用于太赫兹生物传感的同时支持连续模式和无极模式准结合态的不对称哑铃二聚体

IF 6.5 2区 物理与天体物理 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Nanophotonics Pub Date : 2024-07-31 DOI:10.1515/nanoph-2024-0254
Jixin Feng, Xianghui Wang, Weinan Shi, Liang Ma, Yunyun Ji, Fei Fan, Shengjiang Chang
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引用次数: 0

摘要

多共振元表面在多波段纳米光子学应用中具有重要意义。在这里,我们提出了一种新颖的元表面设计方案,用于同时支持连续体准束缚态(QBIC)和其他共振模式,其中 QBIC 共振是通过打破低聚物中的镜像或旋转对称性产生的,而其他共振模式则可以通过合理设计低聚物中元原子的形状同时激发。例如,在一个由不对称哑铃形孔组成的二聚体元表面中,QBIC 和无极模式被同时激发。基于远场多极分解和近场电磁场分布,阐明了 QBIC 和anapole 模式的起源机制。哑铃形二聚体的对称性破缺导致了 QBIC。在一定的不对称变化范围内,环偶极矩和电偶极矩的贡献大小大致相等,但仍占主导地位,这使得无极模式始终存在。与数值模拟结果相同的实验结果进一步证实了所提设计方案的有效性。在太赫兹生物传感实验中,无极模式的灵敏度高达 271.3 GHz (nmol/μl)-1,而 QBIC 可达到 0.015 nmol/μl 的较低检测限,并将检测范围扩大了近一个数量级。我们的发现有利于设计具有不同共振模式的多共振元表面,并促进其在生物传感、激光、滤波和非线性领域的相应应用。
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Asymmetric dumbbell dimers simultaneously supporting quasi-bound states in continuum and anapole modes for terahertz biosensing
Multi-resonant metasurfaces are of great significance in the applications of multi-band nanophotonics. Here, we propose a novel metasurface design scheme for simultaneously supporting quasi-bound states in continuum (QBIC) and other resonant modes, in which QBIC resonance is generated by mirror or rotational symmetry breaking in oligomers while other resonant modes can be simultaneously excited by rationally designing the shapes of meta-atoms within oligomers. As an example, the simultaneous excitation of QBIC and anapole modes are demonstrated in a dimer metasurface composed of asymmetric dumbbell-shaped apertures. Based on the far-field multipole decomposition and near-field electromagnetic field distributions, the origin mechanisms of QBIC and anapole mode are elucidated. The symmetry breaking of dumbbell-shaped dimer results in QBIC. Within a certain asymmetric variation range, the contributions of toroidal dipole moment and electric dipole moment with approximately equal magnitudes remain dominant, which allows the anapole mode to always present. The effectiveness of the proposed design scheme is further confirmed by the experimental results identical with the evolutions of numerical simulation. In terahertz biosensing experiments, the anapole mode exhibits a higher sensitivity of 271.3 GHz (nmol/μl)−1, whereas the QBIC can achieve a lower detection limit of 0.015 nmol/μl and expands the detection range by almost an order of magnitude. Our findings are beneficial to designing multi-resonant metasurfaces with different resonance modes and promote the corresponding applications in the fields of biosensing, lasers, filtering, and nonlinearity.
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来源期刊
Nanophotonics
Nanophotonics NANOSCIENCE & NANOTECHNOLOGY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
13.50
自引率
6.70%
发文量
358
审稿时长
7 weeks
期刊介绍: Nanophotonics, published in collaboration with Sciencewise, is a prestigious journal that showcases recent international research results, notable advancements in the field, and innovative applications. It is regarded as one of the leading publications in the realm of nanophotonics and encompasses a range of article types including research articles, selectively invited reviews, letters, and perspectives. The journal specifically delves into the study of photon interaction with nano-structures, such as carbon nano-tubes, nano metal particles, nano crystals, semiconductor nano dots, photonic crystals, tissue, and DNA. It offers comprehensive coverage of the most up-to-date discoveries, making it an essential resource for physicists, engineers, and material scientists.
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