中国东部沿海大气中的微塑料:不同功能区反映了不同的来源和迁移情况。

IF 3.2 3区 环境科学与生态学 Q3 ENGINEERING, ENVIRONMENTAL Environmental Geochemistry and Health Pub Date : 2024-10-01 DOI:10.1007/s10653-024-02217-7
Sheng Xu, Bowen Cui, Weixin Zhang, Ruijing Liu, Hao Liu, Xiaowei Zhu, Xuqing Huang, Minyi Liu
{"title":"中国东部沿海大气中的微塑料:不同功能区反映了不同的来源和迁移情况。","authors":"Sheng Xu, Bowen Cui, Weixin Zhang, Ruijing Liu, Hao Liu, Xiaowei Zhu, Xuqing Huang, Minyi Liu","doi":"10.1007/s10653-024-02217-7","DOIUrl":null,"url":null,"abstract":"<p><p>Suspended atmospheric microplastics (SAMPs) display varying occurrence characteristics on different underlying surfaces in urban areas. This study investigated the occurrence characteristics, source apportionment, and transportation patterns of SAMPs in two typical underlying surfaces: the downtown area (Site T) and the industrial area (Site C) of a coastal city in China. In the spring of 2023, a total of 32 types comprising 1325 SAMPs were detected. The average MP abundances were found to be 3.74 ± 2.86 n/m<sup>3</sup> in Site T and 2.67 ± 1.68 n/m<sup>3</sup> in Site C. In Site T, SAMPs attributed to living source constituted 78.05%, while industry was the main source in Site C with a proportion reaching 42.89%, consistent with the functional zoning of the underlying surface. Furthermore, HYSPLIT analysis revealed that there was no significant difference between these two sites in long-distance horizontal transport affected by external airflow regardless of altitude; conversely, PCA indicated a notable correlation between vertical velocity and both abundance and species diversity. According to the hourly average wind speeds, the maximum transmission distance was computed as 350 km for updraft and the minimum transmission distances was as low as 32 m for downdraft. Subsequently, the coincidence between the source proportion of SAMPs on random day and meteorological parameters confirmed the synergistic impact on SAMPs transport influenced by functional zoning, geographic environment, and vertical velocity.</p>","PeriodicalId":11759,"journal":{"name":"Environmental Geochemistry and Health","volume":"46 11","pages":"461"},"PeriodicalIF":3.2000,"publicationDate":"2024-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Microplastics in the atmospheric of the eastern coast of China: different function areas reflecting various sources and transport.\",\"authors\":\"Sheng Xu, Bowen Cui, Weixin Zhang, Ruijing Liu, Hao Liu, Xiaowei Zhu, Xuqing Huang, Minyi Liu\",\"doi\":\"10.1007/s10653-024-02217-7\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Suspended atmospheric microplastics (SAMPs) display varying occurrence characteristics on different underlying surfaces in urban areas. This study investigated the occurrence characteristics, source apportionment, and transportation patterns of SAMPs in two typical underlying surfaces: the downtown area (Site T) and the industrial area (Site C) of a coastal city in China. In the spring of 2023, a total of 32 types comprising 1325 SAMPs were detected. The average MP abundances were found to be 3.74 ± 2.86 n/m<sup>3</sup> in Site T and 2.67 ± 1.68 n/m<sup>3</sup> in Site C. In Site T, SAMPs attributed to living source constituted 78.05%, while industry was the main source in Site C with a proportion reaching 42.89%, consistent with the functional zoning of the underlying surface. Furthermore, HYSPLIT analysis revealed that there was no significant difference between these two sites in long-distance horizontal transport affected by external airflow regardless of altitude; conversely, PCA indicated a notable correlation between vertical velocity and both abundance and species diversity. According to the hourly average wind speeds, the maximum transmission distance was computed as 350 km for updraft and the minimum transmission distances was as low as 32 m for downdraft. Subsequently, the coincidence between the source proportion of SAMPs on random day and meteorological parameters confirmed the synergistic impact on SAMPs transport influenced by functional zoning, geographic environment, and vertical velocity.</p>\",\"PeriodicalId\":11759,\"journal\":{\"name\":\"Environmental Geochemistry and Health\",\"volume\":\"46 11\",\"pages\":\"461\"},\"PeriodicalIF\":3.2000,\"publicationDate\":\"2024-10-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Environmental Geochemistry and Health\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://doi.org/10.1007/s10653-024-02217-7\",\"RegionNum\":3,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q3\",\"JCRName\":\"ENGINEERING, ENVIRONMENTAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Environmental Geochemistry and Health","FirstCategoryId":"93","ListUrlMain":"https://doi.org/10.1007/s10653-024-02217-7","RegionNum":3,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q3","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
引用次数: 0

