一氧化碳二聚化的直接阳离子稳定效应促进贵金属表面的二氧化碳还原 C2 途径

IF 6.2 Q2 ENERGY & FUELS Advanced Energy and Sustainability Research Pub Date : 2024-08-06 DOI:10.1002/aesr.202470022

Hon Ho Wong, Mingzi Sun, Tong Wu, Lu Lu, Qiuyang Lu, Baian Chen, Cheuk Hei Chan, Bolong Huang

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摘要

一氧化碳二聚化两个一氧化碳中间体的耦合是二氧化碳还原反应中形成 C2 产物的重要步骤。在文章编号 2400110 中，Bolong Huang 小组证明了阳离子-二聚体稳定性与反应能量之间的线性关系，从而证明阳离子显著促进了 C-C 偶联步骤并提高了 C2 产物的产量。

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Direct Cation Stabilization Effects of CO Dimerization for Boosting C2 Pathways of CO2 Reduction on Noble Metal Surfaces

CO Dimerization

The coupling of two CO intermediates represents a significant step in the formation of C₂ products during the carbon dioxide reduction reaction. In article number 2400110, Bolong Huang’s group demonstrates the linear correlation between the cation–dimer stabilization and reaction energy, supporting that the cations notably facilitate the C-C coupling step and enhance the production of C₂ products.

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来源期刊

Advanced Energy and Sustainability Research

CiteScore

8.20

自引率

3.40%

发文量

期刊介绍： Advanced Energy and Sustainability Research is an open access academic journal that focuses on publishing high-quality peer-reviewed research articles in the areas of energy harvesting, conversion, storage, distribution, applications, ecology, climate change, water and environmental sciences, and related societal impacts. The journal provides readers with free access to influential scientific research that has undergone rigorous peer review, a common feature of all journals in the Advanced series. In addition to original research articles, the journal publishes opinion, editorial and review articles designed to meet the needs of a broad readership interested in energy and sustainability science and related fields. In addition, Advanced Energy and Sustainability Research is indexed in several abstracting and indexing services, including： CAS: Chemical Abstracts Service (ACS) Directory of Open Access Journals (DOAJ) Emerging Sources Citation Index (Clarivate Analytics) INSPEC (IET) Web of Science (Clarivate Analytics).