强场电离非相对论强度下的相对论动力学和自旋轨道动力学

IF 2.9 2区 物理与天体物理 Q2 Physics and Astronomy Physical Review A Pub Date : 2024-09-13 DOI:10.1103/physreva.110.033108
Andrew S. Maxwell, Lars Bojer Madsen
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引用次数: 0

摘要

对于强度为 1013-1014W/cm2 的近红外和中红外场,强场动力学中的自旋轨道动力学和相对论动能修正长期以来一直被忽视,因为最终光电子能量太低,这些效应无法发挥作用。然而,利用精确灵活的路径积分形式主义,我们将精细结构布赖特-保利哈密顿的所有修正项都包括在内。这使得我们能够通过相干自旋态来处理自旋,这也是强场物理学中第一个使用这种方法的模型。我们能够证明,能量最强的重散射波包在重散射过程中受到相对论动能修正的影响。我们对这些影响进行了探究,结果表明,在波长为 1600nm 的激光场中,它们对动力学和光电子能谱产生了显著的影响。此外,我们还发现,如果不考虑相对论对动能的修正,动力学自旋轨道耦合会被严重高估。最后,我们推导出一个新的条件,证明相对论效应开始发挥作用的强度要比解散散射情况下的预期强度低许多数量级。我们的发现可能会对激光诱导电子衍射等成像过程产生重要影响,其中包括高能光电子再碰撞。
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Relativistic and spin-orbit dynamics at nonrelativistic intensities in strong-field ionization
Spin-orbit dynamics and relativistic corrections to the kinetic energy in strong-field dynamics have long been ignored for near- and mid-infrared fields with intensities 10131014W/cm2, as the final photoelectron energies are considered too low for these effects to play a role. However, using a precise and flexible path-integral formalism, we include all correction terms from the fine-structure, Breit-Pauli Hamiltonian. This enables a treatment of spin, through coherent spin states, which is the first model to use this approach in strong-field physics. We are able to show that the most energetically rescattered wave packets are effected by relativistic kinetic energy corrections during rescattering. We probe these effects and show that they yield notable differences for a 1600-nm wavelength laser field on the dynamics and the photoelectron spectra. Furthermore, we find that the dynamical spin-orbit coupling is strongly overestimated if relativistic corrections to kinetic energy are not considered. Finally, we derive a new condition that demonstrates that relativistic effects begin to play a role at intensities many orders of magnitude lower than expected for the case of rescatterering. Our findings may have important implications for imaging processes such as laser-induced electron diffraction, which includes high-energy photoelectron recollisions.
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来源期刊
Physical Review A
Physical Review A 物理-光学
CiteScore
5.40
自引率
24.10%
发文量
0
审稿时长
2.2 months
期刊介绍: Physical Review A (PRA) publishes important developments in the rapidly evolving areas of atomic, molecular, and optical (AMO) physics, quantum information, and related fundamental concepts. PRA covers atomic, molecular, and optical physics, foundations of quantum mechanics, and quantum information, including: -Fundamental concepts -Quantum information -Atomic and molecular structure and dynamics; high-precision measurement -Atomic and molecular collisions and interactions -Atomic and molecular processes in external fields, including interactions with strong fields and short pulses -Matter waves and collective properties of cold atoms and molecules -Quantum optics, physics of lasers, nonlinear optics, and classical optics
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