中国西南邛海湖湿地土壤中重金属和微塑料的污染程度及分布特征

IF 7.2 1区 地球科学 Q1 GEOSCIENCES, MULTIDISCIPLINARY Gondwana Research Pub Date : 2024-08-29 DOI:10.1016/j.gr.2024.07.027
Jinjin Wang , Zailin Chen , Xuemei Wang , Yanqun Wang , Huibin Shi , Yi Huang
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引用次数: 0

摘要

据报道,城市湿地是积累 HMs 和 MPs 的理想栖息地。然而,有关城市湿地环境中土壤中 HMs 和 MPs 复合污染的研究却很少见。本研究采用 ICP-MS 和傅立叶变换红外光谱法研究了中国西南地区琼海湖湿地土壤中 HMs 和 MPs 的特征。结果表明,土壤中 HMs 的平均浓度为 0.84 至 552.75(mg/kg)。根据 EF 和 Igeo 分析结果,土壤中的镉和铬呈显著富集(EF=12.64)和中度富集(EF=2.09),处于中度至重度污染水平(Igeo=2.83)和未受污染至中度污染水平(Igeo=0.23),其他元素处于较低水平。MPs是土壤环境中新出现的微污染物,M1、M2、M3、M4、M8和M9站土壤中MPs的丰度(件/克)分别为3.90、7.00、3.10、3.40、14.80和1.10,平均为5.55±4.92。微塑料的主要形状是薄膜,占 81.55%,其次是纤维,占 11.33%。粒径为 0.1-0.5 毫米的微塑料比例最高。多孔塑料的主要颜色为黑色、蓝色和绿色。根据傅立叶变换红外光谱鉴定,聚乙烯(PE)和聚丙烯(PP)是主要的 MP 材料,分别占 MP 总量的 52.16 % 和 42.31 %。MPs的污染负荷指数(PLI)为2.2,属于Ⅰ级污染。对城市湿地土壤中 HMs 和 MPs 的研究仍处于初步阶段。我们的目的是为评价城市湿地土壤中这两种污染物的污染状况和相关风险提供一个全新的视角,同时也为湿地土壤污染物的后续研究提供有价值的参考。
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Pollution level and distribution characteristics of heavy metals and microplastics in the soils from the Qionghai Lake Wetland, Southwest China

Urban wetlands are reported to be ideal habitats for accumulation of HMs and MPs. However, study on combined pollution of HMs and MPs in soil is rare in urban wetland environment. In this study, the characteristics of HMs and MPs in the soils of the Qionghai Lake wetland in southwest China were studied by using ICP–MS, and FTIR. The results showed that the average concentration of HMs in soil ranges from 0.84 to 552.75 (mg/kg). According to the EF and Igeo analysis results, Cd and Cr in the soil were significant enriched (EF=12.64) and moderately enriched (EF=2.09), and were at the moderate to heavy pollution level (Igeo = 2.83) and the unpolluted to moderate pollution level (Igeo = 0.23), and the other elements were at a low level. MPs are emerging micropollutants in the soil environment, and the abundance (pieces/g) of MPs in the soil was 3.90, 7.00, 3.10, 3.40, 14.80, and 1.10 at Stations M1, M2, M3, M4, M8, and M9, respectively, with an average of 5.55 ± 4.92. Films represented the main microplastic shape, accounting for 81.55 %, followed by fibers, accounting for 11.33 %. The proportion of MPs with a particle size of 0.1–0.5 mm is the highest. Black, blue, and green are the predominant colors found in MPs. Polyethylene (PE) and polypropylene (PP) were the main MP materials based on FTIR identification, accounting for 52.16 % and 42.31 % of the total MPs, respectively. The pollution load index (PLI) of MPs was 2.2, which is a level Ⅰ pollution. The research on HMs and MPs in urban wetland soil is still in its preliminary stage. Our aim is to offer a fresh perspective for evaluating the pollution status and risk associated with these two pollutants in urban wetland soil, while also providing a valuable reference for subsequent studies on wetland soil pollutants.

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来源期刊
Gondwana Research
Gondwana Research 地学-地球科学综合
CiteScore
12.90
自引率
6.60%
发文量
298
审稿时长
65 days
期刊介绍: Gondwana Research (GR) is an International Journal aimed to promote high quality research publications on all topics related to solid Earth, particularly with reference to the origin and evolution of continents, continental assemblies and their resources. GR is an "all earth science" journal with no restrictions on geological time, terrane or theme and covers a wide spectrum of topics in geosciences such as geology, geomorphology, palaeontology, structure, petrology, geochemistry, stable isotopes, geochronology, economic geology, exploration geology, engineering geology, geophysics, and environmental geology among other themes, and provides an appropriate forum to integrate studies from different disciplines and different terrains. In addition to regular articles and thematic issues, the journal invites high profile state-of-the-art reviews on thrust area topics for its column, ''GR FOCUS''. Focus articles include short biographies and photographs of the authors. Short articles (within ten printed pages) for rapid publication reporting important discoveries or innovative models of global interest will be considered under the category ''GR LETTERS''.
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