用于氢气进化电催化剂的单原子支撑二维纳米材料的最新进展

IF 4.2 2区 化学 Q2 BIOCHEMISTRY & MOLECULAR BIOLOGY Molecules Pub Date : 2024-09-11 DOI:10.3390/molecules29184304
Kangkai Fu, Douke Yuan, Ting Yu, Chaojun Lei, Zhenhui Kou, Bingfeng Huang, Siliu Lyu, Feng Zhang, Tongtao Wan
{"title":"用于氢气进化电催化剂的单原子支撑二维纳米材料的最新进展","authors":"Kangkai Fu, Douke Yuan, Ting Yu, Chaojun Lei, Zhenhui Kou, Bingfeng Huang, Siliu Lyu, Feng Zhang, Tongtao Wan","doi":"10.3390/molecules29184304","DOIUrl":null,"url":null,"abstract":"Water electrolysis has been recognized as a promising technology that can convert renewable energy into hydrogen for storage and utilization. The superior activity and low cost of catalysis are key factors in promoting the industrialization of water electrolysis. Single-atom catalysts (SACs) have attracted attention due to their ultra-high atomic utilization, clear structure, and highest hydrogen evolution reaction (HER) performance. In addition, the performance and stability of single-atom (SA) substrates are crucial, and various two-dimensional (2D) nanomaterial supports have become promising foundations for SA due to their unique exposed surfaces, diverse elemental compositions, and flexible electronic structures, to drive single atoms to reach performance limits. The SA supported by 2D nanomaterials exhibits various electronic interactions and synergistic effects, all of which need to be comprehensively summarized. This article aims to organize and discuss the progress of 2D nanomaterial single-atom supports in enhancing HER, including common and widely used synthesis methods, advanced characterization techniques, different types of 2D supports, and the correlation between structural hydrogen evolution performance. Finally, the latest understanding of 2D nanomaterial supports was proposed.","PeriodicalId":19041,"journal":{"name":"Molecules","volume":null,"pages":null},"PeriodicalIF":4.2000,"publicationDate":"2024-09-11","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Recent Advances on Two-Dimensional Nanomaterials Supported Single-Atom for Hydrogen Evolution Electrocatalysts\",\"authors\":\"Kangkai Fu, Douke Yuan, Ting Yu, Chaojun Lei, Zhenhui Kou, Bingfeng Huang, Siliu Lyu, Feng Zhang, Tongtao Wan\",\"doi\":\"10.3390/molecules29184304\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Water electrolysis has been recognized as a promising technology that can convert renewable energy into hydrogen for storage and utilization. The superior activity and low cost of catalysis are key factors in promoting the industrialization of water electrolysis. Single-atom catalysts (SACs) have attracted attention due to their ultra-high atomic utilization, clear structure, and highest hydrogen evolution reaction (HER) performance. In addition, the performance and stability of single-atom (SA) substrates are crucial, and various two-dimensional (2D) nanomaterial supports have become promising foundations for SA due to their unique exposed surfaces, diverse elemental compositions, and flexible electronic structures, to drive single atoms to reach performance limits. The SA supported by 2D nanomaterials exhibits various electronic interactions and synergistic effects, all of which need to be comprehensively summarized. This article aims to organize and discuss the progress of 2D nanomaterial single-atom supports in enhancing HER, including common and widely used synthesis methods, advanced characterization techniques, different types of 2D supports, and the correlation between structural hydrogen evolution performance. Finally, the latest understanding of 2D nanomaterial supports was proposed.\",\"PeriodicalId\":19041,\"journal\":{\"name\":\"Molecules\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":4.2000,\"publicationDate\":\"2024-09-11\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Molecules\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://doi.org/10.3390/molecules29184304\",\"RegionNum\":2,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"BIOCHEMISTRY & MOLECULAR BIOLOGY\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Molecules","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.3390/molecules29184304","RegionNum":2,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"BIOCHEMISTRY & MOLECULAR BIOLOGY","Score":null,"Total":0}
引用次数: 0

摘要

水电解已被公认为是一种前景广阔的技术,它可以将可再生能源转化为氢气并加以储存和利用。催化剂的高活性和低成本是促进水电解工业化的关键因素。单原子催化剂(SAC)因其超高的原子利用率、清晰的结构和最高的氢进化反应(HER)性能而备受关注。此外,单原子(SA)基底的性能和稳定性也至关重要,而各种二维(2D)纳米材料支撑物因其独特的裸露表面、多样的元素组成和灵活的电子结构而成为单原子催化剂的良好基础,可推动单原子达到性能极限。二维纳米材料支撑的 SA 表现出各种电子相互作用和协同效应,所有这些都需要全面总结。本文旨在整理和讨论二维纳米材料单原子支撑在提高氢氧根效率方面的进展,包括常见和广泛应用的合成方法、先进的表征技术、不同类型的二维支撑以及结构氢演化性能之间的相关性。最后,提出了对二维纳米材料支撑的最新认识。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Recent Advances on Two-Dimensional Nanomaterials Supported Single-Atom for Hydrogen Evolution Electrocatalysts
Water electrolysis has been recognized as a promising technology that can convert renewable energy into hydrogen for storage and utilization. The superior activity and low cost of catalysis are key factors in promoting the industrialization of water electrolysis. Single-atom catalysts (SACs) have attracted attention due to their ultra-high atomic utilization, clear structure, and highest hydrogen evolution reaction (HER) performance. In addition, the performance and stability of single-atom (SA) substrates are crucial, and various two-dimensional (2D) nanomaterial supports have become promising foundations for SA due to their unique exposed surfaces, diverse elemental compositions, and flexible electronic structures, to drive single atoms to reach performance limits. The SA supported by 2D nanomaterials exhibits various electronic interactions and synergistic effects, all of which need to be comprehensively summarized. This article aims to organize and discuss the progress of 2D nanomaterial single-atom supports in enhancing HER, including common and widely used synthesis methods, advanced characterization techniques, different types of 2D supports, and the correlation between structural hydrogen evolution performance. Finally, the latest understanding of 2D nanomaterial supports was proposed.
求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Molecules
Molecules 化学-有机化学
CiteScore
7.40
自引率
8.70%
发文量
7524
审稿时长
1.4 months
期刊介绍: Molecules (ISSN 1420-3049, CODEN: MOLEFW) is an open access journal of synthetic organic chemistry and natural product chemistry. All articles are peer-reviewed and published continously upon acceptance. Molecules is published by MDPI, Basel, Switzerland. Our aim is to encourage chemists to publish as much as possible their experimental detail, particularly synthetic procedures and characterization information. There is no restriction on the length of the experimental section. In addition, availability of compound samples is published and considered as important information. Authors are encouraged to register or deposit their chemical samples through the non-profit international organization Molecular Diversity Preservation International (MDPI). Molecules has been launched in 1996 to preserve and exploit molecular diversity of both, chemical information and chemical substances.
期刊最新文献
A Review of Stoichiometric Nickel Sulfide-Based Catalysts for Hydrogen Evolution Reaction in Alkaline Media. A Spin-Labeled Derivative of Gossypol. Advances in Virus Detection Techniques Based on Recombinant Polymerase Amplification. Effectiveness Evaluation of Silicone Oil Emulsion In Situ Polymerization for Dehydration of Waterlogged Wooden Artifacts. Influence of Lactation Stage on Content of Neurotrophic Factors, Leptin, and Insulin in Human Milk.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1