根据大气观测数据推算的 2017-2021 年中国三氟化氮排放量

IF 8.9 2区 环境科学与生态学 Q1 ENGINEERING, ENVIRONMENTAL Environmental Science & Technology Letters Environ. Pub Date : 2024-09-17 DOI:10.1021/acs.estlett.4c0052710.1021/acs.estlett.4c00527
Wenbin Weng, Minde An, Luke M. Western, Ronald G. Prinn, Jianxin Hu, Xingchen Zhao, Matthew Rigby, Yinuo Wang, Siyuan Huang, Honghui Xu, Yan Yu, Wenxue Chi and Bo Yao*, 
{"title":"根据大气观测数据推算的 2017-2021 年中国三氟化氮排放量","authors":"Wenbin Weng,&nbsp;Minde An,&nbsp;Luke M. Western,&nbsp;Ronald G. Prinn,&nbsp;Jianxin Hu,&nbsp;Xingchen Zhao,&nbsp;Matthew Rigby,&nbsp;Yinuo Wang,&nbsp;Siyuan Huang,&nbsp;Honghui Xu,&nbsp;Yan Yu,&nbsp;Wenxue Chi and Bo Yao*,&nbsp;","doi":"10.1021/acs.estlett.4c0052710.1021/acs.estlett.4c00527","DOIUrl":null,"url":null,"abstract":"<p >Rapid growth in the emissions of nitrogen trifluoride (NF<sub>3</sub>), a potent greenhouse gas, poses a threat to the environment and the climate system. This study estimated NF<sub>3</sub> emissions and their spatial distribution in China from 2017 to 2021 based on atmospheric observations from nine background stations in China, by employing a Lagrangian-dispersion-model-based Bayesian inversion technique. We found that NF<sub>3</sub> emissions in China increased from 0.95 (0.82–1.07) Gg yr<sup>–1</sup> in 2017 to 1.41 (1.28–1.55) Gg yr<sup>–1</sup> in 2021, representing a substantial growth of 48% over this period. The absolute increase in NF<sub>3</sub> emissions in China over 2017–2020, 0.65 (0.57–0.74) Gg yr<sup>–1</sup>is comparable to the increase in global emissions (0.63 (0.50–0.75) Gg yr<sup>–1</sup>) over the same period. We identified substantial NF<sub>3</sub> emissions in the Pearl and Yangtze River Delta regions and Hubei Province, where well-established semiconductor industries could have contributed to NF<sub>3</sub> emissions. Moreover, large NF<sub>3</sub> emissions were identified in northern China, including Hebei, Henan, and Shandong Provinces. If control measures are not implemented, increasing NF<sub>3</sub> emissions may delay China’s progress toward achieving its carbon neutrality target by 2060.</p>","PeriodicalId":37,"journal":{"name":"Environmental Science & Technology Letters Environ.","volume":null,"pages":null},"PeriodicalIF":8.9000,"publicationDate":"2024-09-17","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Nitrogen Trifluoride Emissions in China from 2017 to 2021 Derived from Atmospheric Observations\",\"authors\":\"Wenbin Weng,&nbsp;Minde An,&nbsp;Luke M. Western,&nbsp;Ronald G. Prinn,&nbsp;Jianxin Hu,&nbsp;Xingchen Zhao,&nbsp;Matthew Rigby,&nbsp;Yinuo Wang,&nbsp;Siyuan Huang,&nbsp;Honghui Xu,&nbsp;Yan Yu,&nbsp;Wenxue Chi and Bo Yao*,&nbsp;\",\"doi\":\"10.1021/acs.estlett.4c0052710.1021/acs.estlett.4c00527\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<p >Rapid growth in the emissions of nitrogen trifluoride (NF<sub>3</sub>), a potent greenhouse gas, poses a threat to the environment and the climate system. This study estimated NF<sub>3</sub> emissions and their spatial distribution in China from 2017 to 2021 based on atmospheric observations from nine background stations in China, by employing a Lagrangian-dispersion-model-based Bayesian inversion technique. We found that NF<sub>3</sub> emissions in China increased from 0.95 (0.82–1.07) Gg yr<sup>–1</sup> in 2017 to 1.41 (1.28–1.55) Gg yr<sup>–1</sup> in 2021, representing a substantial growth of 48% over this period. The absolute increase in NF<sub>3</sub> emissions in China over 2017–2020, 0.65 (0.57–0.74) Gg yr<sup>–1</sup>is comparable to the increase in global emissions (0.63 (0.50–0.75) Gg yr<sup>–1</sup>) over the same period. We identified substantial NF<sub>3</sub> emissions in the Pearl and Yangtze River Delta regions and Hubei Province, where well-established semiconductor industries could have contributed to NF<sub>3</sub> emissions. Moreover, large NF<sub>3</sub> emissions were identified in northern China, including Hebei, Henan, and Shandong Provinces. If control measures are not implemented, increasing NF<sub>3</sub> emissions may delay China’s progress toward achieving its carbon neutrality target by 2060.</p>\",\"PeriodicalId\":37,\"journal\":{\"name\":\"Environmental Science & Technology Letters Environ.\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":8.9000,\"publicationDate\":\"2024-09-17\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Environmental Science & Technology Letters Environ.\",\"FirstCategoryId\":\"1\",\"ListUrlMain\":\"https://pubs.acs.org/doi/10.1021/acs.estlett.4c00527\",\"RegionNum\":2,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENGINEERING, ENVIRONMENTAL\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Environmental Science & Technology Letters Environ.","FirstCategoryId":"1","ListUrlMain":"https://pubs.acs.org/doi/10.1021/acs.estlett.4c00527","RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENGINEERING, ENVIRONMENTAL","Score":null,"Total":0}
引用次数: 0

