Wenbin Weng, Minde An, Luke M. Western, Ronald G. Prinn, Jianxin Hu, Xingchen Zhao, Matthew Rigby, Yinuo Wang, Siyuan Huang, Honghui Xu, Yan Yu, Wenxue Chi and Bo Yao*,
{"title":"根据大气观测数据推算的 2017-2021 年中国三氟化氮排放量","authors":"Wenbin Weng, Minde An, Luke M. Western, Ronald G. Prinn, Jianxin Hu, Xingchen Zhao, Matthew Rigby, Yinuo Wang, Siyuan Huang, Honghui Xu, Yan Yu, Wenxue Chi and Bo Yao*, ","doi":"10.1021/acs.estlett.4c0052710.1021/acs.estlett.4c00527","DOIUrl":null,"url":null,"abstract":"<p >Rapid growth in the emissions of nitrogen trifluoride (NF<sub>3</sub>), a potent greenhouse gas, poses a threat to the environment and the climate system. This study estimated NF<sub>3</sub> emissions and their spatial distribution in China from 2017 to 2021 based on atmospheric observations from nine background stations in China, by employing a Lagrangian-dispersion-model-based Bayesian inversion technique. We found that NF<sub>3</sub> emissions in China increased from 0.95 (0.82–1.07) Gg yr<sup>–1</sup> in 2017 to 1.41 (1.28–1.55) Gg yr<sup>–1</sup> in 2021, representing a substantial growth of 48% over this period. The absolute increase in NF<sub>3</sub> emissions in China over 2017–2020, 0.65 (0.57–0.74) Gg yr<sup>–1</sup>is comparable to the increase in global emissions (0.63 (0.50–0.75) Gg yr<sup>–1</sup>) over the same period. We identified substantial NF<sub>3</sub> emissions in the Pearl and Yangtze River Delta regions and Hubei Province, where well-established semiconductor industries could have contributed to NF<sub>3</sub> emissions. Moreover, large NF<sub>3</sub> emissions were identified in northern China, including Hebei, Henan, and Shandong Provinces. If control measures are not implemented, increasing NF<sub>3</sub> emissions may delay China’s progress toward achieving its carbon neutrality target by 2060.</p>","PeriodicalId":37,"journal":{"name":"Environmental Science & Technology Letters Environ.","volume":"11 10","pages":"1096–1102 1096–1102"},"PeriodicalIF":8.9000,"publicationDate":"2024-09-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Nitrogen Trifluoride Emissions in China from 2017 to 2021 Derived from Atmospheric Observations\",\"authors\":\"Wenbin Weng, Minde An, Luke M. Western, Ronald G. Prinn, Jianxin Hu, Xingchen Zhao, Matthew Rigby, Yinuo Wang, Siyuan Huang, Honghui Xu, Yan Yu, Wenxue Chi and Bo Yao*, \",\"doi\":\"10.1021/acs.estlett.4c0052710.1021/acs.estlett.4c00527\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Rapid growth in the emissions of nitrogen trifluoride (NF<sub>3</sub>), a potent greenhouse gas, poses a threat to the environment and the climate system. This study estimated NF<sub>3</sub> emissions and their spatial distribution in China from 2017 to 2021 based on atmospheric observations from nine background stations in China, by employing a Lagrangian-dispersion-model-based Bayesian inversion technique. We found that NF<sub>3</sub> emissions in China increased from 0.95 (0.82–1.07) Gg yr<sup>–1</sup> in 2017 to 1.41 (1.28–1.55) Gg yr<sup>–1</sup> in 2021, representing a substantial growth of 48% over this period. The absolute increase in NF<sub>3</sub> emissions in China over 2017–2020, 0.65 (0.57–0.74) Gg yr<sup>–1</sup>is comparable to the increase in global emissions (0.63 (0.50–0.75) Gg yr<sup>–1</sup>) over the same period. We identified substantial NF<sub>3</sub> emissions in the Pearl and Yangtze River Delta regions and Hubei Province, where well-established semiconductor industries could have contributed to NF<sub>3</sub> emissions. Moreover, large NF<sub>3</sub> emissions were identified in northern China, including Hebei, Henan, and Shandong Provinces. If control measures are not implemented, increasing NF<sub>3</sub> emissions may delay China’s progress toward achieving its carbon neutrality target by 2060.</p>\",\"PeriodicalId\":37,\"journal\":{\"name\":\"Environmental Science & Technology Letters Environ.\",\"volume\":\"11 10\",\"pages\":\"1096–1102 1096–1102\"},\"PeriodicalIF\":8.9000,\"publicationDate\":\"2024-09-17\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Environmental Science & Technology Letters Environ.\",\"FirstCategoryId\":\"1\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acs.estlett.4c00527\",\"RegionNum\":2,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, ENVIRONMENTAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Environmental Science & Technology Letters Environ.","FirstCategoryId":"1","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.estlett.4c00527","RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
Nitrogen Trifluoride Emissions in China from 2017 to 2021 Derived from Atmospheric Observations
Rapid growth in the emissions of nitrogen trifluoride (NF3), a potent greenhouse gas, poses a threat to the environment and the climate system. This study estimated NF3 emissions and their spatial distribution in China from 2017 to 2021 based on atmospheric observations from nine background stations in China, by employing a Lagrangian-dispersion-model-based Bayesian inversion technique. We found that NF3 emissions in China increased from 0.95 (0.82–1.07) Gg yr–1 in 2017 to 1.41 (1.28–1.55) Gg yr–1 in 2021, representing a substantial growth of 48% over this period. The absolute increase in NF3 emissions in China over 2017–2020, 0.65 (0.57–0.74) Gg yr–1is comparable to the increase in global emissions (0.63 (0.50–0.75) Gg yr–1) over the same period. We identified substantial NF3 emissions in the Pearl and Yangtze River Delta regions and Hubei Province, where well-established semiconductor industries could have contributed to NF3 emissions. Moreover, large NF3 emissions were identified in northern China, including Hebei, Henan, and Shandong Provinces. If control measures are not implemented, increasing NF3 emissions may delay China’s progress toward achieving its carbon neutrality target by 2060.
期刊介绍:
Environmental Science & Technology Letters serves as an international forum for brief communications on experimental or theoretical results of exceptional timeliness in all aspects of environmental science, both pure and applied. Published as soon as accepted, these communications are summarized in monthly issues. Additionally, the journal features short reviews on emerging topics in environmental science and technology.