V.N. Santhosh , B.L. Madhavan , M. Venkat Ratnam , Dinesh N. Naik
{"title":"气溶胶特性的柱状分布与垂直分布对短波辐射效应调制的影响","authors":"V.N. Santhosh , B.L. Madhavan , M. Venkat Ratnam , Dinesh N. Naik","doi":"10.1016/j.jqsrt.2024.109179","DOIUrl":null,"url":null,"abstract":"<div><p>Quantifying the interaction of atmospheric aerosols with incoming solar radiation remains a challenge owing to the limitations associated with measuring aerosol optical properties. This study investigates how the distribution of aerosol properties, whether columnar or vertical, affects the aerosol radiative forcing (ARF) and heating rates (HRs) across different atmospheric layers under cloud-free conditions in the shortwave region. We also assess the atmospheric parameters, namely, pressure, temperature, water vapour density, and ozone density, from in-situ measurements, reanalysis data, and a standard tropical atmosphere to understand their impact on ARF and HR estimates across seasons. Our findings show that aerosol absorption is highest during monsoon, while it is lowest in the winter. Significant atmospheric warming due to aerosols resulted from the substantial cooling at the surface. Columnar properties of aerosols measured at limited or multiple wavelengths yield similar ARF and HR estimates, provided spectral dependency is considered using the Angstrom exponent across seasons. However, the vertical profiles of aerosol extinction, together with a constant single scattering albedo (SSA) along the atmospheric column versus an actual SSA profile, led to notable differences in ARF and HRs, specifically in pre-monsoon and monsoon periods. Free tropospheric aerosol absorption is underestimated when using columnar properties compared to vertical distribution, while boundary layer absorption is overestimated (> 10 Wm<sup>-2</sup>). The heterogeneity in aerosol types across atmospheric layers significantly influenced aerosol absorption, highlighting the importance of accurate vertical distribution information. HR profiles obtained with vertical distribution reflect the structure of aerosol extinction, whereas those estimated with columnar properties result in smoother profiles that fail to capture altitude gradients. Aerosol-induced HRs are higher within the boundary layer and free troposphere in the monsoon season for all scenarios of defined aerosol properties. These findings underscore the need for actual vertical profile measurements of aerosol properties to quantify aerosol radiation interaction.</p></div>","PeriodicalId":16935,"journal":{"name":"Journal of Quantitative Spectroscopy & Radiative Transfer","volume":"329 ","pages":"Article 109179"},"PeriodicalIF":2.3000,"publicationDate":"2024-09-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S0022407324002863/pdfft?md5=a72790ae85bf0f67eb1137d0ce525196&pid=1-s2.0-S0022407324002863-main.pdf","citationCount":"0","resultStr":"{\"title\":\"Influence of columnar versus vertical distribution of aerosol properties on the modulation of shortwave radiative effects\",\"authors\":\"V.N. Santhosh , B.L. Madhavan , M. Venkat Ratnam , Dinesh N. Naik\",\"doi\":\"10.1016/j.jqsrt.2024.109179\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Quantifying the interaction of atmospheric aerosols with incoming solar radiation remains a challenge owing to the limitations associated with measuring aerosol optical properties. This study investigates how the distribution of aerosol properties, whether columnar or vertical, affects the aerosol radiative forcing (ARF) and heating rates (HRs) across different atmospheric layers under cloud-free conditions in the shortwave region. We also assess the atmospheric parameters, namely, pressure, temperature, water vapour density, and ozone density, from in-situ measurements, reanalysis data, and a standard tropical atmosphere to understand their impact on ARF and HR estimates across seasons. Our findings show that aerosol absorption is highest during monsoon, while it is lowest in the winter. Significant atmospheric warming due to aerosols resulted from the substantial cooling at the surface. Columnar properties of aerosols measured at limited or multiple wavelengths yield similar ARF and HR estimates, provided spectral dependency is considered using the Angstrom exponent across seasons. However, the vertical profiles of aerosol extinction, together with a constant single scattering albedo (SSA) along the atmospheric column versus an actual SSA profile, led to notable differences in ARF and HRs, specifically in pre-monsoon and monsoon periods. Free tropospheric aerosol absorption is underestimated when using columnar properties compared to vertical distribution, while boundary