Nuclear Science and Techniques最新文献

The round-beam operation presents many benefits for scientific experiments regarding synchrotron radiation and the weakening influences of intra-beam scattering in diffraction-limited synchrotron light sources. A round-beam generation method based on the global setting of skew quadrupoles and the application of a non-dominated sorting genetic algorithm was proposed in this study. Two schemes, including large-emittance coupling introduced via betatron coupling and vertical dispersion, were explored in a candidate lattice for an upgrade-proposal of the Shanghai synchrotron radiation facility. Emittance variations with lattice imperfections and their influence on the beam dynamics of beam optic distortions were investigated. The results demonstrated that a precise coupling control ranging from 10 to 100% was achieved under low optical distortion, whereas full-coupling generation and its robustness were achieved by our proposed method by adjusting the skew quadrupole components located in the dispersion-free sections. The Touschek lifetime increased by a factor of 2–2.5.

Based on the dinuclear system model, the synthesis of the predicted double-magic nuclei ({^{298}hbox {Fl}}) and ({^{304}hbox {120}}) was investigated via neutron-rich radioactive beam-induced fusion reactions. The reaction ({^{58}hbox {Ca}}+{^{244}hbox {Pu}}) is predicted to be favorable for producing ({^{298}hbox {Fl}}) with a maximal ER cross section of ({0.301},hbox {pb}). Investigations of the entrance channel effect reveal that the ({^{244}hbox {Pu}}) target is more promising for synthesizing ({^{298}hbox {Fl}}) than the neutron-rich targets ({^{248}hbox {Cm}}) and ({^{249}hbox {Bk}}), because of the influence of the Coulomb barrier. For the synthesis of ({^{304}hbox {120}}), the maximal ER cross section of ({0.046},hbox {fb}) emerges in the reaction ({^{58}hbox {V}}+{^{249}hbox {Bk}}), indicating the need for further advancements in both experimental facilities and reaction mechanisms.

A passive neutron multiplicity measurement device, FH-NCM/S1, based on field-programmable gate arrays (FPGAs), is developed specifically for measuring the mass of plutonium-240 (²⁴⁰Pu) in mixed oxide fuel. FH-NCM/S1 adopts an integrated approach, combining the shift register analysis mode with the pulse-position timestamp mode using an FPGA. The optimal effective length of the ³He neutron detector was determined to be 30 cm, and the thickness of the graphite reflector was ascertained to be 15 cm through MCNP simulations. After fabricating the device, calibration measurements were performed using a ²⁵²Cf neutron source; a detection efficiency of 43.07% and detector die-away time of 55.79 ({upmu })s were observed. Nine samples of plutonium oxide were measured under identical conditions using the FH-NCM/S1 in shift register analysis mode and a plutonium waste multiplicity counter. The obtained double rates underwent corrections for detection efficiency ((varepsilon)) and double gate fraction ((f_{rm d})), resulting in corrected double rates ((D_{rm c})), which were used to validate the accuracy of the shift register analysis mode. Furthermore, the device exhibited fluctuations in the measurement results, and within a single 20 s measurement, these fluctuations remained below 10%. After 30 cycles, the relative error in the mass of ²⁴⁰Pu was less than 5%. Finally, correlation calculations confirmed the robust consistency of both measurement modes. This study holds specific significance for the subsequent design and development of neutron multiplicity devices.

To further research on high-parameter plasma, we plan to develop a two-dimensional hard X-ray (HXR) imaging system at the HL-3 tokamak to measure HXRs with energies ranging from 20 to 300 keV. The application of an array-structured detector ensures that this system can measure HXR-radiation spectra from the entire plasma cross section. Therefore, it is suitable for the study of fast-electron physics, such as radio-frequency wave current drives, fast electrons driving instabilities, and plasma disruptions in fusion research. In this study, we develop a simulation for calculating fast-electron bremsstrahlung in the HL-3 tokamak based on the Monte Carlo simulation code Geant4, in which the plasma geometry and forward scattering of fast-electron bremsstrahlung are considered. The preliminary calculation results indicate that the HXR energy deposition on the detector is symmetrically distributed, even though the plasma distribution is asymmetric owing to the toroidal effect. These simulation results are helpful in constructing the relationship between the energy deposition on the detector and parameter distribution on the plasma cross section during HL-3 experiments. This is beneficial for the reconstruction of the fast-electron-distribution function and for optimizing the design of the HXR-imaging system.

The high-intensity heavy-ion accelerator facility (HIAF) is a scientific research facility complex composed of multiple cascade accelerators of different types, which pose a scheduling problem for devices distributed over a certain range of 2 km, involving over a hundred devices. The white rabbit, a technology-enhancing Gigabit Ethernet, has shown the capability of scheduling distributed timing devices but still faces the challenge of obtaining real-time synchronization calibration parameters with high precision. This study presents a calibration system based on a time-to-digital converter implemented on an ARM-based System-on-Chip (SoC). The system consists of four multi-sample delay lines, a bubble-proof encoder, an edge controller for managing data from different channels, and a highly effective calibration module that benefits from the SoC architecture. The performance was evaluated with an average RMS precision of 5.51 ps by measuring the time intervals from 0 to 24,000 ps with 120,000 data for every test. The design presented in this study refines the calibration precision of the HIAF timing system. This eliminates the errors caused by manual calibration without efficiency loss and provides data support for fault diagnosis. It can also be easily tailored or ported to other devices for specific applications and provides more space for developing timing systems for particle accelerators, such as white rabbits on HIAF.

