{"title":"全纤维素胶体粘合剂","authors":"Xin Zhao, Zeyu Zhang, Tian Ju, Yuyan Jiang, Ming Wei, Jian Li, Yanjun Xie, Shaoliang Xiao","doi":"10.1038/s43246-024-00630-0","DOIUrl":null,"url":null,"abstract":"At present, adhesives widely used in various industries are mainly synthesized from organic chemical raw materials, and research on replacing traditional chemical raw materials with renewable biomass resources to synthesize adhesives is urgently needed. Adhesives possessing colloidal properties are highly favored due to their distinctive self-assembly capability, and robust reinforcement effects. Here, using cellulose as the sole raw material and following a simple and inexpensive strategy, we prepare a high-performance all-cellulose colloidal adhesive that is resistant to boiling water. We achieve a dry-shear strength of 1.97 MPa with this adhesive and a bonding strength of 0.81 MPa after a cycle of boiling-drying-boiling. The curing mechanism of the adhesive are verified using molecular dynamics simulations. These all-cellulose colloidal adhesives demonstrate great potential to replace traditional adhesives in the near future. Adhesives are commonly made from chemically synthesized raw materials. Here, a colloidal adhesive made entirely from cellulose shows strong mechanical properties and resistance to boiling water.","PeriodicalId":10589,"journal":{"name":"Communications Materials","volume":null,"pages":null},"PeriodicalIF":7.5000,"publicationDate":"2024-09-08","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s43246-024-00630-0.pdf","citationCount":"0","resultStr":"{\"title\":\"All-cellulose colloidal adhesive\",\"authors\":\"Xin Zhao, Zeyu Zhang, Tian Ju, Yuyan Jiang, Ming Wei, Jian Li, Yanjun Xie, Shaoliang Xiao\",\"doi\":\"10.1038/s43246-024-00630-0\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"At present, adhesives widely used in various industries are mainly synthesized from organic chemical raw materials, and research on replacing traditional chemical raw materials with renewable biomass resources to synthesize adhesives is urgently needed. Adhesives possessing colloidal properties are highly favored due to their distinctive self-assembly capability, and robust reinforcement effects. Here, using cellulose as the sole raw material and following a simple and inexpensive strategy, we prepare a high-performance all-cellulose colloidal adhesive that is resistant to boiling water. We achieve a dry-shear strength of 1.97 MPa with this adhesive and a bonding strength of 0.81 MPa after a cycle of boiling-drying-boiling. The curing mechanism of the adhesive are verified using molecular dynamics simulations. These all-cellulose colloidal adhesives demonstrate great potential to replace traditional adhesives in the near future. Adhesives are commonly made from chemically synthesized raw materials. Here, a colloidal adhesive made entirely from cellulose shows strong mechanical properties and resistance to boiling water.\",\"PeriodicalId\":10589,\"journal\":{\"name\":\"Communications Materials\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":7.5000,\"publicationDate\":\"2024-09-08\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.nature.com/articles/s43246-024-00630-0.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Communications Materials\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://www.nature.com/articles/s43246-024-00630-0\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"MATERIALS SCIENCE, MULTIDISCIPLINARY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Communications Materials","FirstCategoryId":"1085","ListUrlMain":"https://www.nature.com/articles/s43246-024-00630-0","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"MATERIALS SCIENCE, MULTIDISCIPLINARY","Score":null,"Total":0}
At present, adhesives widely used in various industries are mainly synthesized from organic chemical raw materials, and research on replacing traditional chemical raw materials with renewable biomass resources to synthesize adhesives is urgently needed. Adhesives possessing colloidal properties are highly favored due to their distinctive self-assembly capability, and robust reinforcement effects. Here, using cellulose as the sole raw material and following a simple and inexpensive strategy, we prepare a high-performance all-cellulose colloidal adhesive that is resistant to boiling water. We achieve a dry-shear strength of 1.97 MPa with this adhesive and a bonding strength of 0.81 MPa after a cycle of boiling-drying-boiling. The curing mechanism of the adhesive are verified using molecular dynamics simulations. These all-cellulose colloidal adhesives demonstrate great potential to replace traditional adhesives in the near future. Adhesives are commonly made from chemically synthesized raw materials. Here, a colloidal adhesive made entirely from cellulose shows strong mechanical properties and resistance to boiling water.
期刊介绍：
Communications Materials, a selective open access journal within Nature Portfolio, is dedicated to publishing top-tier research, reviews, and commentary across all facets of materials science. The journal showcases significant advancements in specialized research areas, encompassing both fundamental and applied studies. Serving as an open access option for materials sciences, Communications Materials applies less stringent criteria for impact and significance compared to Nature-branded journals, including Nature Communications.
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