2019 年中国臭氧浓度时空演变特征及人类活动影响研究

IF 1.4 4区 地球科学 Q3 GEOCHEMISTRY & GEOPHYSICS Acta Geochimica Pub Date : 2024-04-30 DOI:10.1007/s11631-024-00695-1
Yongchun Wang, Wang Zhang, Yu’an Liu, Yazhu Wang, Yuting Fu, Zhaohui Feng, Lingqing Wang
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引用次数: 0

摘要

臭氧(O3)污染对人类健康、植被发展和生态环境有着深远的影响,因此成为全球学术界研究的重点。近年来,中国的臭氧污染呈持续上升趋势,臭氧成为唯一一种浓度持续上升而不下降的常规污染物。本研究对2019年中国367个城市的臭氧浓度进行了定量分析,考察了臭氧浓度的空间自相关性和局地聚集性,并研究了人类活动因素与臭氧浓度之间的多种关系。O3的季节波动呈现 "M型 "模式,冬季浓度最高,夏季浓度最低。O3 污染中心向东南方向迁移,高浓度区域沿东部沿海逐渐南移。此外,O3 浓度与人口密度、公路货运量和工业排放物呈很强的正相关,表明人类活动、汽车尾气排放和工业生产是产生 O3 的重要因素。研究结果为中国城市 O3 的特征、成因和发生机制提供了全面的信息,可为全球政府部门制定 O3 污染防治策略提供参考。
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Study on the spatial and temporal evolutionary characteristics of ozone concentration and the impact of human activities in China in 2019

Ozone (O3) pollution has a profound impact on human health, vegetation development, and the ecological environment, making it a critical focus of global academic research. In recent years, O3 pollution in China has been on a steady rise, with ozone emerging as the sole conventional pollutant to consistently increase in concentration without any decline. This study conducted a quantitative analysis of O3 concentrations across 367 Chinese cities in 2019, examining spatial autocorrelation and local clustering of O3 levels, and investigated the diverse relationships between human activity factors and O3 concentration. The seasonal fluctuation of O3 exhibited the “M-type” pattern, with peak concentrations in winter and the lowest levels in summer. The center of O3 pollution migrated southeastward, with the area of highest concentration progressively shifting south along the eastern coast. Moreover, O3 concentration showed a strong positive correlation with population density, road freight volume, and industrial emissions, suggesting that human activities, vehicle emissions, and industrial operations are significant contributors to O3 production. The results provide comprehensive information on the characteristics, causes, and occurrence mechanism of O3 in Chinese cities that can be utilized by global government departments to formulate strategies to prevent and control O3 pollution.

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来源期刊
Acta Geochimica
Acta Geochimica GEOCHEMISTRY & GEOPHYSICS-
CiteScore
2.80
自引率
6.20%
发文量
1134
期刊介绍: Acta Geochimica serves as the international forum for essential research on geochemistry, the science that uses the tools and principles of chemistry to explain the mechanisms behind major geological systems such as the Earth‘s crust, its oceans and the entire Solar System, as well as a number of processes including mantle convection, the formation of planets and the origins of granite and basalt. The journal focuses on, but is not limited to the following aspects: • Cosmochemistry • Mantle Geochemistry • Ore-deposit Geochemistry • Organic Geochemistry • Environmental Geochemistry • Computational Geochemistry • Isotope Geochemistry • NanoGeochemistry All research articles published in this journal have undergone rigorous peer review. In addition to original research articles, Acta Geochimica publishes reviews and short communications, aiming to rapidly disseminate the research results of timely interest, and comprehensive reviews of emerging topics in all the areas of geochemistry.
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