氮化铝颗粒共沉积 Ni-W-P 涂层的耐磨性和耐腐蚀性研究

IF 2.6 4区 化学 Q3 ELECTROCHEMISTRY Journal of Solid State Electrochemistry Pub Date : 2024-09-07 DOI:10.1007/s10008-024-06056-5
Han Liu, Haoyu Wang, Zhiyuan Li, Yi He, Shijun Xu, Chenlu Lei, Quangang Chen, Qing Yuan, Yi Sun, Xiangshan Hou
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引用次数: 0

摘要

本研究通过脉冲电沉积法制备了高性能 Ni-W-P/AlN 复合涂层。随后,研究了纳米 AlN 粒子的引入对 Ni-W-P 涂层性能的影响,并进一步确定了 AlN 粒子的最佳添加量。结果表明,AlN 纳米粒子的加入可减小涂层的晶粒尺寸,并减轻 Ni-W-P 涂层中可观察到的微裂纹缺陷。值得注意的是,镀液浓度为 1.5 g/L 的 AlN 可产生具有最优异特性的涂层。由于 AlN 提高了涂层的机械性能,Ni-W-P/AlN 复合涂层的硬度从 360.6(Ni-W-P 涂层)提高到 620.7 HV,平均摩擦系数从 0.601(Ni-W-P 涂层)降低到 0.356。此外,还在溶解氧含量为 4.93 mg/L 的 3.5% NaCl 溶液中检测了涂层的耐腐蚀性,以评估其在腐蚀条件下的耐久性。值得注意的是,电荷转移电阻(Rct)出现了大幅上升,从 2256 Ω-cm2(Ni-W-P 涂层)升至 1.88 × 104 Ω-cm2,而腐蚀电流密度则出现了下降,从 24.17(Ni-W-P 涂层)降至 1.78 μA/cm2。这项研究为开发高性能防腐耐磨涂层策略提供了新的方向。
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Study of wear and corrosion resistance of co-deposited Ni-W–P coatings with AlN particles

In this study, high-performance Ni-W–P/AlN composite coatings were fabricated through pulsed electrodeposition. Subsequently, the effect of the introduction of AlN nanoparticles on the properties of Ni-W–P coatings was investigated and further determined the optimum addition of AlN particles. The results indicate that the incorporation of AlN nanoparticles reduces the coating’s grain size and mitigates microcrack defects observable in Ni-W–P coatings. Of significance, a bath concentration of 1.5 g/L AlN yields the coating with the most superior characteristics. Due to the enhancement of the mechanical properties of the coating by AlN, the hardness of the Ni-W–P/AlN composite coating is increased from 360.6 (Ni-W–P coating) to 620.7 HV, and the average coefficient of friction was decreased from 0.601 (Ni-W–P coating) to 0.356. Furthermore, the coating’s corrosion resistance was examined in a 3.5% NaCl solution, which had a 4.93 mg/L dissolved oxygen level, to assess its durability under corrosive conditions. Notably, the charge transfer resistance (Rct) sees a substantial increase, rising from 2256 Ω·cm2 (Ni-W–P coating) to 1.88 × 104 Ω·cm2, while the corrosion current density experiences a decline, dropping from 24.17 (Ni-W–P coating) to 1.78 μA/cm2. This study provides a new direction for the development of a high-performance anticorrosive and wear-resistant coating strategy.

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来源期刊
CiteScore
4.80
自引率
4.00%
发文量
227
审稿时长
4.1 months
期刊介绍: The Journal of Solid State Electrochemistry is devoted to all aspects of solid-state chemistry and solid-state physics in electrochemistry. The Journal of Solid State Electrochemistry publishes papers on all aspects of electrochemistry of solid compounds, including experimental and theoretical, basic and applied work. It equally publishes papers on the thermodynamics and kinetics of electrochemical reactions if at least one actively participating phase is solid. Also of interest are articles on the transport of ions and electrons in solids whenever these processes are relevant to electrochemical reactions and on the use of solid-state electrochemical reactions in the analysis of solids and their surfaces. The journal covers solid-state electrochemistry and focusses on the following fields: mechanisms of solid-state electrochemical reactions, semiconductor electrochemistry, electrochemical batteries, accumulators and fuel cells, electrochemical mineral leaching, galvanic metal plating, electrochemical potential memory devices, solid-state electrochemical sensors, ion and electron transport in solid materials and polymers, electrocatalysis, photoelectrochemistry, corrosion of solid materials, solid-state electroanalysis, electrochemical machining of materials, electrochromism and electrochromic devices, new electrochemical solid-state synthesis. The Journal of Solid State Electrochemistry makes the professional in research and industry aware of this swift progress and its importance for future developments and success in the above-mentioned fields.
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