不同气象条件下前体减排对京津冀地区夏季臭氧和 PM2.5 的控制效果

IF 6.5 2区 地球科学 Q1 METEOROLOGY & ATMOSPHERIC SCIENCES Advances in Atmospheric Sciences Pub Date : 2024-09-05 DOI:10.1007/s00376-024-4071-4
Jing Qian, Hong Liao
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引用次数: 0

摘要

我们利用观测到的空气污染物浓度、重新分析的气象参数以及戈达德地球观测系统化学传输模型的结果,研究了最大日 8 小时平均臭氧(MDA8 O3)、PM2.5(直径为 2.5微米或以下)、PM2.5组分与2米温度(T2)或相对湿度(RH)之间的关系,以及在不同夏季温度和湿度条件下,前体物减排对京津冀(BTH)臭氧和PM2.5控制的效果。观测(模拟)的 MDA8 O3 和 PM2.5 浓度均随着 T2 的升高而增加,线性趋势分别为 4.8 (3.2) ppb °C-1 和 1.9 (1.5) µg m-3 °C-1 。模型结果表明,前体排放减少带来的 MDA8 O3 下降对 T2 比对相对湿度更敏感。在较高的 T2 条件下减少较大比例的挥发性有机化合物(VOC)排放对控制 BTH 的夏季 O3 更为有效。对于控制布宜诺斯艾利斯夏季的 PM2.5,减少氮氧化物和小比例的挥发性有机化合物是最佳措施。减少前体排放物对 PM2.5 的降低幅度对相对湿度比对 T2 更敏感,高相对湿度时效率最高。这项研究的结果有助于制定有效的政策,解决北京地区的臭氧和 PM2.5 污染问题。
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Effectiveness of Precursor Emission Reductions for the Control of Summertime Ozone and PM2.5 in the Beijing–Tianjin–Hebei Region under Different Meteorological Conditions

We used observed concentrations of air pollutants, reanalyzed meteorological parameters, and results from the Goddard Earth Observing System Chemical Transport Model to examine the relationships between concentrations of maximum daily 8-h average ozone (MDA8 O3), PM2.5 (particulate matter with diameter of 2.5 µm or less), and PM2.5 components and 2-m temperature (T2) or relative humidity (RH), as well as the effectiveness of precursor emission reductions on the control of O3 and PM2.5 in Beijing–Tianjin–Hebei (BTH) under different summertime temperature and humidity conditions. Both observed (simulated) MDA8 O3 and PM2.5 concentrations increased as T2 went up, with linear trends of 4.8 (3.2) ppb °C−1 and 1.9 (1.5) µg m−3 °C−1, respectively. Model results showed that the decreases in MDA8 O3 from precursor emission reductions were more sensitive to T2 than to RH. Reducing a larger proportion of volatile organic compound (VOC) emissions at higher T2 was more effective for the control of summertime O3 in BTH. For the control of summertime PM2.5 in BTH, reducing nitrogen oxides (NOx) combined with a small proportion of VOCs was the best measure. The magnitude of reduction in PM2.5 from reducing precursor emissions was more sensitive to RH than to T2, with the best efficiency at high RH. Results from this study are helpful for formulating effective policies to tackle O3 and PM2.5 pollution in BTH.

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来源期刊
Advances in Atmospheric Sciences
Advances in Atmospheric Sciences 地学-气象与大气科学
CiteScore
9.30
自引率
5.20%
发文量
154
审稿时长
6 months
期刊介绍: Advances in Atmospheric Sciences, launched in 1984, aims to rapidly publish original scientific papers on the dynamics, physics and chemistry of the atmosphere and ocean. It covers the latest achievements and developments in the atmospheric sciences, including marine meteorology and meteorology-associated geophysics, as well as the theoretical and practical aspects of these disciplines. Papers on weather systems, numerical weather prediction, climate dynamics and variability, satellite meteorology, remote sensing, air chemistry and the boundary layer, clouds and weather modification, can be found in the journal. Papers describing the application of new mathematics or new instruments are also collected here.
期刊最新文献
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