Maximilian Paleschke, David Huber, Friederike Wührl, Cheng-Tien Chiang, Frank O. Schumann, Jürgen Henk, Wolf Widdra
{"title":"暗场紫外光发射电子显微镜中的磁二色性","authors":"Maximilian Paleschke, David Huber, Friederike Wührl, Cheng-Tien Chiang, Frank O. Schumann, Jürgen Henk, Wolf Widdra","doi":"arxiv-2409.04771","DOIUrl":null,"url":null,"abstract":"Photoemission electron microscopy (PEEM) has evolved into an indispensable\ntool for structural and magnetic characterization of surfaces at the nanometer\nscale. In strong contrast to synchrotron-radiation-based X-ray PEEM as a\nleading method for element-specific magnetic properties via magnetic circular\ndichroism (MCD), laboratory ultraviolet (UV) PEEM has seen limited application\nwith much smaller dichroism effects for in-plane magnetization. Here we\nintroduce darkfield PEEM as a novel approach to enhance MCD contrast in\nthreshold photoemission, enabling efficient MCD imaging with significantly\nenhanced contrast by an order-of-magnitude for Fe(001). This advancement paves\nthe way for MCD imaging on femtosecond timescales using modern lasers. The\nexperimental results will be quantitatively benchmarked against advanced\nrelativistic photoemission calculations.","PeriodicalId":501137,"journal":{"name":"arXiv - PHYS - Mesoscale and Nanoscale Physics","volume":null,"pages":null},"PeriodicalIF":0.0000,"publicationDate":"2024-09-07","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Magnetic dichroism in darkfield UV photoemission electron microscopy\",\"authors\":\"Maximilian Paleschke, David Huber, Friederike Wührl, Cheng-Tien Chiang, Frank O. Schumann, Jürgen Henk, Wolf Widdra\",\"doi\":\"arxiv-2409.04771\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Photoemission electron microscopy (PEEM) has evolved into an indispensable\\ntool for structural and magnetic characterization of surfaces at the nanometer\\nscale. In strong contrast to synchrotron-radiation-based X-ray PEEM as a\\nleading method for element-specific magnetic properties via magnetic circular\\ndichroism (MCD), laboratory ultraviolet (UV) PEEM has seen limited application\\nwith much smaller dichroism effects for in-plane magnetization. Here we\\nintroduce darkfield PEEM as a novel approach to enhance MCD contrast in\\nthreshold photoemission, enabling efficient MCD imaging with significantly\\nenhanced contrast by an order-of-magnitude for Fe(001). This advancement paves\\nthe way for MCD imaging on femtosecond timescales using modern lasers. The\\nexperimental results will be quantitatively benchmarked against advanced\\nrelativistic photoemission calculations.\",\"PeriodicalId\":501137,\"journal\":{\"name\":\"arXiv - PHYS - Mesoscale and Nanoscale Physics\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":0.0000,\"publicationDate\":\"2024-09-07\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"arXiv - PHYS - Mesoscale and Nanoscale Physics\",\"FirstCategoryId\":\"1085\",\"ListUrlMain\":\"https://doi.org/arxiv-2409.04771\",\"RegionNum\":0,\"RegionCategory\":null,\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"\",\"JCRName\":\"\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"arXiv - PHYS - Mesoscale and Nanoscale Physics","FirstCategoryId":"1085","ListUrlMain":"https://doi.org/arxiv-2409.04771","RegionNum":0,"RegionCategory":null,"ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"","JCRName":"","Score":null,"Total":0}
Magnetic dichroism in darkfield UV photoemission electron microscopy
Photoemission electron microscopy (PEEM) has evolved into an indispensable
tool for structural and magnetic characterization of surfaces at the nanometer
scale. In strong contrast to synchrotron-radiation-based X-ray PEEM as a
leading method for element-specific magnetic properties via magnetic circular
dichroism (MCD), laboratory ultraviolet (UV) PEEM has seen limited application
with much smaller dichroism effects for in-plane magnetization. Here we
introduce darkfield PEEM as a novel approach to enhance MCD contrast in
threshold photoemission, enabling efficient MCD imaging with significantly
enhanced contrast by an order-of-magnitude for Fe(001). This advancement paves
the way for MCD imaging on femtosecond timescales using modern lasers. The
experimental results will be quantitatively benchmarked against advanced
relativistic photoemission calculations.