S. Q. Shen, Z. Y. Chen, S. Wang, J. Y. Che, Y. J. Chen
{"title":"拉伸 H2+ 强场电离的库仑效应","authors":"S. Q. Shen, Z. Y. Chen, S. Wang, J. Y. Che, Y. J. Chen","doi":"10.1103/physreva.110.033106","DOIUrl":null,"url":null,"abstract":"We numerically and analytically study ionization of <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><msub><mi mathvariant=\"normal\">H</mi><mn>2</mn></msub><msup><mrow></mrow><mo>+</mo></msup></mrow></math> with large internuclear distances <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>R</mi></math> in strong elliptically polarized laser fields. Numerical simulations show that the offset angle in the photoelectron momentum distribution (PMD) is larger for cases of large <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>R</mi></math> than for cases of <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><msub><mi mathvariant=\"normal\">H</mi><mn>2</mn></msub><msup><mrow></mrow><mo>+</mo></msup></mrow></math> with small <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>R</mi></math> and model atoms with similar ionization potentials. In addition, the PMDs for cases of large <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>R</mi></math> show clear interference patterns which disappear for cases of small <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>R</mi></math>. By developing a strong-field model which includes the contributions of the first excited state and the Coulomb potential, we reproduce the phenomena for large <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>R</mi></math>. Tunneling ionization of <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mrow><msub><mi mathvariant=\"normal\">H</mi><mn>2</mn></msub><msup><mrow></mrow><mo>+</mo></msup></mrow></math> with large <math xmlns=\"http://www.w3.org/1998/Math/MathML\"><mi>R</mi></math> involves a complex four-body interaction between the laser, the electron, and the two nuclei. Our model can approximate the four-body interaction as the three-body one and clearly identify the effects of charge resonance and different nuclei on tunneling ionization. Our work suggests a manner for probing complex interactions in strong-field ionization of stretched molecules with high time resolution.","PeriodicalId":20146,"journal":{"name":"Physical Review A","volume":null,"pages":null},"PeriodicalIF":2.9000,"publicationDate":"2024-09-13","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Coulomb effects on strong-field ionization of stretched H2+\",\"authors\":\"S. Q. Shen, Z. Y. Chen, S. Wang, J. Y. Che, Y. J. Chen\",\"doi\":\"10.1103/physreva.110.033106\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"We numerically and analytically study ionization of <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mrow><msub><mi mathvariant=\\\"normal\\\">H</mi><mn>2</mn></msub><msup><mrow></mrow><mo>+</mo></msup></mrow></math> with large internuclear distances <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi>R</mi></math> in strong elliptically polarized laser fields. Numerical simulations show that the offset angle in the photoelectron momentum distribution (PMD) is larger for cases of large <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi>R</mi></math> than for cases of <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mrow><msub><mi mathvariant=\\\"normal\\\">H</mi><mn>2</mn></msub><msup><mrow></mrow><mo>+</mo></msup></mrow></math> with small <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi>R</mi></math> and model atoms with similar ionization potentials. In addition, the PMDs for cases of large <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi>R</mi></math> show clear interference patterns which disappear for cases of small <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi>R</mi></math>. By developing a strong-field model which includes the contributions of the first excited state and the Coulomb potential, we reproduce the phenomena for large <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi>R</mi></math>. Tunneling ionization of <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mrow><msub><mi mathvariant=\\\"normal\\\">H</mi><mn>2</mn></msub><msup><mrow></mrow><mo>+</mo></msup></mrow></math> with large <math xmlns=\\\"http://www.w3.org/1998/Math/MathML\\\"><mi>R</mi></math> involves a complex four-body interaction between the laser, the electron, and the two nuclei. 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引用次数: 0
摘要
我们通过数值和分析研究了核间距 R 较大的 H2+ 在强椭圆偏振激光场中的电离情况。数值模拟结果表明,与具有类似电离势的小 R H2+和模型原子相比,大 R 情况下光电子动量分布(PMD)的偏移角更大。通过建立一个包括第一激发态和库仑势贡献的强场模型,我们再现了大 R 的现象。大 R H2+ 的隧道电离涉及激光、电子和两个原子核之间复杂的四体相互作用。我们的模型可以将四体相互作用近似为三体相互作用,并清晰地识别出电荷共振和不同原子核对隧道电离的影响。我们的工作提出了一种以高时间分辨率探测拉伸分子强场电离中复杂相互作用的方法。
Coulomb effects on strong-field ionization of stretched H2+
We numerically and analytically study ionization of with large internuclear distances in strong elliptically polarized laser fields. Numerical simulations show that the offset angle in the photoelectron momentum distribution (PMD) is larger for cases of large than for cases of with small and model atoms with similar ionization potentials. In addition, the PMDs for cases of large show clear interference patterns which disappear for cases of small . By developing a strong-field model which includes the contributions of the first excited state and the Coulomb potential, we reproduce the phenomena for large . Tunneling ionization of with large involves a complex four-body interaction between the laser, the electron, and the two nuclei. Our model can approximate the four-body interaction as the three-body one and clearly identify the effects of charge resonance and different nuclei on tunneling ionization. Our work suggests a manner for probing complex interactions in strong-field ionization of stretched molecules with high time resolution.
期刊介绍:
Physical Review A (PRA) publishes important developments in the rapidly evolving areas of atomic, molecular, and optical (AMO) physics, quantum information, and related fundamental concepts.
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-Quantum optics, physics of lasers, nonlinear optics, and classical optics