{"title":"使用先进的 PtRu-CGO 催化剂进行创新的加压柴油重整以实现可持续制氢","authors":"","doi":"10.1016/j.enconman.2024.118973","DOIUrl":null,"url":null,"abstract":"<div><p>This study suggests a novel approach for producing hydrogen through the pressurized reforming of commercial diesel, leveraging the PtRu-CGO catalyst. Foundational experiments were performed with PtRu-CGO powder catalysts at conditions up to 9 bar and 800 °C, achieving complete fuel conversion and stable performance with an average hydrogen concentration of approximately 58.7 mol%. Additionally, the structured catalysts developed herein also could maintain high efficiency and durability under a gas hourly space velocity (GHSV) of 10,000 h<sup>−1</sup>. Notably, at 6 bar, the system exhibited an extraordinary efficiency of around 75 % over 300 h of continuous operation. These results underscore the practicality of pressurized diesel reforming for hydrogen production with the PtRu-CGO catalyst, highlighting its potential in the development and optimization of hydrogen energy systems and aiding the shift towards a hydrogen-based economy.</p></div>","PeriodicalId":11664,"journal":{"name":"Energy Conversion and Management","volume":null,"pages":null},"PeriodicalIF":9.9000,"publicationDate":"2024-09-04","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Innovative pressurized diesel reforming for sustainable hydrogen production using advanced PtRu-CGO catalyst\",\"authors\":\"\",\"doi\":\"10.1016/j.enconman.2024.118973\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>This study suggests a novel approach for producing hydrogen through the pressurized reforming of commercial diesel, leveraging the PtRu-CGO catalyst. Foundational experiments were performed with PtRu-CGO powder catalysts at conditions up to 9 bar and 800 °C, achieving complete fuel conversion and stable performance with an average hydrogen concentration of approximately 58.7 mol%. Additionally, the structured catalysts developed herein also could maintain high efficiency and durability under a gas hourly space velocity (GHSV) of 10,000 h<sup>−1</sup>. Notably, at 6 bar, the system exhibited an extraordinary efficiency of around 75 % over 300 h of continuous operation. These results underscore the practicality of pressurized diesel reforming for hydrogen production with the PtRu-CGO catalyst, highlighting its potential in the development and optimization of hydrogen energy systems and aiding the shift towards a hydrogen-based economy.</p></div>\",\"PeriodicalId\":11664,\"journal\":{\"name\":\"Energy Conversion and Management\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":9.9000,\"publicationDate\":\"2024-09-04\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Energy Conversion and Management\",\"FirstCategoryId\":\"5\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0196890424009142\",\"RegionNum\":1,\"RegionCategory\":\"工程技术\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENERGY & FUELS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Energy Conversion and Management","FirstCategoryId":"5","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0196890424009142","RegionNum":1,"RegionCategory":"工程技术","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENERGY & FUELS","Score":null,"Total":0}
Innovative pressurized diesel reforming for sustainable hydrogen production using advanced PtRu-CGO catalyst
This study suggests a novel approach for producing hydrogen through the pressurized reforming of commercial diesel, leveraging the PtRu-CGO catalyst. Foundational experiments were performed with PtRu-CGO powder catalysts at conditions up to 9 bar and 800 °C, achieving complete fuel conversion and stable performance with an average hydrogen concentration of approximately 58.7 mol%. Additionally, the structured catalysts developed herein also could maintain high efficiency and durability under a gas hourly space velocity (GHSV) of 10,000 h−1. Notably, at 6 bar, the system exhibited an extraordinary efficiency of around 75 % over 300 h of continuous operation. These results underscore the practicality of pressurized diesel reforming for hydrogen production with the PtRu-CGO catalyst, highlighting its potential in the development and optimization of hydrogen energy systems and aiding the shift towards a hydrogen-based economy.
期刊介绍:
The journal Energy Conversion and Management provides a forum for publishing original contributions and comprehensive technical review articles of interdisciplinary and original research on all important energy topics.
The topics considered include energy generation, utilization, conversion, storage, transmission, conservation, management and sustainability. These topics typically involve various types of energy such as mechanical, thermal, nuclear, chemical, electromagnetic, magnetic and electric. These energy types cover all known energy resources, including renewable resources (e.g., solar, bio, hydro, wind, geothermal and ocean energy), fossil fuels and nuclear resources.