用于铀污染水处理和环境修复的纳米级零价铁复合材料:综述

IF 5.8 2区 环境科学与生态学 Q1 CHEMISTRY, MULTIDISCIPLINARY Environmental Science: Nano Pub Date : 2024-09-24 DOI:10.1039/d4en00613e
Yinshan Zhu, Shusen Chen, Ziming Li, Hao Li, Muhammad Shaban, Changlun Chen
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引用次数: 0

摘要

随着核电和核工业的发展,一些含铀废水不可避免地会排放到环境中,对人类健康和环境造成威胁。纳米级零价铁(nZVI)及其复合材料具有比表面积大、活性中心多、吸附能力强等特点,可用于处理铀污染水。本综述提出了负载零价铁的基质,包括双金属、无机材料、碳材料以及有机和多孔框架材料。综述了各种基于 nZVI 的复合材料从水溶液中去除铀的最新研究进展。详细介绍了 nZVI 及其复合材料的制备方法、去除机理以及影响去除性能的环境因素。分析了 nZVI 及其复合材料在脱铀方面的优缺点,强调了有利于解决 nZVI 分散和团聚问题的负载方法。最后,简要提出了 nZVI 及其复合材料在铀污染水体修复中的应用前景,并讨论了其在环境修复中的应用前景。
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Nanoscale zero-valent iron composites for uranium-contaminated water treatment and environmental remediation: A review
With the development of nuclear power and the nuclear industry, some uranium-containing wastewater will inevitably be released into the environment, which poses a threat to human health and the environment. Nanoscale zero-valent iron (nZVI) and its composites can be used to treat uranium-contaminated water because of its large specific surface area, many active centres and high adsorption capacity. This review proposed a matrix loaded zero-valent iron, including bimetals, inorganic materials, carbon materials, and organic and porous framework materials. The latest research progress of various nZVI-based composites in removing uranium from aqueous solutions was reviewed. A detailed introduction to the preparation methods, removal mechanisms, and environmental factors affecting the removal performance of nZVI and its composite materials was provided. The advantages and disadvantages of nZVI and its composite materials for uranium removal were analyzed, and loading methods conducive to solving the dispersion and agglomeration problems of nZVI were emphasized. Finally, the application prospects of nZVI and its composites in the remediation of uranium-contaminated water were briefly proposed, and the application prospects in environmental remediation were discussed.
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来源期刊
Environmental Science: Nano
Environmental Science: Nano CHEMISTRY, MULTIDISCIPLINARY-ENVIRONMENTAL SCIENCES
CiteScore
12.20
自引率
5.50%
发文量
290
审稿时长
2.1 months
期刊介绍: Environmental Science: Nano serves as a comprehensive and high-impact peer-reviewed source of information on the design and demonstration of engineered nanomaterials for environment-based applications. It also covers the interactions between engineered, natural, and incidental nanomaterials with biological and environmental systems. This scope includes, but is not limited to, the following topic areas: Novel nanomaterial-based applications for water, air, soil, food, and energy sustainability Nanomaterial interactions with biological systems and nanotoxicology Environmental fate, reactivity, and transformations of nanoscale materials Nanoscale processes in the environment Sustainable nanotechnology including rational nanomaterial design, life cycle assessment, risk/benefit analysis
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