气溶胶特性的柱状分布与垂直分布对短波辐射效应调制的影响

IF 2.3 3区 物理与天体物理 Q2 OPTICS Journal of Quantitative Spectroscopy & Radiative Transfer Pub Date : 2024-09-09 DOI:10.1016/j.jqsrt.2024.109179
V.N. Santhosh , B.L. Madhavan , M. Venkat Ratnam , Dinesh N. Naik
{"title":"气溶胶特性的柱状分布与垂直分布对短波辐射效应调制的影响","authors":"V.N. Santhosh ,&nbsp;B.L. Madhavan ,&nbsp;M. Venkat Ratnam ,&nbsp;Dinesh N. Naik","doi":"10.1016/j.jqsrt.2024.109179","DOIUrl":null,"url":null,"abstract":"<div><p>Quantifying the interaction of atmospheric aerosols with incoming solar radiation remains a challenge owing to the limitations associated with measuring aerosol optical properties. This study investigates how the distribution of aerosol properties, whether columnar or vertical, affects the aerosol radiative forcing (ARF) and heating rates (HRs) across different atmospheric layers under cloud-free conditions in the shortwave region. We also assess the atmospheric parameters, namely, pressure, temperature, water vapour density, and ozone density, from in-situ measurements, reanalysis data, and a standard tropical atmosphere to understand their impact on ARF and HR estimates across seasons. Our findings show that aerosol absorption is highest during monsoon, while it is lowest in the winter. Significant atmospheric warming due to aerosols resulted from the substantial cooling at the surface. Columnar properties of aerosols measured at limited or multiple wavelengths yield similar ARF and HR estimates, provided spectral dependency is considered using the Angstrom exponent across seasons. However, the vertical profiles of aerosol extinction, together with a constant single scattering albedo (SSA) along the atmospheric column versus an actual SSA profile, led to notable differences in ARF and HRs, specifically in pre-monsoon and monsoon periods. Free tropospheric aerosol absorption is underestimated when using columnar properties compared to vertical distribution, while boundary layer absorption is overestimated (&gt; 10 Wm<sup>-2</sup>). The heterogeneity in aerosol types across atmospheric layers significantly influenced aerosol absorption, highlighting the importance of accurate vertical distribution information. HR profiles obtained with vertical distribution reflect the structure of aerosol extinction, whereas those estimated with columnar properties result in smoother profiles that fail to capture altitude gradients. Aerosol-induced HRs are higher within the boundary layer and free troposphere in the monsoon season for all scenarios of defined aerosol properties. These findings underscore the need for actual vertical profile measurements of aerosol properties to quantify aerosol radiation interaction.</p></div>","PeriodicalId":16935,"journal":{"name":"Journal of Quantitative Spectroscopy & Radiative Transfer","volume":"329 ","pages":"Article 109179"},"PeriodicalIF":2.3000,"publicationDate":"2024-09-09","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.sciencedirect.com/science/article/pii/S0022407324002863/pdfft?md5=a72790ae85bf0f67eb1137d0ce525196&pid=1-s2.0-S0022407324002863-main.pdf","citationCount":"0","resultStr":"{\"title\":\"Influence of columnar versus vertical distribution of aerosol properties on the modulation of shortwave radiative effects\",\"authors\":\"V.N. Santhosh ,&nbsp;B.L. Madhavan ,&nbsp;M. Venkat Ratnam ,&nbsp;Dinesh N. Naik\",\"doi\":\"10.1016/j.jqsrt.2024.109179\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><p>Quantifying the interaction of atmospheric aerosols with incoming solar radiation remains a challenge owing to the limitations associated with measuring aerosol optical properties. This study investigates how the distribution of aerosol properties, whether columnar or vertical, affects the aerosol radiative forcing (ARF) and heating rates (HRs) across different atmospheric layers under cloud-free conditions in the shortwave region. We also assess the atmospheric parameters, namely, pressure, temperature, water vapour density, and ozone density, from in-situ measurements, reanalysis data, and a standard tropical atmosphere to understand their impact on ARF and HR estimates across seasons. Our findings show that aerosol absorption is highest during monsoon, while it is lowest in the winter. Significant atmospheric warming due to aerosols resulted from the substantial cooling at the surface. Columnar properties of aerosols measured at limited or multiple wavelengths yield similar ARF and HR estimates, provided spectral dependency is considered using the Angstrom exponent across seasons. However, the vertical profiles of aerosol extinction, together with a constant single scattering albedo (SSA) along the atmospheric column versus an actual SSA profile, led to notable differences in ARF and HRs, specifically in pre-monsoon and monsoon periods. Free tropospheric aerosol absorption is underestimated when using columnar properties compared to vertical distribution, while boundary layer absorption is overestimated (&gt; 10 Wm<sup>-2</sup>). The heterogeneity in aerosol types across atmospheric layers significantly influenced aerosol absorption, highlighting the importance of accurate vertical distribution information. HR profiles obtained with vertical distribution reflect the structure of aerosol extinction, whereas those estimated with columnar properties result in smoother profiles that fail to capture altitude gradients. Aerosol-induced HRs are higher within the boundary layer and free troposphere in the monsoon season for all scenarios of defined aerosol properties. These findings underscore the need for actual vertical profile measurements of aerosol properties to quantify aerosol radiation interaction.</p></div>\",\"PeriodicalId\":16935,\"journal\":{\"name\":\"Journal of Quantitative Spectroscopy & Radiative Transfer\",\"volume\":\"329 \",\"pages\":\"Article 109179\"},\"PeriodicalIF\":2.3000,\"publicationDate\":\"2024-09-09\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.sciencedirect.com/science/article/pii/S0022407324002863/pdfft?md5=a72790ae85bf0f67eb1137d0ce525196&pid=1-s2.0-S0022407324002863-main.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Journal of Quantitative Spectroscopy & Radiative Transfer\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S0022407324002863\",\"RegionNum\":3,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"OPTICS\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Journal of Quantitative Spectroscopy & Radiative Transfer","FirstCategoryId":"101","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S0022407324002863","RegionNum":3,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"OPTICS","Score":null,"Total":0}
引用次数: 0

