拉伸 H2+ 强场电离的库仑效应

IF 2.9 2区 物理与天体物理 Q2 Physics and Astronomy Physical Review A Pub Date : 2024-09-13 DOI:10.1103/physreva.110.033106
S. Q. Shen, Z. Y. Chen, S. Wang, J. Y. Che, Y. J. Chen
{"title":"拉伸 H2+ 强场电离的库仑效应","authors":"S. Q. Shen, Z. Y. Chen, S. Wang, J. Y. Che, Y. J. Chen","doi":"10.1103/physreva.110.033106","DOIUrl":null,"url":null,"abstract":"We numerically and analytically study ionization of <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><msub><mi mathvariant=\"normal\">H</mi><mn>2</mn></msub><msup><mrow></mrow><mo>+</mo></msup></mrow></math> with large internuclear distances <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>R</mi></math> in strong elliptically polarized laser fields. Numerical simulations show that the offset angle in the photoelectron momentum distribution (PMD) is larger for cases of large <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>R</mi></math> than for cases of <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><msub><mi mathvariant=\"normal\">H</mi><mn>2</mn></msub><msup><mrow></mrow><mo>+</mo></msup></mrow></math> with small <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>R</mi></math> and model atoms with similar ionization potentials. In addition, the PMDs for cases of large <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>R</mi></math> show clear interference patterns which disappear for cases of small <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>R</mi></math>. By developing a strong-field model which includes the contributions of the first excited state and the Coulomb potential, we reproduce the phenomena for large <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>R</mi></math>. Tunneling ionization of <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><msub><mi mathvariant=\"normal\">H</mi><mn>2</mn></msub><msup><mrow></mrow><mo>+</mo></msup></mrow></math> with large <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>R</mi></math> involves a complex four-body interaction between the laser, the electron, and the two nuclei. Our model can approximate the four-body interaction as the three-body one and clearly identify the effects of charge resonance and different nuclei on tunneling ionization. Our work suggests a manner for probing complex interactions in strong-field ionization of stretched molecules with high time resolution.","PeriodicalId":20146,"journal":{"name":"Physical Review A","volume":null,"pages":null},"PeriodicalIF":2.9000,"publicationDate":"2024-09-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Coulomb effects on strong-field ionization of stretched H2+\",\"authors\":\"S. Q. Shen, Z. Y. Chen, S. Wang, J. Y. Che, Y. J. Chen\",\"doi\":\"10.1103/physreva.110.033106\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"We numerically and analytically study ionization of <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mrow><msub><mi mathvariant=\\\"normal\\\">H</mi><mn>2</mn></msub><msup><mrow></mrow><mo>+</mo></msup></mrow></math> with large internuclear distances <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi>R</mi></math> in strong elliptically polarized laser fields. Numerical simulations show that the offset angle in the photoelectron momentum distribution (PMD) is larger for cases of large <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi>R</mi></math> than for cases of <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mrow><msub><mi mathvariant=\\\"normal\\\">H</mi><mn>2</mn></msub><msup><mrow></mrow><mo>+</mo></msup></mrow></math> with small <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi>R</mi></math> and model atoms with similar ionization potentials. In addition, the PMDs for cases of large <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi>R</mi></math> show clear interference patterns which disappear for cases of small <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi>R</mi></math>. By developing a strong-field model which includes the contributions of the first excited state and the Coulomb potential, we reproduce the phenomena for large <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi>R</mi></math>. Tunneling ionization of <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mrow><msub><mi mathvariant=\\\"normal\\\">H</mi><mn>2</mn></msub><msup><mrow></mrow><mo>+</mo></msup></mrow></math> with large <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi>R</mi></math> involves a complex four-body interaction between the laser, the electron, and the two nuclei. Our model can approximate the four-body interaction as the three-body one and clearly identify the effects of charge resonance and different nuclei on tunneling ionization. Our work suggests a manner for probing complex interactions in strong-field ionization of stretched molecules with high time resolution.\",\"PeriodicalId\":20146,\"journal\":{\"name\":\"Physical Review A\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":2.9000,\"publicationDate\":\"2024-09-13\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Physical Review A\",\"FirstCategoryId\":\"101\",\"ListUrlMain\":\"https://doi.org/10.1103/physreva.110.033106\",\"RegionNum\":2,\"RegionCategory\":\"物理与天体物理\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"Physics and Astronomy\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Physical Review A","FirstCategoryId":"101","ListUrlMain":"https://doi.org/10.1103/physreva.110.033106","RegionNum":2,"RegionCategory":"物理与天体物理","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"Physics and Astronomy","Score":null,"Total":0}
引用次数: 0

摘要

我们通过数值和分析研究了核间距 R 较大的 H2+ 在强椭圆偏振激光场中的电离情况。数值模拟结果表明,与具有类似电离势的小 R H2+和模型原子相比,大 R 情况下光电子动量分布(PMD)的偏移角更大。通过建立一个包括第一激发态和库仑势贡献的强场模型,我们再现了大 R 的现象。大 R H2+ 的隧道电离涉及激光、电子和两个原子核之间复杂的四体相互作用。我们的模型可以将四体相互作用近似为三体相互作用,并清晰地识别出电荷共振和不同原子核对隧道电离的影响。我们的工作提出了一种以高时间分辨率探测拉伸分子强场电离中复杂相互作用的方法。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

摘要图片

查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Coulomb effects on strong-field ionization of stretched H2+
We numerically and analytically study ionization of H2+ with large internuclear distances R in strong elliptically polarized laser fields. Numerical simulations show that the offset angle in the photoelectron momentum distribution (PMD) is larger for cases of large R than for cases of H2+ with small R and model atoms with similar ionization potentials. In addition, the PMDs for cases of large R show clear interference patterns which disappear for cases of small R. By developing a strong-field model which includes the contributions of the first excited state and the Coulomb potential, we reproduce the phenomena for large R. Tunneling ionization of H2+ with large R involves a complex four-body interaction between the laser, the electron, and the two nuclei. Our model can approximate the four-body interaction as the three-body one and clearly identify the effects of charge resonance and different nuclei on tunneling ionization. Our work suggests a manner for probing complex interactions in strong-field ionization of stretched molecules with high time resolution.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Physical Review A
Physical Review A 物理-光学
CiteScore
5.40
自引率
24.10%
发文量
0
审稿时长
2.2 months
期刊介绍: Physical Review A (PRA) publishes important developments in the rapidly evolving areas of atomic, molecular, and optical (AMO) physics, quantum information, and related fundamental concepts. PRA covers atomic, molecular, and optical physics, foundations of quantum mechanics, and quantum information, including: -Fundamental concepts -Quantum information -Atomic and molecular structure and dynamics; high-precision measurement -Atomic and molecular collisions and interactions -Atomic and molecular processes in external fields, including interactions with strong fields and short pulses -Matter waves and collective properties of cold atoms and molecules -Quantum optics, physics of lasers, nonlinear optics, and classical optics
期刊最新文献
Relativistic and recoil corrections to vacuum polarization in muonic systems: Three-photon exchange, gauge invariance, and numerical values Combined microwave and optical spectroscopy for hyperfine structure analysis in thulium atoms Spectral evidence of vibronic Rabi oscillations in the resonance-enhanced photodissociation of MgH+ Universality and two-body losses: Lessons from the effective non-Hermitian dynamics of two particles Reliable quantum memories with unreliable components
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1