Zhaoyu Liu, Yue Shi, Qianni Jiang, Elliott W. Rosenberg, Jonathan M. DeStefano, Jinjin Liu, Chaowei Hu, Yuzhou Zhao, Zhiwei Wang, Yugui Yao, David Graf, Pengcheng Dai, Jihui Yang, Xiaodong Xu, Jiun-Haw Chu
{"title":"卡戈米金属 CsV3Sb5 中不存在 E2g 向列不稳定性和占主导地位的 A1g 响应","authors":"Zhaoyu Liu, Yue Shi, Qianni Jiang, Elliott W. Rosenberg, Jonathan M. DeStefano, Jinjin Liu, Chaowei Hu, Yuzhou Zhao, Zhiwei Wang, Yugui Yao, David Graf, Pengcheng Dai, Jihui Yang, Xiaodong Xu, Jiun-Haw Chu","doi":"10.1103/physrevx.14.031015","DOIUrl":null,"url":null,"abstract":"Ever since the discovery of the charge density wave (CDW) transition in the kagome metal <math display=\"inline\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><msub><mrow><mi>CsV</mi></mrow><mrow><mn>3</mn></mrow></msub></mrow><mrow><msub><mrow><mi>Sb</mi></mrow><mrow><mn>5</mn></mrow></msub></mrow></math>, the nature of its symmetry breaking has been under intense debate. While evidence suggests that the rotational symmetry is already broken at the CDW transition temperature (<math display=\"inline\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><msub><mi>T</mi><mrow><mi>CDW</mi></mrow></msub></math>), an additional electronic nematic instability well below <math display=\"inline\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><msub><mi>T</mi><mrow><mi>CDW</mi></mrow></msub></math> has been reported based on the diverging elastoresistivity coefficient in the anisotropic channel (<math display=\"inline\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><msub><mi>m</mi><msub><mi>E</mi><mrow><mn>2</mn><mi>g</mi></mrow></msub></msub></math>). Verifying the existence of a nematic transition below <math display=\"inline\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><msub><mi>T</mi><mrow><mi>CDW</mi></mrow></msub></math> is not only critical for establishing the correct description of the CDW order parameter, but also important for understanding low-temperature superconductivity. Here, we report elastoresistivity measurements of <math display=\"inline\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><msub><mrow><mi>CsV</mi></mrow><mrow><mn>3</mn></mrow></msub></mrow><mrow><msub><mrow><mi>Sb</mi></mrow><mrow><mn>5</mn></mrow></msub></mrow></math> using three different techniques probing both isotropic and anisotropic symmetry channels. Contrary to previous reports, we find the anisotropic elastoresistivity coefficient <math display=\"inline\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><msub><mi>m</mi><msub><mi>E</mi><mrow><mn>2</mn><mi>g</mi></mrow></msub></msub></math> is temperature independent, except for a step jump at <math display=\"inline\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><msub><mi>T</mi><mrow><mi>CDW</mi></mrow></msub></math>. The absence of nematic fluctuations is further substantiated by measurements of the elastocaloric effect, which show no enhancement associated with nematic susceptibility. On the other hand, the symmetric elastoresistivity coefficient <math display=\"inline\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><msub><mi>m</mi><msub><mi>A</mi><mrow><mn>1</mn><mi>g</mi></mrow></msub></msub></math> increases below <math display=\"inline\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><msub><mi>T</mi><mrow><mi>CDW</mi></mrow></msub></math>, reaching a peak value of 90 at <math display=\"inline\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><msup><mi>T</mi><mo>*</mo></msup><mo>=</mo><mn>20</mn><mtext> </mtext><mtext> </mtext><mi mathvariant=\"normal\">K</mi></math>. Our results strongly indicate that the phase transition at <math display=\"inline\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><msup><mi>T</mi><mo>*</mo></msup></math> is not nematic in nature and the previously reported diverging elastoresistivity is due to the contamination from the <math display=\"inline\" xmlns=\"http://www.w3.org/1998/Math/MathML\"><msub><mi>A</mi><mrow><mn>1</mn><mi>g</mi></mrow></msub></math> channel.","PeriodicalId":20161,"journal":{"name":"Physical Review X","volume":"48 1","pages":""},"PeriodicalIF":11.6000,"publicationDate":"2024-07-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Absence of E2g Nematic Instability and Dominant A1g Response in the Kagome Metal CsV3Sb5\",\"authors\":\"Zhaoyu Liu, Yue Shi, Qianni Jiang, Elliott W. Rosenberg, Jonathan M. DeStefano, Jinjin Liu, Chaowei Hu, Yuzhou Zhao, Zhiwei Wang, Yugui Yao, David Graf, Pengcheng Dai, Jihui Yang, Xiaodong Xu, Jiun-Haw Chu\",\"doi\":\"10.1103/physrevx.14.031015\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Ever since the discovery of the charge density wave (CDW) transition in the kagome metal <math display=\\\"inline\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mrow><msub><mrow><mi>CsV</mi></mrow><mrow><mn>3</mn></mrow></msub></mrow><mrow><msub><mrow><mi>Sb</mi></mrow><mrow><mn>5</mn></mrow></msub></mrow></math>, the nature of its symmetry breaking has been under intense debate. While evidence suggests that the rotational symmetry is already broken at the CDW transition temperature (<math display=\\\"inline\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><msub><mi>T</mi><mrow><mi>CDW</mi></mrow></msub></math>), an additional electronic nematic instability well below <math display=\\\"inline\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><msub><mi>T</mi><mrow><mi>CDW</mi></mrow></msub></math> has been