测试攻丝粒状填料中的亚当-吉布斯关系

Xinyu Ai, Houfei Yuan, Shuyang Zhang, Zhikun Zeng, Hanyu Li, Chengjie Xia, Yujie Wang
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摘要

无序颗粒填料与过冷液体有许多相似之处,特别是在狭窄的温度或填料分数范围内结构弛豫时间的快速增加。然而,颗粒材料的动力学是否与其对应的热硬球液体的动力学相一致尚不清楚,颗粒体系的特殊摩擦影响在很大程度上仍未得到探索。在此,我们利用 X 射线断层扫描技术对单分散粒状球形填料的缓慢弛豫和稳定状态进行了实验研究。我们首先量化了具有不同摩擦力的粒状球体在爱德华兹集合下的热力学参数(即有效温度和构型熵),并测量了它们在压实过程中的特征弛豫时间。然后,我们展示了颗粒系统松弛过程的统一图景,其中一般遵循亚当-吉布斯(AG)关系。这些结果阐明了颗粒材料与理想无摩擦硬球模型之间的密切关系。
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Testing Adam-Gibbs relationship in tapped Granular Packings
Disordered granular packings share many similarities with supercooled liquids, particu-larly in the rapid increase of structural relaxation time within a narrow range of temperature or packing fraction. However, it is unclear whether the dynamics of granular materials align with those of their corresponding thermal hard sphere liquids, and the particular influence of friction of a granular system remains largely unexplored. Here, we experimentally study the slow relaxation and the steady state of monodisperse granular sphere packings with X-ray tomography. We first quantify the thermodynamic parameters under the Edwards' ensemble, (i.e., effective temperature and configurational entropy), of granular spheres with varying friction, and measure their characteristic relaxation time during compaction processes. We then demonstrate a unified picture of the relaxation process in granular systems in which the Adam-Gibbs (AG) relationship is generally followed. These results clarify the close relation-ship between granular materials and the ideal frictionless hard sphere model.
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