基于海水入侵和微塑料风险耦合评估模型的微塑料在入侵沿海含水层中的迁移和生态风险

IF 12.2 1区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Journal of Hazardous Materials Pub Date : 2024-10-02 DOI:10.1016/j.jhazmat.2024.135996
Guangquan Chen, Yinqiao Zou, Guiyao Xiong, Yancheng Wang, Wenqing Zhao, Xingyong Xu, Xiaobin Zhu, Jichun Wu, Fan Song, Hongjun Yu
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引用次数: 0

摘要

海水与地下水的相互作用会加剧微塑料向沿海含水层的迁移过程,从而增加相关的环境风险。本文旨在分析莱州湾海水入侵与地下水微塑料污染之间的关系,莱州湾是典型的海陆相互作用区域。结果表明,现代海水入侵是控制微塑料迁移的主要过程。研究区域内检测到的微塑料呈现出沿海水入侵方向从近岸海域向地下含水层迁移的模式。此外,微塑料还通过含水层之间的水力交换到达古盐水入侵形成的盐水中。通过比较不同微塑料参数的空间分布,我们发现近岸渔业、商业、旅游、纺织和农业活动是研究区域地下水中微塑料的主要来源。本研究采用三级分类系统,对不同的潜在影响因素赋予适当的权重,进一步优化了与西南印度洋相关的微塑料风险评估模型。结果表明,研究区域海水入侵与微塑料相关的综合生态风险适中,微塑料富集风险较高。这项研究为今后研究沿海地区海水-地下水相互作用和微塑料污染提供了科学依据。
本文章由计算机程序翻译,如有差异,请以英文原文为准。

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Migration and ecological risks of microplastics in intruded coastal aquifers based on a coupled seawater intrusion and microplastic risk assessment model
Seawater-groundwater interactions can enhance the migration process of microplastics to coastal aquifers, posing increased associated environmental risks. Here, we aim to analyze the relationship between seawater intrusion (SWI) and groundwater microplastic pollution in Laizhou Bay (LZB), which is a typical area of sea-land interactions. The results showed that modern seawater intrusion was the main process controlling the migration of microplastics. The detected microplastics in the study area showed a migration pattern from nearshore marine areas to groundwater aquifers along the SWI direction. In addition, the microplastics also reached the brine formed by palaeo-saltwater intrusion through hydraulic exchange between aquifers. By comparing the spatial distributions of different microplastic parameters, we found that nearshore fisheries, commercial, tourism, textile, and agricultural activities were the main sources of microplastics in groundwater in the study area. A risk assessment model of microplastics associated with SWI was further optimized in this study using a three-level classification system by assigning appropriate weights to different potential influencing factors. The results showed moderate comprehensive ecological risks associated with microplastics from seawater intrusion in the study area, with high microplastic enrichment risks. This study provides a scientific basis for future research on seawater-groundwater interactions and microplastic pollution in coastal regions.
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来源期刊
Journal of Hazardous Materials
Journal of Hazardous Materials 工程技术-工程:环境
CiteScore
25.40
自引率
5.90%
发文量
3059
审稿时长
58 days
期刊介绍: The Journal of Hazardous Materials serves as a global platform for promoting cutting-edge research in the field of Environmental Science and Engineering. Our publication features a wide range of articles, including full-length research papers, review articles, and perspectives, with the aim of enhancing our understanding of the dangers and risks associated with various materials concerning public health and the environment. It is important to note that the term "environmental contaminants" refers specifically to substances that pose hazardous effects through contamination, while excluding those that do not have such impacts on the environment or human health. Moreover, we emphasize the distinction between wastes and hazardous materials in order to provide further clarity on the scope of the journal. We have a keen interest in exploring specific compounds and microbial agents that have adverse effects on the environment.
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