石墨烯中流体动力电子的粘性太赫兹光电导性

IF 38.1 1区 材料科学 Q1 MATERIALS SCIENCE, MULTIDISCIPLINARY Nature nanotechnology Pub Date : 2024-10-07 DOI:10.1038/s41565-024-01795-y
M. Kravtsov, A. L. Shilov, Y. Yang, T. Pryadilin, M. A. Kashchenko, O. Popova, M. Titova, D. Voropaev, Y. Wang, K. Shein, I. Gayduchenko, G. N. Goltsman, M. Lukianov, A. Kudriashov, T. Taniguchi, K. Watanabe, D. A. Svintsov, S. Adam, K. S. Novoselov, A. Principi, D. A. Bandurin
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引用次数: 0

摘要

光线入射到材料上会导致其导电性发生变化,这种现象被称为光阻。在半导体中,光阻是负的,因为光诱导电子穿过带隙会增加参与传输的电荷载流子数量。在超导体和普通金属中,光阻为正,原因分别是超导态的破坏和动量松弛散射的增强。在这里,我们报告了掺杂金属石墨烯中与标准行为的定性偏差。我们的研究表明,暴露在连续波太赫兹(THz)辐射下的狄拉克电子可以与晶格热解耦,从而激活流体动力电子传输。在这种情况下,太赫兹驱动的相关电子超弹流会导致石墨烯收缩电阻下降。我们分析了负光阻对载流子密度和辐射功率的依赖关系,结果表明我们的超弹道装置可以作为灵敏的声子冷却波长计运行,因此原则上可以提供皮秒级的响应时间。除了基本影响之外,我们的发现还强调了电子流体力学在设计超快太赫兹传感器和电子温度计方面的实用性。
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Viscous terahertz photoconductivity of hydrodynamic electrons in graphene

Light incident upon materials can induce changes in their electrical conductivity, a phenomenon referred to as photoresistance. In semiconductors, the photoresistance is negative, as light-induced promotion of electrons across the bandgap enhances the number of charge carriers participating in transport. In superconductors and normal metals, the photoresistance is positive because of the destruction of the superconducting state and enhanced momentum-relaxing scattering, respectively. Here we report a qualitative deviation from the standard behaviour in doped metallic graphene. We show that Dirac electrons exposed to continuous-wave terahertz (THz) radiation can be thermally decoupled from the lattice, which activates hydrodynamic electron transport. In this regime, the resistance of graphene constrictions experiences a decrease caused by the THz-driven superballistic flow of correlated electrons. We analyse the dependencies of the negative photoresistance on the carrier density, and the radiation power, and show that our superballistic devices operate as sensitive phonon-cooled bolometers and can thus offer, in principle, a picosecond-scale response time. Beyond their fundamental implications, our findings underscore the practicality of electron hydrodynamics in designing ultra-fast THz sensors and electron thermometers.

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来源期刊
Nature nanotechnology
Nature nanotechnology 工程技术-材料科学:综合
CiteScore
59.70
自引率
0.80%
发文量
196
审稿时长
4-8 weeks
期刊介绍: Nature Nanotechnology is a prestigious journal that publishes high-quality papers in various areas of nanoscience and nanotechnology. The journal focuses on the design, characterization, and production of structures, devices, and systems that manipulate and control materials at atomic, molecular, and macromolecular scales. It encompasses both bottom-up and top-down approaches, as well as their combinations. Furthermore, Nature Nanotechnology fosters the exchange of ideas among researchers from diverse disciplines such as chemistry, physics, material science, biomedical research, engineering, and more. It promotes collaboration at the forefront of this multidisciplinary field. The journal covers a wide range of topics, from fundamental research in physics, chemistry, and biology, including computational work and simulations, to the development of innovative devices and technologies for various industrial sectors such as information technology, medicine, manufacturing, high-performance materials, energy, and environmental technologies. It includes coverage of organic, inorganic, and hybrid materials.
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