利用纳米金刚石组合中的氮空位中心在金刚石砧电池中进行磁测量。

IF 16.4 1区 化学 Q1 CHEMISTRY, MULTIDISCIPLINARY Accounts of Chemical Research Pub Date : 2024-08-01 DOI:10.1063/5.0216877
David P Shelton, Waldo Cabriales, Ashkan Salamat
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引用次数: 0

摘要

利用带负电荷的氮空位(NV-)中心进行光学磁测量的新兴领域为空间分辨物理特性测量提供了一种高灵敏度的实验室工作台技术。由于其他技术往往受限于样品室的空间限制,因此在高压金刚石砧室(DAC)环境中实施这种技术将变得非常普遍。这里描述的仪器和技术允许在 DAC 内使用连续波光学检测磁共振对纳米金刚石层中的 NV- 中心进行更普遍的磁场测量。微带天线可为 DAC 提供均匀的微波场,并与简单的金属垫圈兼容,而沉积纳米金刚石的传感器层可简单测定 B 在 1-100 G 范围内的磁场大小。利用该仪器测量了铁在 18 GPa 下的铁磁转变及其滞后响应。
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Magnetometry in a diamond anvil cell using nitrogen vacancy centers in a nanodiamond ensemble.

The emerging field of optical magnetometry utilizing negative-charged nitrogen vacancy (NV-) centers provides a highly sensitive lab bench technique for spatially resolved physical property measurements. Their implementation in high pressure diamond anvil cell (DAC) environments will become common as other techniques are often limited due to the spatial constraints of the sample chamber. Apparatus and techniques are described here permitting for more general use of magnetic field measurements inside a DAC using continuous wave optical detected magnetic resonance in NV- centers in a layer of nanodiamonds. A microstrip antenna delivers a uniform microwave field to the DAC and is compatible with simple metal gaskets, and the sensor layer of deposited nanodiamonds allows for simple determination of the magnetic field magnitude for B in the 1-100 G range. The ferromagnetic transition in iron at 18 GPa is measured with the apparatus, along with its hysteretic response.

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来源期刊
Accounts of Chemical Research
Accounts of Chemical Research 化学-化学综合
CiteScore
31.40
自引率
1.10%
发文量
312
审稿时长
2 months
期刊介绍: Accounts of Chemical Research presents short, concise and critical articles offering easy-to-read overviews of basic research and applications in all areas of chemistry and biochemistry. These short reviews focus on research from the author’s own laboratory and are designed to teach the reader about a research project. In addition, Accounts of Chemical Research publishes commentaries that give an informed opinion on a current research problem. Special Issues online are devoted to a single topic of unusual activity and significance. Accounts of Chemical Research replaces the traditional article abstract with an article "Conspectus." These entries synopsize the research affording the reader a closer look at the content and significance of an article. Through this provision of a more detailed description of the article contents, the Conspectus enhances the article's discoverability by search engines and the exposure for the research.
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