通过蚀刻橄榄石中快速重离子轨迹的方法合成非圆截面纳米孔时离子速度的影响

S. A. Gorbunov, P. A. Babaev, A. E. Volkov, R. A. Voronkov, R. A. Rymzhanov
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引用次数: 0

摘要

摘要 研究了离子速度对通过快速重离子在橄榄石中的蚀刻轨迹合成非圆形截面纳米孔的影响。所建立的迅猛重离子辐照橄榄石蚀刻原子模型预测了在橄榄石中合成非圆形截面纳米孔的可能性。该模型由描述轨道形成和蚀刻顺序阶段的连接块组成。TREKIS 蒙特卡罗模型描述了入射离子轨迹纳米级附近的初始电子和晶格激发。这些结果被用作分子动力学模拟离子轨迹结构变化的初始条件。结构受损区域冷却后获得的原子坐标可作为橄榄石轨道蚀刻原始原子模型的初始数据。该模型的应用结果表明,通过改变晶体相对于辐照方向的取向,可以控制所产生的纳米孔的横截面。所展示的 Xe 离子模拟结果表明,所产生孔隙的大小取决于入射离子的速度,而不仅仅取决于其线性能量损失。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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On the Effect of Ion Velocity in the Synthesis of Nanopores with a Noncircular Cross Section by the Method of Etching Tracks of Swift Heavy Ions in Olivine

The effect of ion velocity in the synthesis of nanopores with a noncircular cross section by the etching tracks of swift heavy ions in olivine is studied. The developed atomistic model of the etching of olivine irradiated with swift heavy ions predicts the possibility of synthesizing nanopores with a noncircular cross section in it. The model consists of connected blocks that describe the sequential stages of track formation and etching. The TREKIS Monte Carlo model describes the initial electronic and lattice excitations in the nanoscale vicinity of the trajectory of an incident ion. These results are used as initial conditions for the molecular-dynamics simulation of structural changes along the ion trajectory. The obtained atomic coordinates after cooling of the structurally damaged region serve as the initial data for an original atomistic model of track etching in olivine. The results of application of the model demonstrate that it is possible to control the cross section of resulting nanopores by changing the orientation of the crystal relative to the direction of irradiation. The presented simulation results for Xe ions demonstrate that the size of the resulting pores depends on the velocity of the incident ion, and not only on its linear energy losses.

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来源期刊
CiteScore
0.90
自引率
25.00%
发文量
144
审稿时长
3-8 weeks
期刊介绍: Journal of Surface Investigation: X-ray, Synchrotron and Neutron Techniques publishes original articles on the topical problems of solid-state physics, materials science, experimental techniques, condensed media, nanostructures, surfaces of thin films, and phase boundaries: geometric and energetical structures of surfaces, the methods of computer simulations; physical and chemical properties and their changes upon radiation and other treatments; the methods of studies of films and surface layers of crystals (XRD, XPS, synchrotron radiation, neutron and electron diffraction, electron microscopic, scanning tunneling microscopic, atomic force microscopic studies, and other methods that provide data on the surfaces and thin films). Articles related to the methods and technics of structure studies are the focus of the journal. The journal accepts manuscripts of regular articles and reviews in English or Russian language from authors of all countries. All manuscripts are peer-reviewed.
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