使用先进的 PtRu-CGO 催化剂进行创新的加压柴油重整以实现可持续制氢

IF 9.9 1区 工程技术 Q1 ENERGY & FUELS Energy Conversion and Management Pub Date : 2024-09-04 DOI:10.1016/j.enconman.2024.118973
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引用次数: 0

摘要

本研究提出了一种利用 PtRu-CGO 催化剂通过商用柴油加压重整制氢的新方法。在高达 9 巴和 800 摄氏度的条件下,使用 PtRu-CGO 粉末催化剂进行了基础实验,实现了燃料的完全转化和稳定的性能,平均氢浓度约为 58.7 摩尔%。此外,本文开发的结构催化剂还能在气体时空速度(GHSV)为 10,000 h-1 的条件下保持高效率和耐用性。值得注意的是,在 6 巴的条件下,该系统在连续运行 300 小时后显示出约 75% 的超常效率。这些结果证明了使用 PtRu-CGO 催化剂进行加压柴油重整制氢的实用性,突出了其在开发和优化氢能系统方面的潜力,并有助于向氢基经济转变。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Innovative pressurized diesel reforming for sustainable hydrogen production using advanced PtRu-CGO catalyst

This study suggests a novel approach for producing hydrogen through the pressurized reforming of commercial diesel, leveraging the PtRu-CGO catalyst. Foundational experiments were performed with PtRu-CGO powder catalysts at conditions up to 9 bar and 800 °C, achieving complete fuel conversion and stable performance with an average hydrogen concentration of approximately 58.7 mol%. Additionally, the structured catalysts developed herein also could maintain high efficiency and durability under a gas hourly space velocity (GHSV) of 10,000 h−1. Notably, at 6 bar, the system exhibited an extraordinary efficiency of around 75 % over 300 h of continuous operation. These results underscore the practicality of pressurized diesel reforming for hydrogen production with the PtRu-CGO catalyst, highlighting its potential in the development and optimization of hydrogen energy systems and aiding the shift towards a hydrogen-based economy.

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来源期刊
Energy Conversion and Management
Energy Conversion and Management 工程技术-力学
CiteScore
19.00
自引率
11.50%
发文量
1304
审稿时长
17 days
期刊介绍: The journal Energy Conversion and Management provides a forum for publishing original contributions and comprehensive technical review articles of interdisciplinary and original research on all important energy topics. The topics considered include energy generation, utilization, conversion, storage, transmission, conservation, management and sustainability. These topics typically involve various types of energy such as mechanical, thermal, nuclear, chemical, electromagnetic, magnetic and electric. These energy types cover all known energy resources, including renewable resources (e.g., solar, bio, hydro, wind, geothermal and ocean energy), fossil fuels and nuclear resources.
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