首尔(韩国)道路尘埃污染物、轮胎磨损颗粒、空气质量和交通状况的相关性研究

IF 3.9 3区 环境科学与生态学 Q2 ENVIRONMENTAL SCIENCES Atmospheric Pollution Research Pub Date : 2024-09-13 DOI:10.1016/j.apr.2024.102309
Hyeokjin Shin , Minseung Hyun , Sohee Jeong , Hyeonjung Ryu , Min Gyu Lee , Woosuk Chung , Jaehwan Hong , Jung-Taek Kwon , Jaewoong Lee , Younghun Kim
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摘要

本研究评估了交通动态和空气质量对韩国首尔 15 个地点收集的道路尘埃中轮胎磨损颗粒(TWP)、重金属和炭黑(CB)浓度的相互依存关系。采用了皮尔逊相关分析、主成分分析和网络分析来评估交通量、车速、空气质量参数(PM10、PM2.5、氮氧化物和一氧化碳)与道路尘埃中轮胎磨损颗粒(5934-16253 毫克/千克,平均 9581 ± 4086 毫克/千克)、炭黑(371-22287 毫克/千克,平均 4291 ± 6096 毫克/千克)和重金属(铬、锰、铁、镍、铜、锌、砷、镉和铅)浓度之间的相关性。此外,还计算了重金属富集因子以及 TWP 和 CB 的污染指数,以评估车辆产生的颗粒物质对道路扬尘污染的贡献。研究发现,以交通量、车速和重金属(锌、镉和铅)等交通相关变量为特征的群组 B 与这些污染物显著相关,相关系数高达 0.933。在与交通活动相关的锌、铅和镉浓度增加过程中,三氟化硫被认为是一个重要的中介因素,导致污染水平比地球化学背景高出 2-16 倍。道路尘埃中 TWP 和 CB 的存在被确定为交通相关活动造成污染的指标,突出了锌、铅和镉作为新出现的污染物的重要性,需要有针对性的管理策略。
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A correlation study of road dust pollutants, tire wear particles, air quality, and traffic conditions in the Seoul (South Korea)
The interdependence of traffic dynamics and air quality on the concentrations of tire wear particles (TWP), heavy metals, and carbon black (CB) in road dust collected from 15 locations in Seoul, South Korea, was assessed. Pearson correlation, principal component analysis, and network analysis were employed to evaluate the correlations among traffic volume, vehicle speed, air quality parameters (PM10, PM2.5, NOx, and CO), and the concentrations of TWP (5934 to 16,253 mg/kg, average 9581 ± 4086 mg/kg), CB (371–22,287 mg/kg, average 4291 ± 6096 mg/kg), and heavy metals (Cr, Mn, Fe, Ni, Cu, Zn, As, Cd, and Pb) in road dust. The enrichment factors for heavy metals and the pollution index of TWP and CB were also calculated to evaluate the contribution of vehicle-derived particulate substances to road dust contamination. It was found that Cluster B, characterized by traffic-related variables such as traffic volume, vehicle speed, and heavy metals (Zn, Cd, and Pb), was significantly correlated with these pollutants, with correlation coefficients reaching up to 0.933. TWP was identified as a significant mediator in the increase of Zn, Pb, and Cd concentrations linked to traffic activities, contributing to pollution levels that were 2–16 times higher than the geochemical background. The presence of TWP and CB in road dust was identified as an indicator of contamination from traffic-related activities, highlighting the importance of Zn, Pb, and Cd as emerging pollutants that require targeted management strategies.
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来源期刊
Atmospheric Pollution Research
Atmospheric Pollution Research ENVIRONMENTAL SCIENCES-
CiteScore
8.30
自引率
6.70%
发文量
256
审稿时长
36 days
期刊介绍: Atmospheric Pollution Research (APR) is an international journal designed for the publication of articles on air pollution. Papers should present novel experimental results, theory and modeling of air pollution on local, regional, or global scales. Areas covered are research on inorganic, organic, and persistent organic air pollutants, air quality monitoring, air quality management, atmospheric dispersion and transport, air-surface (soil, water, and vegetation) exchange of pollutants, dry and wet deposition, indoor air quality, exposure assessment, health effects, satellite measurements, natural emissions, atmospheric chemistry, greenhouse gases, and effects on climate change.
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