封面：利用光化学驱动的二氧化碳释放和溶剂再生技术实现高能效的直接空气捕集（ChemPlusChem 10/2024）

IF 3 4区化学 Q2 CHEMISTRY, MULTIDISCIPLINARY ChemPlusChem Pub Date : 2024-10-15 DOI:10.1002/cplu.202481001

Dr. Uvinduni I. Premadasa, Dr. Benjamin Doughty, Dr. Radu Custelcean, Dr. Ying-Zhong Ma

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引用次数: 0

摘要

利用蜕变态光酸（mPAH）进行光化学驱动的二氧化碳释放始于反式-顺式光异构化，随后结构发生变化，质子转移到二氧化碳捕获产生的碳酸氢根离子上。mPAH可逆地调节溶液pH值，为在环境条件下利用丰富的太阳能而不是热能实现高效节能的按需二氧化碳释放和溶剂回收提供了新途径。更多详情，请参阅 Uvinduni I. Premadasa、Ying-Zhong Ma 及合作者的概念报告（DOI: 10.1002/cplu.202300713）。

本文章由计算机程序翻译，如有差异，请以英文原文为准。

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Front Cover: Towards Energy-Efficient Direct Air Capture with Photochemically-Driven CO2 Release and Solvent Regeneration (ChemPlusChem 10/2024)

Photochemically driven CO₂ release using metastable-state photoacids (mPAH) initiates with trans–cis photoisomerization, followed by subsequent structural changes and proton transfer to bicarbonate ions resulting from CO₂ capture. mPAHs reversibly regulate solution pH, providing a new avenue towards energy efficient on-demand CO₂ release and solvent regeneration under ambient conditions using abundant solar energy instead of heat. More details can be found in the Concept by Uvinduni I. Premadasa, Ying-Zhong Ma, and co-workers (DOI: 10.1002/cplu.202300713).

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来源期刊

ChemPlusChem CHEMISTRY, MULTIDISCIPLINARY-

CiteScore

5.90

自引率

0.00%

发文量

200

审稿时长

1 months

期刊介绍： ChemPlusChem is a peer-reviewed, general chemistry journal that brings readers the very best in multidisciplinary research centering on chemistry. It is published on behalf of Chemistry Europe, an association of 16 European chemical societies. Fully comprehensive in its scope, ChemPlusChem publishes articles covering new results from at least two different aspects (subfields) of chemistry or one of chemistry and one of another scientific discipline (one chemistry topic plus another one, hence the title ChemPlusChem). All suitable submissions undergo balanced peer review by experts in the field to ensure the highest quality, originality, relevance, significance, and validity.