预混合崖体稳定碳氢化合物-空气火焰和氨气/氢气/氮气-空气火焰的稀薄吹脱行为

Tong Su, Boyan Xu, Rob J. M. Bastiaans, Nicholas Worth
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引用次数: 0

摘要

研究了湍流预混合崖体稳定碳氢化合物火焰和氨/氢/氮火焰的贫化吹脱(LBO)行为,并对其进行了实验和数值比较。同时采用高速 PIV 和 OH-PLIF 来解析火焰和流场的时间信息,从而计算出火焰表面的曲率和流体动力应变率。此外,还使用 OH* 和 NH2* 化学发光图像来检查相同体积流速下的火焰结构,以及从远离 LBO 到靠近 LBO 的四种等效比率下的火焰结构。与甲烷和丙烷火焰相比,在 20 米/秒的速度下,NH3/H2/N2(70%/22.5%/7.5%)火焰对 LBO 的抵抗力稍强。在接近贫油吹脱时,碳氢化合物火焰结构从 "V 形 "变为 "M 形",导致反应不完全,最终引发 LBO。然而,氨气混合物火焰根部附近剪切层中强烈的 OH* 强度表明,反应非常剧烈,可以提高火焰的稳定性。沿 NH3/H2/N2 火焰表面广泛分布的正曲率(Le<1)也可促进燃烧。由于火焰形状和位置的剧烈变化较小,NH3/H2/N2 火焰前沿的应变率变化也较小,这可以扩大稳定性极限。此外,氨气混合物火焰的焰根附近氢气消耗速度较快,而且与绝热温度相比温度损失较低,这也有助于氨气混合物在接近贫气吹脱时保持稳定。
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Lean Blow-Off Behaviour of Premixed Bluff-Body Stabilized Hydrocarbon-Air Flames and Ammonia/Hydrogen/Nitrogen-Air Flames
The lean blow-off (LBO) behavior of turbulent premixed bluff-body stabilized hydrocarbon flames and ammonia/hydrogen/nitrogen flame is investigated and compared both experimentally and numerically. Simultaneous high-speed PIV and OH-PLIF are employed to resolve temporal flame and flow field information, allowing the curvature and hydrodynamic strain rates along the flame surfaces to be calculated. OH* and NH2* chemiluminescence images are also used to examine flame structures at the same bulk flow velocity but at four equivalence ratios from far away from to near LBO. A NH3/H2/N2 (70%/22.5%/7.5%) flame is slightly more resilient to LBO compared with methane and propane flames at 20 m/s. The hydrocarbon flame structures change from 'V-shape' to 'M-shape' when approaching lean blow-off, resulting in incomplete reactions and finally trigger the LBO. However, the strong OH* intensity in the shear layer near flame root for the ammonia blend flames indicate a robust reaction which can increase flame stability. Widely-distributed positive curvature along the flame surface of the NH3/H2/N2 flames (Le<1) may also enhance combustion. The less strain rates change along NH3/H2/N2 flames fronts due to less dramatic changes to the flame shape and position can extend the stability limits. Furthermore, the faster consumption rates of hydrogen near the flame root for the ammonia blend flames, and the lower temperature loss compared with the adiabatic temperature also contribute to the stabilization of ammonia blends near lean blow-off.
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