耗碳混凝土(CCC):电弧炉还原渣的力学性能和碳吸收综合研究

IF 7.2 2区 工程技术 Q1 CHEMISTRY, MULTIDISCIPLINARY Journal of CO2 Utilization Pub Date : 2024-07-01 DOI:10.1016/j.jcou.2024.102889
Hong-Joon Choi , Taekgeun Oh , Namkon Lee , Indong Jang , Jung-Jun Park , Doo-Yeol Yoo
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引用次数: 0

摘要

本研究进行了一系列测试,以验证和评估碳消耗混凝土(CCC)的力学特性、孔隙结构和化学成分,该混凝土采用电弧炉(EAF)炉渣来提高碳消耗。根据电弧炉还原渣(ERS)粉末的水泥替代率和捕获二氧化碳(CO)的纳米气泡水的使用情况,对混合变量进行了分类。机械性能通过抗压强度测试进行评估,而在高浓度 CO 气氛中的收缩行为则通过比较自生收缩、干燥收缩和碳化收缩进行观察。基质均匀性是通过汞渗入孔隙度(MIP)分析确定的。能量色散光谱仪 (EDS) 制图、差热分析 (DTG)、傅立叶变换红外光谱仪 (FTIR) 和 X 射线衍射 (XRD) 被用来检测碳固定的数量和主要成分的产生。加入 ERS 对耐久性有积极的影响,如增加抗碳化收缩性和减少长期孔隙率。同时,由于主要成分的形成增加,抗压强度也有所提高。最终证实,ERS 的加入会对二氧化碳的消耗量产生积极影响。
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Carbon consuming concrete (CCC): A comprehensive study on mechanical properties and carbon uptake with electric arc furnace reduction slag

This study executed a series of tests to validate and assess the mechanical characteristics, pore structures, and chemical components of carbon consuming concrete (CCC), which employs an electric arc furnace (EAF) slag to enhance carbon consumption. Mixing variables were categorized based on the cement replacement ratio of electric arc furnace reduction slag (ERS) powder and the use of nanobubble water, which captured carbon dioxide (CO2). The mechanical performance was appraised through a compressive strength test, while the shrinkage behavior in a high-concentration CO2 atmosphere was observed to compare autogenous, drying, and carbonation shrinkage. Matrix homogeneity was determined through mercury intrusion porosimetry (MIP) analysis. Energy-dispersive spectrometer (EDS) mapping, differential thermogravimetry (DTG), Fourier transform infrared spectroscopy (FTIR), and X-ray diffraction (XRD) were employed to examine the quantity of carbon fixation and the production of major components. The inclusion of ERS exhibited positive impacts on durability, such as increasing carbonation shrinkage resistance and reducing porosity in the long term. Concurrently, enhancements in compressive strengths were observed owing to the elevated formation of major components. Ultimately, it was established that the incorporation of ERS positively influences the amount of CO2 consumption.

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来源期刊
Journal of CO2 Utilization
Journal of CO2 Utilization CHEMISTRY, MULTIDISCIPLINARY-ENGINEERING, CHEMICAL
CiteScore
13.90
自引率
10.40%
发文量
406
审稿时长
2.8 months
期刊介绍: The Journal of CO2 Utilization offers a single, multi-disciplinary, scholarly platform for the exchange of novel research in the field of CO2 re-use for scientists and engineers in chemicals, fuels and materials. The emphasis is on the dissemination of leading-edge research from basic science to the development of new processes, technologies and applications. The Journal of CO2 Utilization publishes original peer-reviewed research papers, reviews, and short communications, including experimental and theoretical work, and analytical models and simulations.
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