A sustainability-oriented assessment of the nuclear energy system can provide informative and convincing decision-making support for nuclear development strategies in China. In our previous study, four authentic nuclear fuel cycle (NFC) transition scenarios were proposed, featuring different development stages and exhibiting distinct environmental, economic, and technical characteristics. However, because of the multiple and often conflicting criteria embedded therein, determining the top-priority NFC alternative for a sustainability orientation remains challenging. To address this issue, this study proposed a novel hybrid multi-criteria decision-making framework comprising fuzzy AHP, PROMETHEE GAIA, and MOORA. Initially, an improved fuzzy AHP weighting model was developed to determine criteria weights under uncertainty and investigate the influence of various weight aggregation and defuzzification approaches. Subsequently, PROMETHEE GAIA was used to address conflicts among the criteria and prioritize alternatives on a visualized k-dimensional GAIA plane. As a result, the alternative for direct recycling PWR spent fuel in fast reactors is considered the most sustainable. Furthermore, a sensitivity analysis was conducted to examine the influence of criteria weight variation and validate the screening results. Finally, using MOORA, some significant optimization ideas and valuable insights were provided to support decision-makers in shaping nuclear development strategies.

A Johann-type X-ray spectrometer was successfully developed at the hard X-ray branch (in-vacuum undulator with a 24-mm periodic length) of the energy material beamline (E-line) at the Shanghai Synchrotron Radiation Facility (SSRF). This spectrometer was utilized to implement X-ray emission spectroscopy (XES), high-energy resolution fluorescence-detected X-ray absorption spectroscopy (HERFD-XAS), and resonant inelastic X-ray scattering. Seven spherically bent crystals were positioned on the respective vertical 500-mm-diameter Rowland circles, adopting an area detector to increase the solid angle to 1.75(%) of 4 (pi) sr, facilitating the study of low-concentrate systems under complex reaction conditions. Operated under the atmosphere pressure, the spectrometer covers the energy region from 3.5 to 18 keV, with the Bragg angle ranging from 73(^{circ }) to 86(^{circ }) during vertical scanning. It offers a promised energy resolution of sub-eV (XES) and super-eV (HERFD-XAS). Generally, these comprehensive core-level spectroscopy methods based on hard X-rays at the E-line with an extremely high photon flux can meet the crucial requirements of a green energy strategy. Moreover, they provide substantial support for scientific advances in fundamental research.

In recent years, the gap between the supply and demand of medical radioisotopes has increased, necessitating new methods for producing medical radioisotopes. Photonuclear reactions based on gamma sources have unique advantages in terms of producing high specific activity and innovative medical radioisotopes. However, the lack of experimental data on reaction cross sections for photonuclear reactions of medical radioisotopes of interest has severely limited the development and production of photonuclear transmutation medical radioisotopes. In this study, the entire process of the generation, decay, and measurement of medical radioisotopes was simulated using online gamma activation and offline gamma measurements combined with a shielding gamma-ray spectrometer. Based on a quasi-monochromatic gamma beam from the Shanghai Laser Electron Gamma Source (SLEGS), the feasibility of this measurement of production cross section for surveyed medical radioisotopes was simulated, and specific solutions for measuring medical radioisotopes with ultra-low production cross sections were provided. The feasibility of this method for high-precision measurements of the reaction cross section of medical radioisotopes was demonstrated.

In this study, we revisit the previous mass relations of mirror nuclei by considering 1/N- and 1/Z-dependent terms and the shell effect across a shell. The root-mean-squared deviation is 66 keV for 116 nuclei with neutron number (N ge 10), as compared with experimental data compiled in the AME2020 database. The predicted mass excesses of 173 proton-rich nuclei, including 98 unknown nuclei, are tabulated in the Supplemental Material herein with competitive accuracy.

As a complement to X-ray computed tomography (CT), neutron tomography has been extensively used in nuclear engineering, materials science, cultural heritage, and industrial applications. Reconstruction of the attenuation matrix for neutron tomography with a traditional analytical algorithm requires hundreds of projection views in the range of 0° to 180° and typically takes several hours to complete. Such a low time-resolved resolution degrades the quality of neutron imaging. Decreasing the number of projection acquisitions is an important approach to improve the time resolution of images; however, this requires efficient reconstruction algorithms. Therefore, sparse-view reconstruction algorithms in neutron tomography need to be investigated. In this study, we investigated the three-dimensional reconstruction algorithm for sparse-view neutron CT scans. To enhance the reconstructed image quality of neutron CT, we propose an algorithm that uses OS-SART to reconstruct images and a split Bregman to solve for the total variation (SBTV). A comparative analysis of the performances of each reconstruction algorithm was performed using simulated and actual experimental data. According to the analyzed results, OS-SART-SBTV is superior to the other algorithms in terms of denoising, suppressing artifacts, and preserving detailed structural information of images.