reported based on the diverging elastoresistivity coefficient in the anisotropic channel (<math display=\\\"inline\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><msub><mi>m</mi><msub><mi>E</mi><mrow><mn>2</mn><mi>g</mi></mrow></msub></msub></math>). Verifying the existence of a nematic transition below <math display=\\\"inline\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><msub><mi>T</mi><mrow><mi>CDW</mi></mrow></msub></math> is not only critical for establishing the correct description of the CDW order parameter, but also important for understanding low-temperature superconductivity. Here, we report elastoresistivity measurements of <math display=\\\"inline\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mrow><msub><mrow><mi>CsV</mi></mrow><mrow><mn>3</mn></mrow></msub></mrow><mrow><msub><mrow><mi>Sb</mi></mrow><mrow><mn>5</mn></mrow></msub></mrow></math> using three different techniques probing both isotropic and anisotropic symmetry channels. Contrary to previous reports, we find the anisotropic elastoresistivity coefficient <math display=\\\"inline\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><msub><mi>m</mi><msub><mi>E</mi><mrow><mn>2</mn><mi>g</mi></mrow></msub></msub></math> is temperature independent, except for a step jump at <math display=\\\"inline\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><msub><mi>T</mi><mrow><mi>CDW</mi></mrow></msub></math>. The absence of nematic fluctuations is further substantiated by measurements of the elastocaloric effect, which show no enhancement associated with nematic susceptibility. On the other hand, the symmetric elastoresistivity coefficient <math display=\\\"inline\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><msub><mi>m</mi><msub><mi>A</mi><mrow><mn>1</mn><mi>g</mi></mrow></msub></msub></math> increases below <math display=\\\"inline\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><msub><mi>T</mi><mrow><mi>CDW</mi></mrow></msub></math>, reaching a peak value of 90 at <math display=\\\"inline\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><msup><mi>T</mi><mo>*</mo></msup><mo>=</mo><mn>20</mn><mtext> </mtext><mtext> </mtext><mi mathvariant=\\\"normal\\\">K</mi></math>. Our results strongly indicate that the phase transition at <math display=\\\"inline\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><msup><mi>T</mi><mo>*</mo></msup></math> is not nematic in nature and the previously reported diverging elastoresistivity is due to the contamination from the <math display=\\\"inline\\\" xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><msub><mi>A</mi><mrow><mn>1</mn><mi>g</mi></mrow></msub></math> channel.\",\"PeriodicalId\":20161,\"journal\":{\"name\":\"Physical Review X\",\"volume\":\"48 1\",\"pages\":\"\"},\"PeriodicalIF\":11.6000,\"publicationDate\":\"2024-07-29\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Physical Review X\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://doi.org/10.1103/physrevx.14.031015\",\"RegionNum\":1,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"PHYSICS, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Physical Review X","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1103/physrevx.14.031015","RegionNum":1,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"PHYSICS, MULTIDISCIPLINARY","Score":null,"Total":0}
Absence of E2g Nematic Instability and Dominant A1g Response in the Kagome Metal CsV3Sb5
Ever since the discovery of the charge density wave (CDW) transition in the kagome metal , the nature of its symmetry breaking has been under intense debate. While evidence suggests that the rotational symmetry is already broken at the CDW transition temperature (), an additional electronic nematic instability well below has been reported based on the diverging elastoresistivity coefficient in the anisotropic channel (). Verifying the existence of a nematic transition below is not only critical for establishing the correct description of the CDW order parameter, but also important for understanding low-temperature superconductivity. Here, we report elastoresistivity measurements of using three different techniques probing both isotropic and anisotropic symmetry channels. Contrary to previous reports, we find the anisotropic elastoresistivity coefficient is temperature independent, except for a step jump at . The absence of nematic fluctuations is further substantiated by measurements of the elastocaloric effect, which show no enhancement associated with nematic susceptibility. On the other hand, the symmetric elastoresistivity coefficient increases below , reaching a peak value of 90 at . Our results strongly indicate that the phase transition at is not nematic in nature and the previously reported diverging elastoresistivity is due to the contamination from the channel.
期刊介绍:
Physical Review X (PRX) stands as an exclusively online, fully open-access journal, emphasizing innovation, quality, and enduring impact in the scientific content it disseminates. Devoted to showcasing a curated selection of papers from pure, applied, and interdisciplinary physics, PRX aims to feature work with the potential to shape current and future research while leaving a lasting and profound impact in their respective fields. Encompassing the entire spectrum of physics subject areas, PRX places a special focus on groundbreaking interdisciplinary research with broad-reaching influence.