layer absorption is overestimated (> 10 Wm<sup>-2</sup>). The heterogeneity in aerosol types across atmospheric layers significantly influenced aerosol absorption, highlighting the importance of accurate vertical distribution information. HR profiles obtained with vertical distribution reflect the structure of aerosol extinction, whereas those estimated with columnar properties result in smoother profiles that fail to capture altitude gradients. Aerosol-induced HRs are higher within the boundary layer and free troposphere in the monsoon season for all scenarios of defined aerosol properties. These findings underscore the need for actual vertical profile measurements of aerosol properties to quantify aerosol radiation interaction.</p></div>\",\"PeriodicalId\":16935,\"journal\":{\"name\":\"Journal of Quantitative Spectroscopy & Radiative Transfer\",\"volume\":\"329 \",\"pages\":\"Article 109179\"},\"PeriodicalIF\":2.3000,\"publicationDate\":\"2024-09-09\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.sciencedirect.com/science/article/pii/S0022407324002863/pdfft?md5=a72790ae85bf0f67eb1137d0ce525196&pid=1-s2.0-S0022407324002863-main.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Quantitative Spectroscopy & Radiative Transfer\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0022407324002863\",\"RegionNum\":3,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"OPTICS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Quantitative Spectroscopy & Radiative Transfer","FirstCategoryId":"101","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0022407324002863","RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"OPTICS","Score":null,"Total":0}
Influence of columnar versus vertical distribution of aerosol properties on the modulation of shortwave radiative effects
Quantifying the interaction of atmospheric aerosols with incoming solar radiation remains a challenge owing to the limitations associated with measuring aerosol optical properties. This study investigates how the distribution of aerosol properties, whether columnar or vertical, affects the aerosol radiative forcing (ARF) and heating rates (HRs) across different atmospheric layers under cloud-free conditions in the shortwave region. We also assess the atmospheric parameters, namely, pressure, temperature, water vapour density, and ozone density, from in-situ measurements, reanalysis data, and a standard tropical atmosphere to understand their impact on ARF and HR estimates across seasons. Our findings show that aerosol absorption is highest during monsoon, while it is lowest in the winter. Significant atmospheric warming due to aerosols resulted from the substantial cooling at the surface. Columnar properties of aerosols measured at limited or multiple wavelengths yield similar ARF and HR estimates, provided spectral dependency is considered using the Angstrom exponent across seasons. However, the vertical profiles of aerosol extinction, together with a constant single scattering albedo (SSA) along the atmospheric column versus an actual SSA profile, led to notable differences in ARF and HRs, specifically in pre-monsoon and monsoon periods. Free tropospheric aerosol absorption is underestimated when using columnar properties compared to vertical distribution, while boundary layer absorption is overestimated (> 10 Wm-2). The heterogeneity in aerosol types across atmospheric layers significantly influenced aerosol absorption, highlighting the importance of accurate vertical distribution information. HR profiles obtained with vertical distribution reflect the structure of aerosol extinction, whereas those estimated with columnar properties result in smoother profiles that fail to capture altitude gradients. Aerosol-induced HRs are higher within the boundary layer and free troposphere in the monsoon season for all scenarios of defined aerosol properties. These findings underscore the need for actual vertical profile measurements of aerosol properties to quantify aerosol radiation interaction.
期刊介绍:
Papers with the following subject areas are suitable for publication in the Journal of Quantitative Spectroscopy and Radiative Transfer:
- Theoretical and experimental aspects of the spectra of atoms, molecules, ions, and plasmas.
- Spectral lineshape studies including models and computational algorithms.
- Atmospheric spectroscopy.
- Theoretical and experimental aspects of light scattering.
- Application of light scattering in particle characterization and remote sensing.
- Application of light scattering in biological sciences and medicine.
- Radiative transfer in absorbing, emitting, and scattering media.
- Radiative transfer in stochastic media.