摘要

大气中的悬浮微塑料(SAMPs)在城市地区的不同底层表面呈现出不同的出现特征。本研究调查了中国某沿海城市市中心区(T点)和工业区(C点)两个典型地表的悬浮微塑料发生特征、来源分布和迁移模式。2023 年春季,共检测到 32 种类型、1325 个 SAMP。在 T 站点,生活源 SAMP 占 78.05%,而在 C 站点,工业是主要来源,比例达到 42.89%,这与地表下的功能分区一致。此外,HYSPLIT 分析表明,在受外部气流影响的长距离水平迁移方面,这两个地点之间没有显著差异,与海拔高度无关;相反,PCA 表明垂直速度与丰度和物种多样性之间存在明显的相关性。根据每小时平均风速计算,上升气流的最大传输距离为 350 公里,而下沉气流的最小传输距离则低至 32 米。随后,随机日 SAMPs 来源比例与气象参数的吻合证实了功能分区、地理环境和垂直速度对 SAMPs 迁移的协同影响。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Microplastics in the atmospheric of the eastern coast of China: different function areas reflecting various sources and transport.

Suspended atmospheric microplastics (SAMPs) display varying occurrence characteristics on different underlying surfaces in urban areas. This study investigated the occurrence characteristics, source apportionment, and transportation patterns of SAMPs in two typical underlying surfaces: the downtown area (Site T) and the industrial area (Site C) of a coastal city in China. In the spring of 2023, a total of 32 types comprising 1325 SAMPs were detected. The average MP abundances were found to be 3.74 ± 2.86 n/m3 in Site T and 2.67 ± 1.68 n/m3 in Site C. In Site T, SAMPs attributed to living source constituted 78.05%, while industry was the main source in Site C with a proportion reaching 42.89%, consistent with the functional zoning of the underlying surface. Furthermore, HYSPLIT analysis revealed that there was no significant difference between these two sites in long-distance horizontal transport affected by external airflow regardless of altitude; conversely, PCA indicated a notable correlation between vertical velocity and both abundance and species diversity. According to the hourly average wind speeds, the maximum transmission distance was computed as 350 km for updraft and the minimum transmission distances was as low as 32 m for downdraft. Subsequently, the coincidence between the source proportion of SAMPs on random day and meteorological parameters confirmed the synergistic impact on SAMPs transport influenced by functional zoning, geographic environment, and vertical velocity.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Environmental Geochemistry and Health
Environmental Geochemistry and Health 环境科学-工程:环境
CiteScore
8.00
自引率
4.80%
发文量
279
审稿时长
4.2 months
期刊介绍: Environmental Geochemistry and Health publishes original research papers and review papers across the broad field of environmental geochemistry. Environmental geochemistry and health establishes and explains links between the natural or disturbed chemical composition of the earth’s surface and the health of plants, animals and people. Beneficial elements regulate or promote enzymatic and hormonal activity whereas other elements may be toxic. Bedrock geochemistry controls the composition of soil and hence that of water and vegetation. Environmental issues, such as pollution, arising from the extraction and use of mineral resources, are discussed. The effects of contaminants introduced into the earth’s geochemical systems are examined. Geochemical surveys of soil, water and plants show how major and trace elements are distributed geographically. Associated epidemiological studies reveal the possibility of causal links between the natural or disturbed geochemical environment and disease. Experimental research illuminates the nature or consequences of natural or disturbed geochemical processes. The journal particularly welcomes novel research linking environmental geochemistry and health issues on such topics as: heavy metals (including mercury), persistent organic pollutants (POPs), and mixed chemicals emitted through human activities, such as uncontrolled recycling of electronic-waste; waste recycling; surface-atmospheric interaction processes (natural and anthropogenic emissions, vertical transport, deposition, and physical-chemical interaction) of gases and aerosols; phytoremediation/restoration of contaminated sites; food contamination and safety; environmental effects of medicines; effects and toxicity of mixed pollutants; speciation of heavy metals/metalloids; effects of mining; disturbed geochemistry from human behavior, natural or man-made hazards; particle and nanoparticle toxicology; risk and the vulnerability of populations, etc.
期刊最新文献
Mercury in saliva, milk, and hair of nursing mothers in southeastern Iranian mothers: levels, distribution and risk assessment. Radon quantification in water and dose estimation via inhalation and ingestion across age groups in the Pattan region of North Kashmir, India. Effects of microplastics on 3,5-dichloroaniline adsorption, degradation, bioaccumulation and phytotoxicity in soil-chive systems. The impact of prenatal exposure to fine particulate matter and its components on maternal and neonatal thyroid function and birth weight: a prospective cohort study. Chemical analysis of toxic elements: total cadmium, lead, mercury, arsenic and inorganic arsenic in local and imported rice consumed in the Kingdom of Saudi Arabia.
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1