勒克瑙城市大气中排灯节烟花造成的空气悬浮颗粒悬浮时间分析

IF 2.9 4区 环境科学与生态学 Q3 ENVIRONMENTAL SCIENCES Air Quality Atmosphere and Health Pub Date : 2024-08-17 DOI:10.1007/s11869-024-01629-9
SS Kalikinkar Mahanta, Hari Om Prasad, Sreekanth Bojjagani
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引用次数: 0

摘要

该研究分析了印度勒克瑙两个不同城市景观点之间排灯节鞭炮燃烧产生的颗粒污染物的额外负荷和悬浮时间。评估了排灯节和非排灯节期间的 PM#(1、2.5 和 10)和 PSD(范围:0.2 μm 至 20 μm),以及 PM2.5 中 15 种元素和 6 种离子的化学式。在商业区,排灯节前到排灯节当天和排灯节前到排灯节后,大气中的 PM#负荷分别增加了 3 至 5 倍和 1.5 至 2 倍。而在住宅区,观察到 PM# 分别增加了 2 至 3 倍和 1 至 1.5 倍。由于当地的污染源组合不同,排灯节烟花造成的 PM# 悬浮时间的变化在住宅区为 ~10 天,在商业区为 ~6 天。此外,在两个研究地点观察到的单模态和双模态 PSD 分布以及 PSD 之间的接近性显示了排灯节和非排灯节期间相对污染源的影响。在排灯节和排灯节后的 PM2.5 中发现了大量排灯节烟花的化学标记,但在排灯节前的 PM2.5 中则较少。排灯节烟花标记与 PCA 组出现之间的强相关性进一步证实了 PM# 的悬浮期,即使在排灯节后的日子里也是如此。
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Analysis for suspension time of airborne particles due to Diwali fireworks in an urban atmosphere Lucknow

The study analyzed the additional load and suspension time of particle pollutants emerging from Diwali firecracker combustion between two different urban landscape sites in Lucknow, India. PM# (1, 2.5, and 10) and PSD (range: 0.2 μm to 20 μm), and chemical speciation of 15-elements and 6-ions of PM2.5 were assessed for Diwali and non-Diwali-days. In the commercial site, pre-Diwali-days to Diwali-day and pre-Diwali-days to post-Diwali-days added an extra load of PM# in the atmosphere by 3 to 5 times and 1.5 to 2 times respectively. Whereas, in the residential site, 2 to 3 times and 1 to 1.5 times increased PM# was observed. Variations in PM# suspension time due to Diwali fireworks were found as ~10 days at residential site and ~6 days at commercial site due to dissimilarities in the local source mix. Further, unimodal and bimodal PSD distributions and nearness observed between PSDs in two of the study sites revealed the influence of relative sources during Diwali and non-Diwali-days. Chemical markers of Diwali fireworks were identified as abundant in PM2.5 during Diwali and post-Diwali-days, but less in pre-Diwali-days. A strong correlation between markers of Diwali fireworks and their occurrence with PCA groups further confirmed the suspension period of PM# even during post-Diwali-days.

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来源期刊
Air Quality Atmosphere and Health
Air Quality Atmosphere and Health ENVIRONMENTAL SCIENCES-
CiteScore
8.80
自引率
2.00%
发文量
146
审稿时长
>12 weeks
期刊介绍: Air Quality, Atmosphere, and Health is a multidisciplinary journal which, by its very name, illustrates the broad range of work it publishes and which focuses on atmospheric consequences of human activities and their implications for human and ecological health. It offers research papers, critical literature reviews and commentaries, as well as special issues devoted to topical subjects or themes. International in scope, the journal presents papers that inform and stimulate a global readership, as the topic addressed are global in their import. Consequently, we do not encourage submission of papers involving local data that relate to local problems. Unless they demonstrate wide applicability, these are better submitted to national or regional journals. Air Quality, Atmosphere & Health addresses such topics as acid precipitation; airborne particulate matter; air quality monitoring and management; exposure assessment; risk assessment; indoor air quality; atmospheric chemistry; atmospheric modeling and prediction; air pollution climatology; climate change and air quality; air pollution measurement; atmospheric impact assessment; forest-fire emissions; atmospheric science; greenhouse gases; health and ecological effects; clean air technology; regional and global change and satellite measurements. This journal benefits a diverse audience of researchers, public health officials and policy makers addressing problems that call for solutions based in evidence from atmospheric and exposure assessment scientists, epidemiologists, and risk assessors. Publication in the journal affords the opportunity to reach beyond defined disciplinary niches to this broader readership.
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