摘要

三氟化氮(NF3)是一种强效温室气体,其排放量的快速增长对环境和气候系统构成了威胁。本研究基于中国9个背景站的大气观测数据,采用基于拉格朗日-色散模型的贝叶斯反演技术,估算了2017年至2021年中国的三氟化氮排放量及其空间分布。我们发现,中国的 NF3 排放量从 2017 年的 0.95(0.82-1.07)Gg yr-1 增加到 2021 年的 1.41(1.28-1.55)Gg yr-1,在此期间大幅增长了 48%。2017-2020 年间,中国 NF3 排放量的绝对增幅为 0.65 (0.57-0.74) 千兆克/年-1,与同期全球排放量的增幅(0.63 (0.50-0.75) 千兆克/年-1)相当。我们在珠江三角洲和长江三角洲地区以及湖北省发现了大量的三氟化氮排放,这些地区完善的半导体工业可能是三氟化氮排放的来源。此外,在华北地区,包括河北省、河南省和山东省,也发现了大量的 NF3 排放。如果不采取控制措施,NF3排放量的增加可能会推迟中国到 2060 年实现碳中和目标的进程。
本文章由计算机程序翻译,如有差异,请以英文原文为准。
查看原文
分享 分享
微信好友 朋友圈 QQ好友 复制链接
本刊更多论文
Nitrogen Trifluoride Emissions in China from 2017 to 2021 Derived from Atmospheric Observations

Rapid growth in the emissions of nitrogen trifluoride (NF3), a potent greenhouse gas, poses a threat to the environment and the climate system. This study estimated NF3 emissions and their spatial distribution in China from 2017 to 2021 based on atmospheric observations from nine background stations in China, by employing a Lagrangian-dispersion-model-based Bayesian inversion technique. We found that NF3 emissions in China increased from 0.95 (0.82–1.07) Gg yr–1 in 2017 to 1.41 (1.28–1.55) Gg yr–1 in 2021, representing a substantial growth of 48% over this period. The absolute increase in NF3 emissions in China over 2017–2020, 0.65 (0.57–0.74) Gg yr–1is comparable to the increase in global emissions (0.63 (0.50–0.75) Gg yr–1) over the same period. We identified substantial NF3 emissions in the Pearl and Yangtze River Delta regions and Hubei Province, where well-established semiconductor industries could have contributed to NF3 emissions. Moreover, large NF3 emissions were identified in northern China, including Hebei, Henan, and Shandong Provinces. If control measures are not implemented, increasing NF3 emissions may delay China’s progress toward achieving its carbon neutrality target by 2060.

求助全文
通过发布文献求助,成功后即可免费获取论文全文。 去求助
来源期刊
Environmental Science & Technology Letters Environ.
Environmental Science & Technology Letters Environ. ENGINEERING, ENVIRONMENTALENVIRONMENTAL SC-ENVIRONMENTAL SCIENCES
CiteScore
17.90
自引率
3.70%
发文量
163
期刊介绍: Environmental Science & Technology Letters serves as an international forum for brief communications on experimental or theoretical results of exceptional timeliness in all aspects of environmental science, both pure and applied. Published as soon as accepted, these communications are summarized in monthly issues. Additionally, the journal features short reviews on emerging topics in environmental science and technology.
期刊最新文献
Issue Editorial Masthead Issue Publication Information Call for Papers for a Special Issue on “Ocean Health” First Identification of Toxic Cyclotriphosphazenes as New Pollutants Prevailing in Various Urban Environments: A Class of Widely Used Flame Retardant Electrolyte Additives in Lithium-Ion Batteries Human Internal Exposure to Rubber-Derived Chemicals – A Pilot Investigation
×
引用
GB/T 7714-2015
复制
MLA
复制
APA
复制
导出至
BibTeX EndNote RefMan NoteFirst NoteExpress
×
×
提示
您的信息不完整,为了账户安全,请先补充。
现在去补充
×
提示
您因"违规操作"
具体请查看互助需知
我知道了
×
提示
现在去查看 取消
×
提示
确定
0
微信
客服QQ
Book学术公众号 扫码关注我们
反馈
×
意见反馈
请填写您的意见或建议
请填写您的手机或邮箱
已复制链接
已复制链接
快去分享给好友吧!
我知道了
×
扫码分享
扫码分享
Book学术官方微信
Book学术文献互助
Book学术文献互助群
群 号:481959085
Book学术
文献互助 智能选刊 最新文献 互助须知 联系我们:info@booksci.cn
Book学术提供免费学术资源搜索服务,方便国内外学者检索中英文文献。致力于提供最便捷和优质的服务体验。
Copyright © 2023 Book学术 All rights reserved.
ghs 京公网安备 11010802042870号 京ICP备2023020795号-1