绘制微塑料运动图:预测颗粒尺度上非浮力微塑料迁移模式的相图

IF 10.8 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL 环境科学与技术 Pub Date : 2024-09-28 DOI:10.1021/acs.est.4c08128
Hadeel Al-Zawaidah, Merel Kooi, Ton Hoitink, Bart Vermeulen, Kryss Waldschläger
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引用次数: 0

摘要

微塑料对水生环境构成了诸多威胁,但人们对其迁移机制的了解仍然有限。从天然沉积物研究中汲取灵感,为解决这一知识空白提供了宝贵的见解。用于描述沉积物迁移的一个关键无量纲数字是迁移阶段,指的是水流剪切速度与颗粒沉降速度之间的比率。然而,由于形状和密度等物理特性的变化,现有的沉积物迁移理论是否适用于微塑料令人担忧。为了应对这一挑战,我们采用了物理建模方法,研究了湍流明渠流中 24 种不同的非浮力微塑料颗粒。利用三维颗粒跟踪技术,共记录并分析了 720 条轨迹。微塑料颗粒表现出与天然沉积物类似的迁移模式,包括滚动/滑动、盐化和悬浮。迁移阶段与这些模式以及平均前进速度和在水体中的平均位置密切相关。值得注意的是,颗粒形状是影响迁移动力学的关键因素。由于沉降速度较低,与球形颗粒相比,纤维颗粒往往更靠近水面,前进速度较低。根据实验室结果,提出了一种新的微塑料相图,类似于现有的沉积物相图。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Mapping Microplastic Movement: A Phase Diagram to Predict Nonbuoyant Microplastic Modes of Transport at the Particle Scale
Microplastics pose numerous threats to aquatic environments, yet understanding their transport mechanisms remains limited. Drawing from natural sediment research provides valuable insights to address this knowledge gap. One key dimensionless number used to describe sediment transport is the transport stage, referring to the ratio between the flow shear velocity and the particle settling velocity. However, variations in physical properties, such as shape and density, raise concerns about the applicability of existing sediment transport theories to microplastics. To address this challenge, we employed a physical modeling approach, examining 24 different nonbuoyant microplastic particles in a turbulent open channel flow. Utilizing 3D particle tracking, a total of 720 trajectories were recorded and analyzed. Microplastic particles exhibited transport modes akin to natural sediments, including rolling/sliding, saltation, and suspension. The transport stage strongly correlated with these modes, as well as with the mean forward velocity and mean position in the water column. Notably, particle shape emerged as a critical factor influencing transport dynamics. Due to their lower settling velocity, fibers tended to stay closer to the water surface with lower forward velocities compared to spheres. Based on the laboratory results, a new phase diagram for microplastics is introduced analogous to an existing diagram for sediments.
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来源期刊
环境科学与技术
环境科学与技术 环境科学-工程:环境
CiteScore
17.50
自引率
9.60%
发文量
12359
审稿时长
2.8 months
期刊介绍: Environmental Science & Technology (ES&T) is a co-sponsored academic and technical magazine by the Hubei Provincial Environmental Protection Bureau and the Hubei Provincial Academy of Environmental Sciences. Environmental Science & Technology (ES&T) holds the status of Chinese core journals, scientific papers source journals of China, Chinese Science Citation Database source journals, and Chinese Academic Journal Comprehensive Evaluation Database source journals. This publication focuses on the academic field of environmental protection, featuring articles related to environmental protection and technical advancements.
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