{"title":"液体溶剂直接空气捕集的成本和二氧化碳去除率随环境条件而变化","authors":"Patrick Shorey, Ahmed Abdulla","doi":"10.1038/s43247-024-01773-1","DOIUrl":null,"url":null,"abstract":"Emission trajectories produced by integrated assessment models increasingly suggest that gigatonnes of carbon removal will be required to stabilize atmospheric greenhouse gas concentrations at safe levels. This can be accomplished using the direct air capture of carbon dioxide, among other technologies. Process models of these systems assume that they would operate at standard ambient temperature and pressure, when capture rates vary with ambient conditions, including temperature, relative humidity, and other factors. Here, we build an open-source model of a liquid solvent direct air capture technology and analyze its capture performance as a function of hourly varying ambient environmental conditions across Canada. We find that, in the cool climate considered, capture performance is degraded due to both varying environmental conditions and the intermittent operation that could result. Our findings can be used to calibrate policy and investment decisions, and to support engineers in making operational design choices. In Canada, the performance of liquid-solvent direct air capture plants degrades in cold climates, while in warm climates, the performance is boosted but requires increased use of water, according to an analysis that uses an open-source model that combines chemical processes and cost data.","PeriodicalId":10530,"journal":{"name":"Communications Earth & Environment","volume":null,"pages":null},"PeriodicalIF":8.1000,"publicationDate":"2024-10-19","publicationTypes":"Journal Article","fieldsOfStudy":null,"isOpenAccess":false,"openAccessPdf":"https://www.nature.com/articles/s43247-024-01773-1.pdf","citationCount":"0","resultStr":"{\"title\":\"Liquid solvent direct air capture’s cost and carbon dioxide removal vary with ambient environmental conditions\",\"authors\":\"Patrick Shorey, Ahmed Abdulla\",\"doi\":\"10.1038/s43247-024-01773-1\",\"DOIUrl\":null,\"url\":null,\"abstract\":\"Emission trajectories produced by integrated assessment models increasingly suggest that gigatonnes of carbon removal will be required to stabilize atmospheric greenhouse gas concentrations at safe levels. This can be accomplished using the direct air capture of carbon dioxide, among other technologies. Process models of these systems assume that they would operate at standard ambient temperature and pressure, when capture rates vary with ambient conditions, including temperature, relative humidity, and other factors. Here, we build an open-source model of a liquid solvent direct air capture technology and analyze its capture performance as a function of hourly varying ambient environmental conditions across Canada. We find that, in the cool climate considered, capture performance is degraded due to both varying environmental conditions and the intermittent operation that could result. Our findings can be used to calibrate policy and investment decisions, and to support engineers in making operational design choices. In Canada, the performance of liquid-solvent direct air capture plants degrades in cold climates, while in warm climates, the performance is boosted but requires increased use of water, according to an analysis that uses an open-source model that combines chemical processes and cost data.\",\"PeriodicalId\":10530,\"journal\":{\"name\":\"Communications Earth & Environment\",\"volume\":null,\"pages\":null},\"PeriodicalIF\":8.1000,\"publicationDate\":\"2024-10-19\",\"publicationTypes\":\"Journal Article\",\"fieldsOfStudy\":null,\"isOpenAccess\":false,\"openAccessPdf\":\"https://www.nature.com/articles/s43247-024-01773-1.pdf\",\"citationCount\":\"0\",\"resultStr\":null,\"platform\":\"Semanticscholar\",\"paperid\":null,\"PeriodicalName\":\"Communications Earth & Environment\",\"FirstCategoryId\":\"93\",\"ListUrlMain\":\"https://www.nature.com/articles/s43247-024-01773-1\",\"RegionNum\":1,\"RegionCategory\":\"地球科学\",\"ArticlePicture\":[],\"TitleCN\":null,\"AbstractTextCN\":null,\"PMCID\":null,\"EPubDate\":\"\",\"PubModel\":\"\",\"JCR\":\"Q1\",\"JCRName\":\"ENVIRONMENTAL SCIENCES\",\"Score\":null,\"Total\":0}","platform":"Semanticscholar","paperid":null,"PeriodicalName":"Communications Earth & Environment","FirstCategoryId":"93","ListUrlMain":"https://www.nature.com/articles/s43247-024-01773-1","RegionNum":1,"RegionCategory":"地球科学","ArticlePicture":[],"TitleCN":null,"AbstractTextCN":null,"PMCID":null,"EPubDate":"","PubModel":"","JCR":"Q1","JCRName":"ENVIRONMENTAL SCIENCES","Score":null,"Total":0}
Liquid solvent direct air capture’s cost and carbon dioxide removal vary with ambient environmental conditions
Emission trajectories produced by integrated assessment models increasingly suggest that gigatonnes of carbon removal will be required to stabilize atmospheric greenhouse gas concentrations at safe levels. This can be accomplished using the direct air capture of carbon dioxide, among other technologies. Process models of these systems assume that they would operate at standard ambient temperature and pressure, when capture rates vary with ambient conditions, including temperature, relative humidity, and other factors. Here, we build an open-source model of a liquid solvent direct air capture technology and analyze its capture performance as a function of hourly varying ambient environmental conditions across Canada. We find that, in the cool climate considered, capture performance is degraded due to both varying environmental conditions and the intermittent operation that could result. Our findings can be used to calibrate policy and investment decisions, and to support engineers in making operational design choices. In Canada, the performance of liquid-solvent direct air capture plants degrades in cold climates, while in warm climates, the performance is boosted but requires increased use of water, according to an analysis that uses an open-source model that combines chemical processes and cost data.
期刊介绍:
Communications Earth & Environment is an open access journal from Nature Portfolio publishing high-quality research, reviews and commentary in all areas of the Earth, environmental and planetary sciences. Research papers published by the journal represent significant advances that bring new insight to a specialized area in Earth science, planetary science or environmental science.
Communications Earth & Environment has a 2-year impact factor of 7.9 (2022 Journal Citation Reports®). Articles published in the journal in 2022 were downloaded 1,412,858 times. Median time from submission to the first editorial decision is 8 days.