energy resolution of sub-eV (XES) and super-eV (HERFD-XAS). Generally, these comprehensive core-level spectroscopy methods based on hard X-rays at the E-line with an extremely high photon flux can meet the crucial requirements of a green energy strategy. Moreover, they provide substantial support for scientific advances in fundamental research.

在上海同步辐射中心(SSRF)能量材料光束线(E-line)的硬 X 射线分支(周期长度为 24 毫米的真空中起落架)上成功研制了约翰型 X 射线光谱仪。该光谱仪用于实施 X 射线发射光谱(XES)、高能量分辨率荧光检测 X 射线吸收光谱(HERFD-XAS)和共振非弹性 X 射线散射。七块球形弯曲晶体被放置在各自垂直的直径为500毫米的罗兰圆上,采用面积探测器将固角增大到1.75(%)的4(pi)sr,为研究复杂反应条件下的低浓度体系提供了便利。该光谱仪在大气压力下运行,覆盖了从3.5到18 keV的能量区域,垂直扫描时的布拉格角范围为73(^{circ } )到86(^{circ } )。它的能量分辨率可达亚电子伏特(XES)和超电子伏特(HERFD-XAS)。一般来说,这些基于 E 线硬 X 射线的综合核心级光谱方法具有极高的光子通量,可以满足绿色能源战略的关键要求。此外,它们还为基础研究的科学进步提供了实质性支持。
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引用次数: 0
期刊
Nuclear Science and Techniques
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