迈向循环碳经济:二氧化碳捕集与综合利用的最新发展与技术经济评估

IF 2.2 4区 化学 Q2 Engineering Chemical Papers Pub Date : 2024-08-01 DOI:10.1007/s11696-024-03610-3
Xing Gang Zhang, Archina Buthiyappan, Nuradila Zahirah Mohd Azmi, Abdul Aziz Abdul Raman
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摘要

文章回顾了二氧化碳综合捕集与利用(ICCU)的最新进展,与传统的碳捕集与利用相比,ICCU 具有多种优势。文章对基于同质吸附和催化系统以及异质材料的各种 ICCU 工艺进行了点评。由于 ICCU 工艺中吸附和催化过程的配置各不相同,异质材料可以以各种形式加以利用,包括吸附剂和催化剂的叠加、物理混合和双功能材料的使用。此外,还研究了各种环保、再生简单、能耗低的双功能材料的开发,这些材料可用于二氧化碳捕集与水气反向变换反应(ICCU-RWGS)、二氧化碳捕集与甲烷干重整(ICCU-DRM)以及二氧化碳捕集与甲烷化(ICCU-Methanation)。还详细讨论了合成双功能材料的组件选择和操作参数的影响。此外,为了考虑大规模的工业应用,本综述还包括 ICCU 的技术经济和环境评估。综述认为,与碳捕集与封存和碳捕集与利用相比,ICCU 在技术、经济和环境方面都具有优势。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Towards circular carbon economy: recent developments and techno-economic assessment of integrated carbon dioxide capture and utilization

The article reviews the latest advances in integrated CO2 capture and utilization (ICCU), which presents several benefits over conventional carbon capture and utilization. A variety of ICCU processes based on homogeneous adsorption and catalytic systems, as well as heterogeneous materials are reviewed critically in the article. Due to the varying configurations of adsorption and catalytic processes in the ICCU process, heterogeneous materials can be utilized in various forms, including the superposition of adsorbent and catalyst, physical mixing and the use of dual-functional materials. The development of various bifunctional materials that are eco-friendly, simple to regenerate, and consume less energy for integrated CO2 capture and reverse water–gas shift reaction (ICCU-RWGS), integrated CO2 capture and dry reforming of methane (ICCU-DRM), and integrated CO2 capture and methanation (ICCU-Methanation) has also been investigated. A detailed discussion has also been conducted on the selection of components and the effect of operating parameters to synthesize bifunctional materials. Additionally, in order to consider large scale industrial applications this review also included techno-economic and environmental assessments of ICCU. The review concluded that Compared to carbon capture and storage and carbon capture and utilization, ICCU offers advantages in terms of technology, economy, and the environment.

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来源期刊
Chemical Papers
Chemical Papers Chemical Engineering-General Chemical Engineering
CiteScore
3.30
自引率
4.50%
发文量
590
期刊介绍: Chemical Papers is a peer-reviewed, international journal devoted to basic and applied chemical research. It has a broad scope covering the chemical sciences, but favors interdisciplinary research and studies that bring chemistry together with other disciplines.
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