{"title":"不同气象条件下前体减排对京津冀地区夏季臭氧和 PM2.5 的控制效果","authors":"Jing Qian, Hong Liao","doi":"10.1007/s00376-024-4071-4","DOIUrl":null,"url":null,"abstract":"<p>We used observed concentrations of air pollutants, reanalyzed meteorological parameters, and results from the Goddard Earth Observing System Chemical Transport Model to examine the relationships between concentrations of maximum daily 8-h average ozone (MDA8 O<sub>3</sub>), PM<sub>2.5</sub> (particulate matter with diameter of 2.5 µm or less), and PM<sub>2.5</sub> components and 2-m temperature (T2) or relative humidity (RH), as well as the effectiveness of precursor emission reductions on the control of O<sub>3</sub> and PM<sub>2.5</sub> in Beijing–Tianjin–Hebei (BTH) under different summertime temperature and humidity conditions. Both observed (simulated) MDA8 O<sub>3</sub> and PM<sub>2.5</sub> concentrations increased as T2 went up, with linear trends of 4.8 (3.2) ppb °C<sup>−1</sup> and 1.9 (1.5) µg m<sup>−3</sup> °C<sup>−1</sup>, respectively. Model results showed that the decreases in MDA8 O<sub>3</sub> from precursor emission reductions were more sensitive to T2 than to RH. Reducing a larger proportion of volatile organic compound (VOC) emissions at higher T2 was more effective for the control of summertime O<sub>3</sub> in BTH. For the control of summertime PM<sub>2.5</sub> in BTH, reducing nitrogen oxides (NO<sub><i>x</i></sub>) combined with a small proportion of VOCs was the best measure. The magnitude of reduction in PM<sub>2.5</sub> from reducing precursor emissions was more sensitive to RH than to T2, with the best efficiency at high RH. Results from this study are helpful for formulating effective policies to tackle O<sub>3</sub> and PM<sub>2.5</sub> pollution in BTH.</p>","PeriodicalId":7249,"journal":{"name":"Advances in Atmospheric Sciences","volume":null,"pages":null},"PeriodicalIF":6.5000,"publicationDate":"2024-09-05","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Effectiveness of Precursor Emission Reductions for the Control of Summertime Ozone and PM2.5 in the Beijing–Tianjin–Hebei Region under Different Meteorological Conditions\",\"authors\":\"Jing Qian, Hong Liao\",\"doi\":\"10.1007/s00376-024-4071-4\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p>We used observed concentrations of air pollutants, reanalyzed meteorological parameters, and results from the Goddard Earth Observing System Chemical Transport Model to examine the relationships between concentrations of maximum daily 8-h average ozone (MDA8 O<sub>3</sub>), PM<sub>2.5</sub> (particulate matter with diameter of 2.5 µm or less), and PM<sub>2.5</sub> components and 2-m temperature (T2) or relative humidity (RH), as well as the effectiveness of precursor emission reductions on the control of O<sub>3</sub> and PM<sub>2.5</sub> in Beijing–Tianjin–Hebei (BTH) under different summertime temperature and humidity conditions. Both observed (simulated) MDA8 O<sub>3</sub> and PM<sub>2.5</sub> concentrations increased as T2 went up, with linear trends of 4.8 (3.2) ppb °C<sup>−1</sup> and 1.9 (1.5) µg m<sup>−3</sup> °C<sup>−1</sup>, respectively. Model results showed that the decreases in MDA8 O<sub>3</sub> from precursor emission reductions were more sensitive to T2 than to RH. Reducing a larger proportion of volatile organic compound (VOC) emissions at higher T2 was more effective for the control of summertime O<sub>3</sub> in BTH. For the control of summertime PM<sub>2.5</sub> in BTH, reducing nitrogen oxides (NO<sub><i>x</i></sub>) combined with a small proportion of VOCs was the best measure. The magnitude of reduction in PM<sub>2.5</sub> from reducing precursor emissions was more sensitive to RH than to T2, with the best efficiency at high RH. Results from this study are helpful for formulating effective policies to tackle O<sub>3</sub> and PM<sub>2.5</sub> pollution in BTH.</p>\",\"PeriodicalId\":7249,\"journal\":{\"name\":\"Advances in Atmospheric Sciences\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":6.5000,\"publicationDate\":\"2024-09-05\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Advances in Atmospheric Sciences\",\"FirstCategoryId\":\"89\",\"ListUrlMain\":\"https://doi.org/10.1007/s00376-024-4071-4\",\"RegionNum\":2,\"RegionCategory\":\"地球科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"METEOROLOGY & ATMOSPHERIC SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Advances in Atmospheric Sciences","FirstCategoryId":"89","ListUrlMain":"https://doi.org/10.1007/s00376-024-4071-4","RegionNum":2,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"METEOROLOGY & ATMOSPHERIC SCIENCES","Score":null,"Total":0}
Effectiveness of Precursor Emission Reductions for the Control of Summertime Ozone and PM2.5 in the Beijing–Tianjin–Hebei Region under Different Meteorological Conditions
We used observed concentrations of air pollutants, reanalyzed meteorological parameters, and results from the Goddard Earth Observing System Chemical Transport Model to examine the relationships between concentrations of maximum daily 8-h average ozone (MDA8 O3), PM2.5 (particulate matter with diameter of 2.5 µm or less), and PM2.5 components and 2-m temperature (T2) or relative humidity (RH), as well as the effectiveness of precursor emission reductions on the control of O3 and PM2.5 in Beijing–Tianjin–Hebei (BTH) under different summertime temperature and humidity conditions. Both observed (simulated) MDA8 O3 and PM2.5 concentrations increased as T2 went up, with linear trends of 4.8 (3.2) ppb °C−1 and 1.9 (1.5) µg m−3 °C−1, respectively. Model results showed that the decreases in MDA8 O3 from precursor emission reductions were more sensitive to T2 than to RH. Reducing a larger proportion of volatile organic compound (VOC) emissions at higher T2 was more effective for the control of summertime O3 in BTH. For the control of summertime PM2.5 in BTH, reducing nitrogen oxides (NOx) combined with a small proportion of VOCs was the best measure. The magnitude of reduction in PM2.5 from reducing precursor emissions was more sensitive to RH than to T2, with the best efficiency at high RH. Results from this study are helpful for formulating effective policies to tackle O3 and PM2.5 pollution in BTH.
期刊介绍:
Advances in Atmospheric Sciences, launched in 1984, aims to rapidly publish original scientific papers on the dynamics, physics and chemistry of the atmosphere and ocean. It covers the latest achievements and developments in the atmospheric sciences, including marine meteorology and meteorology-associated geophysics, as well as the theoretical and practical aspects of these disciplines.
Papers on weather systems, numerical weather prediction, climate dynamics and variability, satellite meteorology, remote sensing, air chemistry and the boundary layer, clouds and weather modification, can be found in the journal. Papers describing the application of new mathematics or new instruments are also collected here.