{"title":"一种独特的喹啉基荧光探针对亚硫酸氢盐的超快检测及其在智能手机辅助食品检测和生物成像中的应用。","authors":"Xiaoyu Huang, Jiaxing Li, Yuetian Guo, Mingyu Tian, Xiaomei Yan, Lijun Tang, Keli Zhong","doi":"10.1016/j.talanta.2024.126977","DOIUrl":null,"url":null,"abstract":"<p><p>Sulfur dioxide (SO<sub>2</sub>) is one of the major pollutants in the atmosphere, which is highly susceptible to inhalation by the human body and is converted into its derivatives (HSO<sub>3</sub><sup>-</sup>/SO<sub>3</sub><sup>2-</sup>), which is hazardous to both human health and the ecological environment. Therefore the detection of SO<sub>2</sub> derivatives (HSO<sub>3</sub><sup>-</sup>/SO<sub>3</sub><sup>2-</sup>) is very important. In this work, we have prepared ID-QL, a water-soluble fluorescent probe based on the intramolecular charge transfer (ICT) mechanism, it exhibits colorimetric and fluorescent dual-channel response to HSO<sub>3</sub><sup>-</sup> with ultrafast, highly selective and sensitive detection. In particular, ID-QL can be used for quantitative detection of HSO<sub>3</sub><sup>-</sup> in real food samples. We developed a portable test strip for ID-QL and successfully combined it with smartphone to achieve convenient, low-cost and portable detection of HSO<sub>3</sub><sup>-</sup> in real samples. The probe displays good mitochondrial targeting ability and can be used for visual monitoring and imaging of sulfites in live cells and zebrafish.</p>","PeriodicalId":435,"journal":{"name":"Talanta","volume":null,"pages":null},"PeriodicalIF":5.6000,"publicationDate":"2024-10-01","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Ultrafast detection of bisulfite by a unique quinolinium-based fluorescent probe and its applications in smartphone-assisted food detection and bioimaging.\",\"authors\":\"Xiaoyu Huang, Jiaxing Li, Yuetian Guo, Mingyu Tian, Xiaomei Yan, Lijun Tang, Keli Zhong\",\"doi\":\"10.1016/j.talanta.2024.126977\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p><p>Sulfur dioxide (SO<sub>2</sub>) is one of the major pollutants in the atmosphere, which is highly susceptible to inhalation by the human body and is converted into its derivatives (HSO<sub>3</sub><sup>-</sup>/SO<sub>3</sub><sup>2-</sup>), which is hazardous to both human health and the ecological environment. Therefore the detection of SO<sub>2</sub> derivatives (HSO<sub>3</sub><sup>-</sup>/SO<sub>3</sub><sup>2-</sup>) is very important. In this work, we have prepared ID-QL, a water-soluble fluorescent probe based on the intramolecular charge transfer (ICT) mechanism, it exhibits colorimetric and fluorescent dual-channel response to HSO<sub>3</sub><sup>-</sup> with ultrafast, highly selective and sensitive detection. In particular, ID-QL can be used for quantitative detection of HSO<sub>3</sub><sup>-</sup> in real food samples. We developed a portable test strip for ID-QL and successfully combined it with smartphone to achieve convenient, low-cost and portable detection of HSO<sub>3</sub><sup>-</sup> in real samples. The probe displays good mitochondrial targeting ability and can be used for visual monitoring and imaging of sulfites in live cells and zebrafish.</p>\",\"PeriodicalId\":435,\"journal\":{\"name\":\"Talanta\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":5.6000,\"publicationDate\":\"2024-10-01\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Talanta\",\"FirstCategoryId\":\"92\",\"ListUrlMain\":\"https://doi.org/10.1016/j.talanta.2024.126977\",\"RegionNum\":1,\"RegionCategory\":\"化学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"CHEMISTRY, ANALYTICAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Talanta","FirstCategoryId":"92","ListUrlMain":"https://doi.org/10.1016/j.talanta.2024.126977","RegionNum":1,"RegionCategory":"化学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"CHEMISTRY, ANALYTICAL","Score":null,"Total":0}
Ultrafast detection of bisulfite by a unique quinolinium-based fluorescent probe and its applications in smartphone-assisted food detection and bioimaging.
Sulfur dioxide (SO2) is one of the major pollutants in the atmosphere, which is highly susceptible to inhalation by the human body and is converted into its derivatives (HSO3-/SO32-), which is hazardous to both human health and the ecological environment. Therefore the detection of SO2 derivatives (HSO3-/SO32-) is very important. In this work, we have prepared ID-QL, a water-soluble fluorescent probe based on the intramolecular charge transfer (ICT) mechanism, it exhibits colorimetric and fluorescent dual-channel response to HSO3- with ultrafast, highly selective and sensitive detection. In particular, ID-QL can be used for quantitative detection of HSO3- in real food samples. We developed a portable test strip for ID-QL and successfully combined it with smartphone to achieve convenient, low-cost and portable detection of HSO3- in real samples. The probe displays good mitochondrial targeting ability and can be used for visual monitoring and imaging of sulfites in live cells and zebrafish.
期刊介绍:
Talanta provides a forum for the publication of original research papers, short communications, and critical reviews in all branches of pure and applied analytical chemistry. Papers are evaluated based on established guidelines, including the fundamental nature of the study, scientific novelty, substantial improvement or advantage over existing technology or methods, and demonstrated analytical applicability. Original research papers on fundamental studies, and on novel sensor and instrumentation developments, are encouraged. Novel or improved applications in areas such as clinical and biological chemistry, environmental analysis, geochemistry, materials science and engineering, and analytical platforms for omics development are welcome.
Analytical performance of methods should be determined, including interference and matrix effects, and methods should be validated by comparison with a standard method, or analysis of a certified reference material. Simple spiking recoveries may not be sufficient. The developed method should especially comprise information on selectivity, sensitivity, detection limits, accuracy, and reliability. However, applying official validation or robustness studies to a routine method or technique does not necessarily constitute novelty. Proper statistical treatment of the data should be provided. Relevant literature should be cited, including related publications by the authors, and authors should discuss how their proposed methodology compares with previously reported methods.