摘要

由于气溶胶光学特性测量的局限性,量化大气气溶胶与入射太阳辐射的相互作用仍然是一项挑战。本研究调查了气溶胶特性的分布(无论是柱状还是垂直分布)如何影响短波区域无云条件下不同大气层的气溶胶辐射强迫(ARF)和加热率(HRs)。我们还评估了大气参数,即气压、温度、水蒸气密度和臭氧密度,这些参数来自现场测量、再分析数据和标准热带大气,以了解它们对不同季节气溶胶辐射强迫和升温速率估计值的影响。我们的研究结果表明,气溶胶吸收在季风季节最高,而在冬季最低。气溶胶导致的大气显著变暖源于地表的大幅降温。在有限波长或多个波长上测量气溶胶的柱状特性可得出相似的 ARF 和 HR 估计值,前提是在不同季节使用安氏指数考虑光谱依赖性。然而,气溶胶消光的垂直剖面,以及沿大气柱恒定的单散射反照率(SSA)与实际的 SSA 剖面,导致了 ARF 和 HR 的显著差异,特别是在季风前和季风期。与垂直分布相比,使用柱状特性时自由对流层气溶胶吸收被低估,而边界层吸收被高估(> 10 Wm-2)。各大气层气溶胶类型的异质性对气溶胶吸收有很大影响,这突出了准确的垂直分布信息的重要性。利用垂直分布获得的气溶胶消光曲线反映了气溶胶消光的结构,而利用柱状特性估算的气溶胶消光曲线则较为平滑,无法捕捉高度梯度。在季风季节,在所有确定气溶胶特性的情况下,气溶胶引起的边界层和自由对流层的 HR 都较高。这些发现突出表明,需要对气溶胶特性进行实际垂直剖面测量,以量化气溶胶辐射相互作用。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

摘要图片

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Influence of columnar versus vertical distribution of aerosol properties on the modulation of shortwave radiative effects

Quantifying the interaction of atmospheric aerosols with incoming solar radiation remains a challenge owing to the limitations associated with measuring aerosol optical properties. This study investigates how the distribution of aerosol properties, whether columnar or vertical, affects the aerosol radiative forcing (ARF) and heating rates (HRs) across different atmospheric layers under cloud-free conditions in the shortwave region. We also assess the atmospheric parameters, namely, pressure, temperature, water vapour density, and ozone density, from in-situ measurements, reanalysis data, and a standard tropical atmosphere to understand their impact on ARF and HR estimates across seasons. Our findings show that aerosol absorption is highest during monsoon, while it is lowest in the winter. Significant atmospheric warming due to aerosols resulted from the substantial cooling at the surface. Columnar properties of aerosols measured at limited or multiple wavelengths yield similar ARF and HR estimates, provided spectral dependency is considered using the Angstrom exponent across seasons. However, the vertical profiles of aerosol extinction, together with a constant single scattering albedo (SSA) along the atmospheric column versus an actual SSA profile, led to notable differences in ARF and HRs, specifically in pre-monsoon and monsoon periods. Free tropospheric aerosol absorption is underestimated when using columnar properties compared to vertical distribution, while boundary layer absorption is overestimated (> 10 Wm-2). The heterogeneity in aerosol types across atmospheric layers significantly influenced aerosol absorption, highlighting the importance of accurate vertical distribution information. HR profiles obtained with vertical distribution reflect the structure of aerosol extinction, whereas those estimated with columnar properties result in smoother profiles that fail to capture altitude gradients. Aerosol-induced HRs are higher within the boundary layer and free troposphere in the monsoon season for all scenarios of defined aerosol properties. These findings underscore the need for actual vertical profile measurements of aerosol properties to quantify aerosol radiation interaction.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
CiteScore
5.30
自引率
21.70%
发文量
273
审稿时长
58 days
期刊介绍: Papers with the following subject areas are suitable for publication in the Journal of Quantitative Spectroscopy and Radiative Transfer: - Theoretical and experimental aspects of the spectra of atoms, molecules, ions, and plasmas. - Spectral lineshape studies including models and computational algorithms. - Atmospheric spectroscopy. - Theoretical and experimental aspects of light scattering. - Application of light scattering in particle characterization and remote sensing. - Application of light scattering in biological sciences and medicine. - Radiative transfer in absorbing, emitting, and scattering media. - Radiative transfer in stochastic media.
期刊最新文献
On radial quadrature method applied to spherical wave expansion of Gaussian beams Optical properties of semi-transparent sensor covers determined from their spectral intensity distribution function Editorial Board Improved line list of methane in the 900–1050 cm-1 region Computational toolbox for scattering of focused light from flattened or elongated particles using spheroidal wavefunctions
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1