二维范德华磁体 CrI3 中的稳健二阶拓扑绝缘体。

IF 12.2 2区 材料科学 Q1 CHEMISTRY, MULTIDISCIPLINARY Materials Horizons Pub Date : 2024-10-08 DOI:10.1039/d4mh00620h
Xiaorong Zou, Yingxi Bai, Ying Dai, Baibiao Huang, Chengwang Niu
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引用次数: 0

摘要

CrI3 为探索二维(2D)磁体中的基础物理学和自旋电子器件的创新设计提供了一个有趣的平台,而且在拓扑物理学研究中也发挥了重要作用。然而,二维 CrI3 单层和双层长期以来一直被认为是拓扑琐碎的。在这里,我们发现了二维 CrI3 单层和双层都是二阶拓扑绝缘体(SOTIs),其第二斯蒂费尔-惠特尼数 w2 = 1 不为零,从而揭开了二维 CrI3 带拓扑的一个隐秘面。此外,浮边态和隙内角态的出现也明确证实了拓扑学上的非琐碎性。值得注意的是,与大多数已知的磁拓扑态不同,我们提出二维 CrI3 单层和双层中的 SOTIs 对磁跃迁具有高度的鲁棒性,在铁磁和反铁磁构型下都能保持不变。这些有趣的预测不仅提供了对二维 CrI3 带拓扑的全面理解,还为实现自旋电子学应用中的磁性 SOTI 提供了一个有利的平台。
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Robust second-order topological insulator in 2D van der Waals magnet CrI3.

CrI3 offers an intriguing platform for exploring fundamental physics and the innovative design of spintronics devices in two-dimensional (2D) magnets, and moreover has been instrumental in the study of topological physics. However, the 2D CrI3 monolayer and bilayers have long been thought to be topologically trivial. Here we uncover a hidden facet of the band topology of 2D CrI3 by showing that both the CrI3 monolayer and bilayers are second-order topological insulators (SOTIs) with a nonzero second Stiefel-Whitney number w2 = 1. Furthermore, the topologically nontrivial nature can be explicitly confirmed via the emergence of floating edge states and in-gap corner states. Remarkably, in contrast to most known magnetic topological states, we put forward that the SOTIs in 2D CrI3 monolayer and bilayers are highly robust against magnetic transitions, which remain intact under both ferromagnetic and antiferromagnetic configurations. These interesting predictions not only provide a comprehensive understanding of the band topology of 2D CrI3 but also offer a favorable platform to realize magnetic SOTIs for spintronics applications.

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来源期刊
Materials Horizons
Materials Horizons CHEMISTRY, MULTIDISCIPLINARY-MATERIALS SCIENCE, MULTIDISCIPLINARY
CiteScore
18.90
自引率
2.30%
发文量
306
审稿时长
1.3 months
期刊介绍: Materials Horizons is a leading journal in materials science that focuses on publishing exceptionally high-quality and innovative research. The journal prioritizes original research that introduces new concepts or ways of thinking, rather than solely reporting technological advancements. However, groundbreaking articles featuring record-breaking material performance may also be published. To be considered for publication, the work must be of significant interest to our community-spanning readership. Starting from 2021, all articles published in Materials Horizons will be indexed in MEDLINE©. The journal publishes various types of articles, including Communications, Reviews, Opinion pieces, Focus articles, and Comments. It serves as a core journal for researchers from academia, government, and industry across all areas of materials research. Materials Horizons is a Transformative Journal and compliant with Plan S. It has an impact factor of 13.3 and is indexed in MEDLINE.
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