Maria Alessia Vecchio , Marta Costas-Rodríguez , Laura Caiazzo , Federica Bruschi , Kasper Hobin , Frank Vanhaecke , Marco Grotti
{"title":"通过对穹顶 C 的雪进行锶同位素分析了解过去六十年沉积在南极洲的矿物尘埃的来源","authors":"Maria Alessia Vecchio , Marta Costas-Rodríguez , Laura Caiazzo , Federica Bruschi , Kasper Hobin , Frank Vanhaecke , Marco Grotti","doi":"10.1016/j.atmosenv.2024.120850","DOIUrl":null,"url":null,"abstract":"<div><div>The strontium (Sr) concentration and <sup>87</sup>Sr/<sup>86</sup>Sr isotope ratio have been determined in 132 snow pit samples collected at Dome C, on the East Antarctic Plateau, corresponding to the period 1958–2019, and in 12 surface snow samples collected at the same site in 2016–2017. The average Sr concentration was 8.1 ± 5.7 pg g<sup>−1</sup> (mean ± SD) in snow pit samples and 10.1 ± 8.0 pg g<sup>−1</sup> (mean ± SD) in surface snow, without any significant temporal trend. The <sup>87</sup>Sr/<sup>86</sup>Sr isotope ratio showed small variations (<0.15%), with an average <sup>87</sup>Sr/<sup>86</sup>Sr value of 0.7094 ± 0.0010 (mean ± SD) in snow pit and 0.7103 ± 0.0004 (mean ± SD) in surface snow samples. These results seem to suggest that no change in the source(s) of mineral dust has occurred throughout the period investigated.</div><div>Comparison of the <sup>87</sup>Sr/<sup>86</sup>Sr isotope ratio of the snow samples with those of potential source areas suggests that the mineral dust reaching the East Antarctic plateau over the last decades is of a mixed origin, with a contribution from Patagonia and one or more other source(s) having a more radiogenic Sr isotopic signature, with a major fraction coming from South Australia.</div></div>","PeriodicalId":250,"journal":{"name":"Atmospheric Environment","volume":"338 ","pages":"Article 120850"},"PeriodicalIF":4.2000,"publicationDate":"2024-09-29","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"","citationCount":"0","resultStr":"{\"title\":\"Provenance of mineral dust deposited on Antarctica over the last sixty years by strontium isotopic analysis of snow from Dome C\",\"authors\":\"Maria Alessia Vecchio , Marta Costas-Rodríguez , Laura Caiazzo , Federica Bruschi , Kasper Hobin , Frank Vanhaecke , Marco Grotti\",\"doi\":\"10.1016/j.atmosenv.2024.120850\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"<div><div>The strontium (Sr) concentration and <sup>87</sup>Sr/<sup>86</sup>Sr isotope ratio have been determined in 132 snow pit samples collected at Dome C, on the East Antarctic Plateau, corresponding to the period 1958–2019, and in 12 surface snow samples collected at the same site in 2016–2017. The average Sr concentration was 8.1 ± 5.7 pg g<sup>−1</sup> (mean ± SD) in snow pit samples and 10.1 ± 8.0 pg g<sup>−1</sup> (mean ± SD) in surface snow, without any significant temporal trend. The <sup>87</sup>Sr/<sup>86</sup>Sr isotope ratio showed small variations (<0.15%), with an average <sup>87</sup>Sr/<sup>86</sup>Sr value of 0.7094 ± 0.0010 (mean ± SD) in snow pit and 0.7103 ± 0.0004 (mean ± SD) in surface snow samples. These results seem to suggest that no change in the source(s) of mineral dust has occurred throughout the period investigated.</div><div>Comparison of the <sup>87</sup>Sr/<sup>86</sup>Sr isotope ratio of the snow samples with those of potential source areas suggests that the mineral dust reaching the East Antarctic plateau over the last decades is of a mixed origin, with a contribution from Patagonia and one or more other source(s) having a more radiogenic Sr isotopic signature, with a major fraction coming from South Australia.</div></div>\",\"PeriodicalId\":250,\"journal\":{\"name\":\"Atmospheric Environment\",\"volume\":\"338 \",\"pages\":\"Article 120850\"},\"PeriodicalIF\":4.2000,\"publicationDate\":\"2024-09-29\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Atmospheric Environment\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://www.sciencedirect.com/science/article/pii/S1352231024005259\",\"RegionNum\":2,\"RegionCategory\":\"环境科学与生态学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q2\",\"JCRName\":\"ENVIRONMENTAL SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Atmospheric Environment","FirstCategoryId":"93","ListUrlMain":"https://www.sciencedirect.com/science/article/pii/S1352231024005259","RegionNum":2,"RegionCategory":"环境科学与生态学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q2","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
Provenance of mineral dust deposited on Antarctica over the last sixty years by strontium isotopic analysis of snow from Dome C
The strontium (Sr) concentration and 87Sr/86Sr isotope ratio have been determined in 132 snow pit samples collected at Dome C, on the East Antarctic Plateau, corresponding to the period 1958–2019, and in 12 surface snow samples collected at the same site in 2016–2017. The average Sr concentration was 8.1 ± 5.7 pg g−1 (mean ± SD) in snow pit samples and 10.1 ± 8.0 pg g−1 (mean ± SD) in surface snow, without any significant temporal trend. The 87Sr/86Sr isotope ratio showed small variations (<0.15%), with an average 87Sr/86Sr value of 0.7094 ± 0.0010 (mean ± SD) in snow pit and 0.7103 ± 0.0004 (mean ± SD) in surface snow samples. These results seem to suggest that no change in the source(s) of mineral dust has occurred throughout the period investigated.
Comparison of the 87Sr/86Sr isotope ratio of the snow samples with those of potential source areas suggests that the mineral dust reaching the East Antarctic plateau over the last decades is of a mixed origin, with a contribution from Patagonia and one or more other source(s) having a more radiogenic Sr isotopic signature, with a major fraction coming from South Australia.
期刊介绍:
Atmospheric Environment has an open access mirror journal Atmospheric Environment: X, sharing the same aims and scope, editorial team, submission system and rigorous peer review.
Atmospheric Environment is the international journal for scientists in different disciplines related to atmospheric composition and its impacts. The journal publishes scientific articles with atmospheric relevance of emissions and depositions of gaseous and particulate compounds, chemical processes and physical effects in the atmosphere, as well as impacts of the changing atmospheric composition on human health, air quality, climate change, and ecosystems.